We have demonstrated a direct frequency comparison between two $^{87}{rm Sr}$ lattice clocks operated in intercontinentally separated laboratories in real time. Two-way satellite time and frequency transfer technique based on the carrier phase was employed for a direct comparison with a baseline of 9 000 km between Japan and Germany. A clock comparison was achieved for 83 640 s resulting in a fractional difference of $(1.1pm1.6) times 10^{-15}$, where the statistical part is the biggest contribution to the uncertainty. This measurement directly confirms the agreement of the two optical clocks on an intercontinental scale.
Fiber-based remote comparison of $^{87}$Sr lattice clocks in 24 km distant laboratories is demonstrated. The instability of the comparison reaches $5times10^{-16}$ over an averaging time of 1000 s, which is two orders of magnitude shorter than that of conventional satellite links and is limited by the instabilities of the optical clocks. By correcting the systematic shifts that are predominated by the differential gravitational redshift, the residual fractional difference is found to be $(1.0pm7.3)times10^{-16}$, confirming the coincidence between the two clocks. The accurate and speedy comparison of distant optical clocks paves the way for a future optical redefinition of the second.
Progress in realizing the SI second had multiple technological impacts and enabled to further constraint theoretical models in fundamental physics. Caesium microwave fountains, realizing best the second according to its current definition with a relative uncertainty of 2-4x10^(-16), have already been superseded by atomic clocks referenced to an optical transition, both more stable and more accurate. Are we ready for a new definition of the second? Here we present an important step in this direction: our system of five clocks connects with an unprecedented consistency the optical and the microwave worlds. For the first time, two state-of-the-art strontium optical lattice clocks are proven to agree within their accuracy budget, with a total uncertainty of 1.6x10^(-16). Their comparison with three independent caesium fountains shows a degree of reproducibility henceforth solely limited at the level of 3.1x10^(-16) by the best realizations of the microwave-defined second.
We propose a space-based gravitational wave detector consisting of two spatially separated, drag-free satellites sharing ultra-stable optical laser light over a single baseline. Each satellite contains an optical lattice atomic clock, which serves as a sensitive, narrowband detector of the local frequency of the shared laser light. A synchronized two-clock comparison between the satellites will be sensitive to the effective Doppler shifts induced by incident gravitational waves (GWs) at a level competitive with other proposed space-based GW detectors, while providing complementary features. The detected signal is a differential frequency shift of the shared laser light due to the relative velocity of the satellites, and the detection window can be tuned through the control sequence applied to the atoms internal states. This scheme enables the detection of GWs from continuous, spectrally narrow sources, such as compact binary inspirals, with frequencies ranging from ~3 mHz - 10 Hz without loss of sensitivity, thereby bridging the detection gap between space-based and terrestrial optical interferometric GW detectors. Our proposed GW detector employs just two satellites, is compatible with integration with an optical interferometric detector, and requires only realistic improvements to existing ground-based clock and laser technologies.
We developed an all-optical link system for making remote comparisons of two distant ultra-stable optical clocks. An optical carrier transfer system based on a fiber interferometer was employed to compensate the phase noise accumulated during the propagation through a fiber link. Transfer stabilities of $2times10^{-15}$ at 1 second and $4times10^{-18}$ at 1000 seconds were achieved in a 90-km link. An active polarization control system was additionally introduced to maintain the transmitted light in an adequate polarization, and consequently, a stable and reliable comparison was accomplished. The instabilities of the all-optical link system, including those of the erbium doped fiber amplifiers (EDFAs) which are free from phase-noise compensation, were below $2times10^{-15}$ at 1 second and $7times10^{-17}$ at 1000 seconds. The system was available for the direct comparison of two distant $^{87}$Sr lattice clocks via an urban fiber link of 60 km. This technique will be essential for the measuring the reproducibility of optical frequency standards.
Electrometry is performed using Rydberg states to evaluate the quadratic Stark shift of the $5s^2$ $^1textrm{S}_0-5s5p$ $^3textrm{P}_0$ clock transition in strontium. By measuring the Stark shift of the highly excited $5s75d;^1textrm{D}_2$ state using electromagnetically induced transparency, we characterize the electric field with sufficient precision to provide tight constraints on the systematic shift to the clock transition. Using the theoretically derived, and experimentally verified, polarizability for this Rydberg state we can measure the residual field with an uncertainty well below $1 textrm{V} textrm{m}^{-1}$. This resolution allows us to constrain the fractional frequency uncertainty of the quadratic Stark shift of the clock transition to $2times10^{-20}$.