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Register a new userLinear and Non-linear Response of Lithographically Defined Plasmonic Nanoantennas
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We present numerical studies, nano-fabrication and optical characterization of bowtie nanoantennas demonstrating their superior performance with respect to the electric field enhancement as compared to other Au nanoparticle shapes. For optimized parameters, we found mean intensity enhancement factors >2300x in the feed-gap of the antenna, decreasing to 1300x when introducing a 5nm titanium adhesion layer. Using electron beam lithography we fabricated gold bowties on various substrates with feed-gaps and tip radii as small as 10nm. In polarization resolved measurement we experimentally observed a blue shift of the surface plasmon resonance from 1.72eV to 1.35eV combined with a strong modification of the electric field enhancement in the feed-gap. Under excitation with a 100fs pulsed laser source, we observed non-linear light emission arising from two-photon photoluminescence and second harmonic generation from the gold. The bowtie nanoantenna shows a high potential for outstanding conversion efficiencies and the enhancement of other optical effects which could be exploited in future nanophotonic devices.
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We report the observation of the generation and routing of single plasmons generated by localized excitons in a WSe$_2$ monolayer flake exfoliated onto lithographically defined Au-plasmonic waveguides. Statistical analysis of the position of different quantum emitters shows that they are $(3.3 pm 0.7)times$ more likely to form close to the edges of the plasmonic waveguides. By characterizing individual emitters we confirm their single-photon character via the observation of antibunching of the signal ($g^{(2)}(0) = 0.42$) and demonstrate that specific emitters couple to the modes of the proximal plasmonic waveguide. Time-resolved measurements performed on emitters close to, and far away from the plasmonic nanostructures indicate that Purcell factors up to $15 pm 3$ occur, depending on the precise location of the quantum emitter relative to the tightly confined plasmonic mode. Measurement of the point spread function of five quantum emitters relative to the waveguide with <50nm precision are compared with numerical simulations to demonstrate potential for higher increases of the coupling efficiency for ideally positioned emitters. The integration of such strain-induced quantum emitters with deterministic plasmonic routing is a step toward deep-subwavelength on-chip single quantum light sources.
Topological edge states exhibit dissipationless transport and electrically-driven topological phase transitions, making them ideal for next-generation transistors that are not constrained by Moores law. Nevertheless, their dispersion has never been probed and is often assumed to be simply linear, without any rigorous justification. Here we determine the non-linear electrical response of topological edge states in the ballistic regime and demonstrate the way this response ascertains the presence of symmetry breaking terms in the edge dispersion, such as deviations from non-linearity and tilted spin quantization axes. The non-linear response stems from discontinuities in the band occupation on either side of a Zeeman gap, and its direction is set by the spin orientation with respect to the Zeeman field. We determine the edge dispersion for several classes of topological materials and discuss experimental measurement.
Nodal-line semimetals are topological semimetals characterized by one-dimensional band-touching loops protected by the combined symmetry of inversion $mathcal{P}$ and time-reversal $mathcal{T}$ in absence of spin-orbit coupling. These nodal loops can be understood as a one-parameter family of Dirac points exhibiting the parity anomaly associated to $mathcal{P}*mathcal{T}$ symmetry. We find that the parity anomaly also appears in the non-linear optical response of these systems in an analogous way to the linear response transport. We analyze the presence of a tilting term in the Hamiltonian as an element that does not spoil $mathcal{P}*mathcal{T}$ symmetry: while it is $mathcal{P}*mathcal{T}$-symmetric, it breaks separately both $mathcal{P}$ and $mathcal{T}$ symmetries, allowing for the potential experimental observability of the linear and non-linear Hall conductivities in appropriate nodal-line semimetals.
We theoretically investigate the critical current of a thermally-biased SIS Josephson junction formed by electrodes made by different BCS superconductors. The response of the device is analyzed as a function of the asymmetry parameter, $r=T_{c_1} /T_{c_2}$. We highlight the appearance of jumps in the critical current of an asymmetric junction, namely, when $r eq1$. In fact, in such case at temperatures at which the BCS superconducting gaps coincide, the critical current suddenly increases or decreases. In particular, we thoroughly discuss the counterintuitively behaviour of the critical current, which increases by enhancing the temperature of one lead, instead of monotonically reducing. In this case, we found that the largest jump of the critical current is obtained for moderate asymmetries, $rsimeq3$. In view of these results, the discussed behavior can be speculatively proposed as a temperature-based threshold single-photon detector with photon-counting capabilities, which operates non-linearly in the non-dissipative channel.
Nanophotonic (nanoplasmonic) structures confine, guide, and concentrate light on the nanoscale. Advancement of nanophotonics critically depends on active nanoscale control of these phenomena. Localized control of the insulator and metallic phases of vanadium dioxide (VO2) would open up a universe of applications in nanophotonics via modulation of the local dielectric environment of nanophotonic structures allowing them to function as active devices. Here we show dynamic reversible control of VO2 insulator-to-metal transition (IMT) locally on the scale of 15 nm or less and control of nanoantennas, observed in the near-field for the first time. Using polarization-selective near-field imaging techniques, we monitor simultaneously the IMT in VO2 and the change of plasmons on gold infrared nanoantennas. Structured nanodomains of the metallic VO2 locally and reversibly transform infrared plasmonic dipolar antennas to monopole antennas. Fundamentally, the IMT in VO2 can be triggered on femtosecond timescale to allow ultrafast nanoscale control of optical phenomena. These unique capabilities open up exciting novel applications in active nanophotonics.
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