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Register a new userExcitonic Bose-Einstein condensation in Ta2NiSe5 above room temperature
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We show that finite temperature variational cluster approximation (VCA) calculations on an extended Falicov-Kimball model can reproduce angle-resolved photoemission spectroscopy (ARPES) results on Ta2NiSe5 across a semiconductor-to-semiconductor structural phase transition at 325 K. We demonstrate that the characteristic temperature dependence of the flat-top valence band observed by ARPES is reproduced by the VCA calculation on the realistic model for an excitonic insulator only when the strong excitonic fluctuation is taken into account. The present calculations indicate that Ta2NiSe5 falls in the Bose-Einstein condensation regime of the excitonic insulator state.
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Using the band structure calculation and mean-field analysis of the derived three-chain Hubbard model with phonon degrees of freedom, we discuss the origin of the orthorhombic-to-monoclinic phase transition of the layered chalcogenide Ta$_2$NiSe$_5$. We show that the Bose-Einstein condensation of excitonic electron-hole pairs cooperatively induces the instability of the phonon mode at momentum $qrightarrow 0$ in the quasi-one-dimensional Ta-NiSe-Ta chain, resulting in the structural phase transition of the system. The calculated single-particle spectra reproduce the deformation of the band structure observed in the angle-resolved photoemission spectroscopy experiment.
We present a novel experimental approach to Bose-Einstein condensation by increasing the particle number of the system at almost constant temperature. In particular the emergence of a new condensate is observed in multi-component F=1 spinor condensates of 87-Rb. Furthermore we develop a simple rate-equation model for multi-component BEC thermodynamics at finite temperature which well reproduces the measured effects.
The excitonic insulator is an intriguing correlated electron phase formed of condensed excitons. A promising candidate is the small band gap semiconductor Ta2NiSe5. Here we investigate the quasiparticle and coherent phonon dynamics in Ta2NiSe5 in a time resolved pump probe experiment. Using the models originally developed by Kabanov et al. for superconductors, we show that the materials intrinsic gap can be described as almost temperature independent for temperatures up to about 250 K to 275 K. This behavior supports the existence of the excitonic insulator state in Ta2NiSe5. The onset of an additional temperature dependent component to the gap above these temperatures suggests that the material is located in the BEC-BCS crossover regime. Furthermore, we show that this state is very stable against strong photoexcitation, which reveals that the free charge carriers are unable to effectively screen the attractive Coulomb interaction between electrons and holes, likely due to the quasi one-dimensional structure of Ta2NiSe5.
In a recent paper cite{Radu}, Radu textit{et al.} report experimental results they claim to support Bose-Einstein condensation (BEC) of magnons in Cs$_2$CuCl$_4$. It is true that an experimentally measured critical power law scaling exponent in agreement with the BEC universality class would support the realization of a BEC in magnetic systems that order as a canted antiferromagnet. It can be shown, however, that the claim of Radu {it et al.} is overstated in this instance, because their determination of the critical exponent $phi$ relies on a model-dependent theoretical approximation to the critical field $H_{textrm{c1}}$ for which the associated errors are neglected. We show that when these errors are included, the uncertainty in the obtained exponent is so large that the available experimental data cannot be used to differentiate between contending universality classes.
We report evidence for the existence of a supercurrent of magnons in a magnon Bose-Einstein condensate prepared in a room temperature yttrium-iron-garnet magnetic film and subject to a thermal gradient. The magnon condensate is formed in a parametrically populated magnon gas, and its temporal evolution is studied by time-, frequency- and wavector-resolved Brillouin light scattering spectroscopy. It has been found that local heating in the focal point of a probing laser beam enhances the temporal decrease in the density of the freely evolving magnon condensate after the termination of the pumping pulse, but it does not alter the relaxation dynamics of the gaseous magnon phase. This phenomenon is understood as the appearance of a magnon supercurrent within the condensate due to a temperature- and, consequently, magnetisation-gradient induced phase gradient in the condensate wave function.
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