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Register a new userBreakdown of the Isobaric Multiplet Mass Equation for the A = 20 and 21 Multiplets
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Using the Penning trap mass spectrometer TITAN, we performed the first direct mass measurements of 20,21Mg, isotopes that are the most proton-rich members of the A = 20 and A = 21 isospin multiplets. These measurements were possible through the use of a unique ion-guide laser ion source, a development that suppressed isobaric contamination by six orders of magnitude. Compared to the latest atomic mass evaluation, we find that the mass of 21Mg is in good agreement but that the mass of 20Mg deviates by 3{sigma}. These measurements reduce the uncertainties in the masses of 20,21Mg by 15 and 22 times, respectively, resulting in a significant departure from the expected behavior of the isobaric multiplet mass equation in both the A = 20 and A = 21 multiplets. This presents a challenge to shell model calculations using either the isospin non-conserving USDA/B Hamiltonians or isospin non-conserving interactions based on chiral two- and three-nucleon forces.
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Mass measurements on radionuclides along the potassium isotope chain have been performed with the ISOLTRAP Penning trap mass spectrometer. For 35K T1/2=178ms) to 46K (T1/2=105s) relative mass uncertainties of 2x10-8 and better have been achieved. The accurate mass determination of 35K (dm=0.54keV) has been exploited to test the Isobaric Multiplet Mass Equation (IMME) for the A=35, T=3/2 isospinquartet. The experimental results indicate a deviation from the generally adopted quadratic form.
Masses of $^{52}$Co, $^{52}$Co$^m$, $^{52}$Fe, $^{52}$Fe$^m$, and $^{52}$Mn have been measured with the JYFLTRAP double Penning trap mass spectrometer. Of these, $^{52}$Co and $^{52}$Co$^m$ have been experimentally determined for the first time and found to be more bound than predicted by extrapolations. The isobaric multiplet mass equation for the $T=2$ quintet at $A=52$ has been studied employing the new mass values. No significant breakdown (beyond the $3sigma$ level) of the quadratic form of the IMME was observed ($chi^2/n=2.4$). The cubic coefficient was 6.0(32) keV ($chi^2/n=1.1$). The excitation energies for the isomer and the $T=2$ isobaric analogue state in $^{52}$Co have been determined to be 374(13) keV and 2922(13) keV, respectively. The $Q$ value for the proton decay from the $19/2^-$ isomer in $^{53}$Co has been determined with an unprecedented precision, $Q_{p} = 1558.8(17)$ keV. The proton separation energies of $^{52}$Co and $^{53}$Ni relevant for the astrophysical rapid proton capture process have been experimentally determined for the first time. end{abstract}
The observed mass excesses of analog nuclear states with the same mass number $A$ and isospin $T$ can be used to test the isobaric multiplet mass equation (IMME), which has, in most cases, been validated to a high degree of precision. A recent measurement [Kankainen et al., Phys. Rev. C 93 041304(R) (2016)] of the ground-state mass of $^{31}$Cl led to a substantial breakdown of the IMME for the lowest $A = 31, T = 3/2$ quartet. The second-lowest $A = 31, T = 3/2$ quartet is not complete, due to uncertainties associated with the identity of the $^{31}$S member state. Using a fast $^{31}$Cl beam implanted into a plastic scintillator and a high-purity Ge $gamma$-ray detection array, $gamma$ rays from the $^{31}$Cl$(betagamma)$$^{31}$S sequence were measured. Shell-model calculations using USDB and the recently-developed USDE interactions were performed for comparison. Isospin mixing between the $^{31}$S isobaric analog state (IAS) at 6279.0(6) keV and a nearby state at 6390.2(7) keV was observed. The second $T = 3/2$ state in $^{31}$S was observed at $E_x = 7050.0(8)$ keV. Isospin mixing in $^{31}$S does not by itself explain the IMME breakdown in the lowest quartet, but it likely points to similar isospin mixing in the mirror nucleus $^{31}$P, which would result in a perturbation of the $^{31}$P IAS energy. USDB and USDE calculations both predict candidate $^{31}$P states responsible for the mixing in the energy region slightly above $E_x = 6400$ keV. The second quartet has been completed thanks to the identification of the second $^{31}$S $T = 3/2$ state, and the IMME is validated in this quartet.
If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$sigma$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both within 1$sigma$, while being 8 and 34 times more precise, respectively. Using the $^{29}$Mg mass excess and previous measurements of $^{29}$Cl we uncovered a cubic coefficient of $d$ = 28(7) keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of $^{28}$S and the one-neutron separation energy of $^{29}$Cl, which have both come from a single measurement. Finally, our results were compared to ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement.
We study the a, b and c coefficients of the isobaric-multiplet mass equation using a macroscopic-microscopic approach developed by P. Moeller and his collaborators in ADNDT 59, 185 (1995) and ADNDT 109-110, 1 (2016). We show that already the macroscopic part of the finite-range liquid-drop model (FRLDM) describes the general trend of the a and b coefficients relatively well, while the staggering behavior of b coefficients for doublets and quartets can be understood in terms of the difference of average proton and neutron pairing energies. The sets of isobaric masses, predicted by the full macroscopic-microscopic approaches, are used to explore the general trends of IMME coefficients up to A=100. We conclude that while the agreement for a coefficients is quite satisfactory, the global approaches have less sensitivity to predict the staggering pattern observed for b coefficients of doublets and quartets. The best set of theoretical b coefficients for multiplets up to about A=100 is used to predict masses of proton-rich nuclei based on the known experimental masses of neutron-rich mirror partners, and subsequently to investigate their one- and two-proton separation energies. The estimated position of the proton-drip line is in fair agreement with known experimental data. These masses are important for simulations of the astrophysical rp-process.
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