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Register a new userCoherent generation of nonclassical light on chip via detuned photon blockade
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The on-chip generation of non-classical states of light is a key-requirement for future optical quantum hardware. In solid-state cavity quantum electrodynamics, such non-classical light can be generated from self-assembled quantum dots strongly coupled to photonic crystal cavities. Their anharmonic strong light-matter interaction results in large optical nonlinearities at the single photon level, where the admission of a single photon into the cavity may enhance (photon-tunnelling) or diminish (photon-blockade) the probability for a second photon to enter the cavity. Here, we demonstrate that detuning the cavity and QD resonances enables the generation of high-purity non-classical light from strongly coupled systems. For specific detunings we show that not only the purity but also the efficiency of single-photon generation increases significantly, making high-quality single-photon generation by photon-blockade possible with current state-of-the-art samples.
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We report the observation of nonclassical light generated via photon blockade in a photonic crystal cavity with a strongly coupled quantum dot. By tuning the frequency of the probe laser with respect to the cavity and quantum dot resonance we can probe the system in either photon blockade or photon-induced tunneling regime. The transition from one regime to the other is confirmed by the measurement of the second order correlation that changes from anti-bunching to bunching.
Excitons in a semiconductor monolayer form a collective resonance that can reflect resonant light with extraordinarily high efficiency. Here, we investigate the nonlinear optical properties of such atomistically thin mirrors and show that finite-range interactions between excitons can lead to the generation of highly non-classical light. We describe two scenarios, in which optical nonlinearities arise either from direct photon coupling to excitons in excited Rydberg states or from resonant two-photon excitation of Rydberg excitons with finite-range interactions. The latter case yields conditions of electromagnetically induced transparency and thereby provides an efficient mechanism for single-photon switching between high transmission and reflectance of the monolayer, with a tunable dynamical timescale of the emerging photon-photon interactions. Remarkably, it turns out that the resulting high degree of photon correlations remains virtually unaffected by Rydberg-state decoherence, in excess of non-radiative decoherence observed for ground-state excitons in two-dimensional semiconductors. This robustness to imperfections suggests a promising new approach to quantum photonics at the level of individual photons.
It is shown that non-centrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered coupled microcavities. The proposed scheme exploits the unconventional photon blockade of a coherent driving field at the input of a coupled cavity system, where one of the two cavities is engineered to resonate at both fundamental and second harmonic frequencies, respectively. Remarkably, the unconventional blockade mechanism occurs with reasonably low quality factors at both harmonics, and does not require a sharp doubly-resonant condition for the second cavity, thus proving its feasibility with current semiconductor technology.
We performed quantum manipulations of the multi-level spin system S=5/2 of a Mn$^{2+}$ ion, by means of a two-tone pulse drive. The detuning between the excitation and readout radio frequency pulses allows one to select the number of photons involved in a Rabi oscillation as well as increase the frequency of this nutation. Thus detuning can lead to a resonant multi-photon process. Our analytical model for a two-photon process as well as a numerical generalization fit well the experimental findings, with implications in the use of multi-level spin systems as tunable solid state qubits.
In the present study, we developed a fabrication process of an electrically driven single-photon LED based on InP QDs emitting in the red spectral range, the wavelength of interest coinciding with the high efficiency window of Si APDs. A deterministic lithography technique allowed for the pre-selection of a suitable QD, here exclusively operated under electrical carrier injection. The final device was characterized under micro-electroluminescence in direct current, as well as in pulsed excitation mode. In particular, under pulsed excitation of one device, single-photon emission of a spectral line, identified as an exciton, has been observed with $g^{(2)}_mathrm{raw}(0)=0.42pm0.02$, where the non-zero $g^{(2)}$-value is mainly caused by background contribution in the spectrum and re-excitation processes due to the electrical pulse length. The obtained results constitute an important step forward in the fabrication of electrically driven single-photon sources, where deterministic lithography techniques can be used to sensibly improve the device performances. In principle, the developed process can be extended to any desired emitter wavelength above $600,mathrm{nm}$ up to the telecom bands.
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