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Nonequilibrium Brownian motion beyond the effective temperature

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 Publication date 2014
  fields Physics
and research's language is English




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The condition of thermal equilibrium simplifies the theoretical treatment of fluctuations as found in the celebrated Einsteins relation between mobility and diffusivity for Brownian motion. Several recent theories relax the hypothesis of thermal equilibrium resulting in at least two main scenarios. With well separated timescales, as in aging glassy systems, equilibrium Fluctuation-Dissipation Theorem applies at each scale with its own effective temperature. With mixed timescales, as for example in active or granular fluids or in turbulence, temperature is no more well-defined, the dynamical nature of fluctuations fully emerges and a Generalized Fluctuation-Dissipation Theorem (GFDT) applies. Here, we study experimentally the mixed timescale regime by studying fluctuations and linear response in the Brownian motion of a rotating intruder immersed in a vibro-fluidized granular medium. Increasing the packing fraction, the system is moved from a dilute single-timescale regime toward a denser multiple-timescale stage. Einsteins relation holds in the former and is violated in the latter. The violation cannot be explained in terms of effective temperatures, while the GFDT is able to impute it to the emergence of a strong coupling between the intruder and the surrounding fluid. Direct experimental measurements confirm the development of spatial correlations in the system when the density is increased.



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One goal of this paper is to discuss the classical definition of granular temperature as an extension of its thermodynamic equivalent and a useful concept which provides an important characterization of fluidized granular matter. Following a review of some basic concepts and techniques (with emphasis on fundamental issues) we present new results for a system that can exhibit strong violations of equipartition, yet is amenable to description by classical granular hydrodynamics, namely a binary granular gas mixture. A second goal of this article is to present a result that pertains to dense granular and molecular solids alike, namely the existence of a correction to the elastic energy which is related to the heat flux in the equations of continuum mechanics. The latter is of the same (second) order in the strain as the elastic energy. Although recent definitions of temperatures for granular matter, glasses and other disordered many-body systems are not within the scope of this article we do make several general comments on this subject in the closing section.
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