No Arabic abstract
Femtosecond electron bunches with keV energies and eV energy spread are needed by condensed matter physicists to resolve state transitions in carbon nanotubes, molecular structures, organic salts, and charge density wave materials. These semirelativistic electron sources are not only of interest for ultrafast electron diffraction, but also for electron energy-loss spectroscopy and as a seed for x-ray FELs. Thus far, the output energy spread (hence pulse duration) of ultrafast electron guns has been limited by the achievable electric field at the surface of the emitter, which is 10 MV/m for DC guns and 200 MV/m for RF guns. A single-cycle THz electron gun provides a unique opportunity to not only achieve GV/m surface electric fields but also with relatively low THz pulse energies, since a single-cycle transform-limited waveform is the most efficient way to achieve intense electric fields. Here, electron bunches of 50 fC from a flat copper photocathode are accelerated from rest to tens of eV by a microjoule THz pulse with peak electric field of 72 MV/m at 1 kHz repetition rate. We show that scaling to the readily-available GV/m THz field regime would translate to monoenergetic electron beams of ~100 keV.
A vacuum autoresonance accelerator scheme for electrons, which employs terahertz radiation and currently available magnetic fields, is suggested. Based on numerical simulations, parameter values, which could make the scheme experimentally feasible, are identified and discussed.
Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes, existing techniques are limited by the achievable electron probe bunch length, charge, and timing jitter. We present the first experimental demonstration of pump-probe UED with THz-driven compression and time-stamping that enable UED probes with unprecedented temporal resolution. This technique utilizes two counter-propagating quasi-single-cycle THz pulses generated from two OH-1 organic crystals coupled into an optimized THz compressor structure. Ultrafast dynamics of photoexcited bismuth films show an improved temporal resolution from 178 fs down to 85 fs when the THz-compressed UED probes are used with no time-stamping correction. Furthermore, we use a novel time-stamping technique to reveal transient oscillations in the dynamical response of THz-excited single-crystal gold films previously inaccessible by standard UED, achieving a time-stamped temporal resolution down to 5 fs.
Ultrashort photoemitted electron bunches can provide high electron currents within sub-picosecond timeframes, enabling time-resolved investigations of ultrafast physical processes with nanoscale resolution. Non-resonant conductive nanotips are typically employed to realize nanoscale photoelectron sources with high brightness. However, such emitters require complex non-scalable fabrication procedures featuring poor reproducibility. Planar resonant antennas fabricated via photolithography have been recently investigated, also because of their superior field enhancement properties. Nevertheless, the electron emission from these structures is parallel to the substrate plane, which limits their practical use as electron sources. In this work, we present an innovative out-of-plane, resonant nanoantenna design for field-driven photoemission enabled by high-resolution 3D printing. Numerical and experimental evidences demonstrate that gold-coated, terahertz resonant nanocones provide large local electric fields at their apex, automatically ensuring out-of-plane coherent electron emission and acceleration. We show that the resonant structures can be conveniently arranged in an array form, for a further significant electron extraction enhancement via a collective terahertz response. Remarkably, such collective behaviour can also be harvested to boost photoemission from an individual nano-source. Our approach opens the path for a new generation of photocathodes that can be reproducibly fabricated and designed at will, significantly relaxing the requirement for intense terahertz drivers.
A technique is proposed to generate attosecond pulse trains of radiation from a Free-Electron Laser amplifier. The optics-free technique synthesises a comb of longitudinal modes by applying a series of spatio-temporal shifts between the co-propagating radiation and electron bunch in the FEL. The modes may be phase-locked by modulating the electron beam energy at the mode spacing frequency. Three-dimensional simulations demonstrate the generation of a train of 400as pulses at giga-watt power levels evenly spaced by 2.5fs at a wavelength of 124 Angstrom. In the X-ray at wavelength 1.5 Angstrom, trains of 23as pulses evenly spaced by 150as and of peak power up to 6GW are predicted.
We disclose an unanticipated link between plasmonics and nonlinear frequency down-conversion in laser-induced gas-plasmas. For two-color femtosecond pump pulses, a plasmonic resonance is shown to broaden the terahertz emission spectra significantly. We identify the resonance as a leaky mode, which contributes to the emission spectra whenever electrons are excited along a direction where the plasma size is smaller than the plasma wavelength. As a direct consequence, such resonances can be controlled by changing the polarization properties of elliptically-shaped driving laser pulses. Both, experimental results and 3D Maxwell consistent simulations confirm that a significant terahertz pulse shortening and spectral broadening can be achieved by exploiting the transverse driving laser beam shape as an additional degree of freedom.