No Arabic abstract
Magnetic measurements have been carried out in the superconducting and normal states of the optimally doped nonmagnetic bismuthate superconductor Ba0.63K0.37BiO3. The magnetic data along with previous muSR, resistivity, and tunneling data consistently show that there is a large polaronic enhancement in the density of states and effective electron-phonon coupling constant. The first-principle calculation within the density-functional theory indicates a small electron-phonon coupling constant of about 0.3-0.4, which can only lead to about 1 K superconductivity within the conventional phonon-mediated mechanism. Remarkably, the polaronic effect increases the electron-phonon coupling constant to about 1.4, which is large enough to leads to 32 K superconductivity. The present work thus uncovers the mystery of high-temperature superconductivity in bismuthate superconductors, which will also provide important insight into the pairing mechanism of other high-temperature superconductors.
The spin dynamics of an optimally doped YBa2Cu3O7 (Tc = 93 K) crystal array have been investigated in a wide range of momentum and energy (Q - E) space using the time-of-flight neutron scattering method. Incommensurate spin modulation in Q is a characteristic feature, as it is in the under-doped YBa2Cu3O6.7 with a different incommensurability. A linear relationship between the incommensurability and Tc is proposed. Along with the discovery of the same incommensurability in under-doped La2-ySryCuO4, it may be a generic characteristic of the high-Tc oxide superconductor.
In the last two decades there have been tremendous attempts to built an adequate theory of high-temperature superconductivity. Most studies (including our efforts) used some model Hamiltonians with input parameters not directly related to the material. The dielectric response function of electrons in strongly correlated high-temperature superconductors is apriori unknown. Hence one has to start with the generic Hamiltonian including unscreened Coulomb and Froehlich electron-phonon interactions operating on the same scale since any ad-hoc assumption on their range and relative magnitude might fail. Using such a generic Hamiltonian I have built the analytical theory of high-temperature superconductivity in doped polar insulators predicting the critical temperature in excess of a hundred Kelvin without any adjustable parameters. The many-particle electron system is described by an analytically solvable polaronic t-Jp Hamiltonian with reduced hopping integral, t, allowed double on-site occupancy, large phonon-induced antiferromagnetic exchange, Jp >> t, and a high-temperature superconducting state of small superlight bipolarons protected from clustering.
An angle-resolved photoemission study of the scattering rate in the superconducting phase of the high-temperature superconductor LSCO with $x=0.145$ and $x=0.17$, as a function of binding energy and momentum, is presented. We observe that the scattering rate scales linearly with binding energy up to the high-energy scale $E_1sim0.4$ eV. The scattering rate is found to be strongly anisotropic, with a minimum along the (0,0)-($pi,pi$) direction. A possible connection to a quantum-critical point is discussed.
We have discovered that samples of a new material produced by special processing of crystals of Sr2RuO4 (which is known to be a triplet superconductor with Tc values ~1.0-1.5K) exhibit signatures of superconductivity (zero DC resistance and expulsion of magnetic flux) at temperatures exceeding 200K. The special processing includes deposition of a silver coating and laser micromachining; Ag doping and enhanced oxygen are observed in the resultant surface layer. The transition, whether measured resistively or by magnetic field expulsion, is broad. When the transition is registered by resistive methods, the critical temperature is markedly reduced when the measuring current is increased. The resistance disappears by about 190K. The highest value of Tc registered by magneto-optical visualization is about 220K and even higher values (up to 250K) are indicated from the SQUID-magnetometer measurements.
Combined synchrotron angle-dispersive powder diffraction and micro-Raman spectroscopy are used to investigate the pressure-induced lattice instabilities that are accompanied by T$_{rm c}$ anomalies in YBa$_{rm 2}$Cu$_{rm 4}$O$_{rm 8}$, in comparison with the optimally doped YBa$_{rm 2}$Cu$_{rm 3}$O$_{rm 7-delta}$ and the non-superconducting PrBa$_{rm 2}$Cu$_{rm 3}$O$_{rm 6.92}$. In the first two superconducting systems there is a clear anomaly in the evolution of the lattice parameters and an increase of lattice disorder with pressure, that starts at $approx3.7 GPa$ as well as irreversibility that induces a hysteresis. On the contrary, in the Pr-compound the lattice parameters follow very well the expected equation of state (EOS) up to 7 GPa. In complete agreement with the structural data, the micro-Raman data of the superconducting compounds show that the energy and width of the A$_{rm g}$ phonons show anomalies at the same pressure range where the lattice parameters deviate from the EOS and the average Cu2-O$_{pl}$ bond length exhibits a strong contraction and correlate with the non-linear pressure dependence of T$_{rm c}$. This is not the case for the non superconducting Pr sample, clearly indicating a connection with the charge carriers. It appears that the cuprates close to optimal doping are at the edge of lattice instability.