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Register a new userProbing the dynamics of a nuclear spin bath in diamond through time-resolved central spin magnetometry
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Using fast electron spin resonance spectroscopy of a single nitrogen-vacancy defect in diamond, we demonstrate real-time readout of the Overhauser field produced by its nuclear spin environment under ambient conditions. These measurements enable narrowing the Overhauser field distribution by post-selection, corresponding to a conditional preparation of the nuclear spin bath. Correlations of the Overhauser field fluctuations are quantitatively inferred by analysing the Allan deviation over consecutive measurements. This method allows to extract the dynamics of weakly coupled nuclear spins of the reservoir.
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The quantum coherence and gate fidelity of electron spin qubits in semiconductors is often limited by noise arising from coupling to a bath of nuclear spins. Isotopic enrichment of spin-zero nuclei such as $^{28}$Si has led to spectacular improvements of the dephasing time $T_2^*$ which, surprisingly, can extend two orders of magnitude beyond theoretical expectations. Using a single-atom $^{31}$P qubit in enriched $^{28}$Si, we show that the abnormally long $T_2^*$ is due to the controllable freezing of the dynamics of the residual $^{29}$Si nuclei close to the donor. Our conclusions are supported by a nearly parameter-free modeling of the $^{29}$Si nuclear spin dynamics, which reveals the degree of back-action provided by the electron spin as it interacts with the nuclear bath. This study clarifies the limits of ergodic assumptions in analyzing many-body spin-problems under conditions of strong, frequent measurement, and provides novel strategies for maximizing coherence and gate fidelity of spin qubits in semiconductors.
The generation and manipulation of carrier spin polarization in semiconductors solely by electric fields has garnered significant attention as both an interesting manifestation of spin-orbit physics as well as a valuable capability for potential spintronics devices. One realization of these spin-orbit phenomena, the spin Hall effect (SHE), has been studied as a means of all-electrical spin current generation and spin separation in both semiconductor and metallic systems. Previous measurements of the spin Hall effect have focused on steady-state generation and time-averaged detection, without directly addressing the accumulation dynamics on the timescale of the spin coherence time. Here, we demonstrate time-resolved measurement of the dynamics of spin accumulation generated by the extrinsic spin Hall effect in a doped GaAs semiconductor channel. Using electrically-pumped time-resolved Kerr rotation, we image the accumulation, precession, and decay dynamics near the channel boundary with spatial and temporal resolution and identify multiple evolution time constants. We model these processes using time-dependent diffusion analysis utilizing both exact and numerical solution techniques and find that the underlying physical spin coherence time differs from the dynamical rates of spin accumulation and decay observed near the sample edges.
In this paper, we study the electron spin decoherence of single defects in silicon carbide (SiC) nuclear spin bath. We find that, although the natural abundance of $^{29}rm{Si}$ ($p_{rm{Si}}=4.7%$) is about 4 times larger than that of $^{13}{rm C}$ ($p_{rm{C}}=1.1%$), the electron spin coherence time of defect centers in SiC nuclear spin bath in strong magnetic field ($B>300~rm{Gauss}$) is longer than that of nitrogen-vacancy (NV) centers in $^{13}{rm C}$ nuclear spin bath in diamond. The reason for this counter-intuitive result is the suppression of heteronuclear-spin flip-flop process in finite magnetic field. Our results show that electron spin of defect centers in SiC are excellent candidates for solid state spin qubit in quantum information processing.
A phenomenological model is constructed, that captures the effects of coupling magnetic and elastic degrees of freedom, in the presence of external, stochastic perturbations, in terms of the interaction of magnetic moments with a bath, whose individual degrees of freedom cannot be resolved and only their mesoscopic properties are relevant. In the present work, the consequences of identifying the effects of dissipation as resulting from interactions with a bath of spins are explored, in addition to elastic, degrees of freedom. The corresponding stochastic differential equations are solved numerically and the moments of the magnetization are computed. The stochastic equations implicitly define a measure on the space of spin configurations, whose moments at equal times satisfy a hierarchy of deterministic, ordinary differential equations. Closure assumptions are used to truncate the hierarchy and the same moments are computed. We focus on the advantages and problems that each approach presents, for the approach to equilibrium and, in particular, the emergence of longitudinal damping.
An exact reduced dynamical map along with its operator sum representation is derived for a central spin interacting with a thermal spin environment. The dynamics of the central spin shows high sustainability of quantum traits such as coherence and entanglement in the low-temperature regime. However, for sufficiently high temperature and when the number of bath particles approaches the thermodynamic limit, this feature vanishes and the dynamics closely mimics Markovian evolution. The properties of the long-time-averaged state and the trapped information of the initial state for the central qubit are also investigated in detail, confirming that the nonergodicity of the dynamics can be attributed to the finite temperature and finite size of the bath. It is shown that if a certain stringent resonance condition is satisfied, the long-time-averaged state retains quantum coherence, which can have far reaching technological implications in engineering quantum devices. An exact time-local master equation of the canonical form is derived. With the help of this master equation, the nonequilibrium properties of the central spin system are studied by investigating the detailed balance condition and irreversible entropy production rate. The result reveals that the central qubit thermalizes only in the limit of very high temperature and large number of bath spins.
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