No Arabic abstract
We provide the first evidence for coherence and Rabi oscillations of spin-solitons pinned by the local breaking of translational symmetry in isotropic Heisenberg chains (simple antiferromagnetic-N{e}el or spin-Peierls).We show that these correlated spin systems made of hundreds of coupled spin bear an overall spin S=1/2 and can be manipulated as a single spin. This is clearly contrary to all known spin-qubits which are paramagnetic centres, highly diluted to prevent decoherence. These results offer an alternative approach for spin-qubits paving the way for the implementation of a new type of quantum computer.
The dissipative response of a quantum system upon a time-dependent drive can be exploited as a probe of its geometric and topological properties. In this work, we explore the implications of such phenomena in the context of two-dimensional gases subjected to a uniform magnetic field. It is shown that a filled Landau level exhibits a quantized circular dichroism, which can be traced back to its underlying non-trivial topology. Based on selection rules, we find that this quantized circular dichroism can be suitably described in terms of Rabi oscillations, whose frequencies satisfy simple quantization laws. Moreover, we discuss how these quantized dissipative responses can be probed locally, both in the bulk and at the boundaries of the quantum Hall system. This work suggests alternative forms of topological probes in quantum systems based on circular dichroism.
We report on multiple photon monochromatic quantum oscillations (Rabi oscillations) observed by pulsed EPR (Electron Paramagnetic Resonance) of Mn$^{2+}$ (S=5/2) impurities in MgO. We find that when the microwave magnetic field is similar or large than the anisotropy splitting, the Rabi oscillations have a spectrum made of many frequencies not predicted by the S=1/2 Rabi model. We show that these new frequencies come from multiple photon coherent manipulation of the multi-level spin impurity. We develop a model based on the crystal field theory and the rotating frame approximation, describing the observed phenomenon with a very good agreement.
The quasi two-dimensional Mott insulator $alpha$-RuCl$_3$ is proximate to the sought-after Kitaev quantum spin liquid (QSL). In a layer of $alpha$-RuCl$_3$ on graphene the dominant Kitaev exchange is further enhanced by strain. Recently, quantum oscillation (QO) measurements of such $alpha$-RuCl$_3$ / graphene heterostructures showed an anomalous temperature dependence beyond the standard Lifshitz-Kosevich (LK) description. Here, we develop a theory of anomalous QO in an effective Kitaev-Kondo lattice model in which the itinerant electrons of the graphene layer interact with the correlated magnetic layer via spin interactions. At low temperatures a heavy Fermi liquid emerges such that the neutral Majorana fermion excitations of the Kitaev QSL acquire charge by hybridising with the graphene Dirac band. Using ab-initio calculations to determine the parameters of our low energy model we provide a microscopic theory of anomalous QOs with a non-LK temperature dependence consistent with our measurements. We show how remnants of fractionalized spin excitations can give rise to characteristic signatures in QO experiments.
Finite-temperature spin transport in the quantum Heisenberg spin chain is known to be superdiffusive, and has been conjectured to lie in the Kardar-Parisi-Zhang (KPZ) universality class. Using a kinetic theory of transport, we compute the KPZ coupling strength for the Heisenberg chain as a function of temperature, directly from microscopics; the results agree well with density-matrix renormalization group simulations. We establish a rigorous quantum-classical correspondence between the giant quasiparticles that govern superdiffusion and solitons in the classical continuous Landau-Lifshitz ferromagnet. We conclude that KPZ universality has the same origin in classical and quantum integrable isotropic magnets: a finite-temperature gas of low-energy classical solitons.
Coulomb spin liquids are topological magnetic states obeying an emergent Gauss law. Little distinction has been made between different kinds of Coulomb liquids. Here we show how a series of distinct Coulomb liquids can be generated straightforwardly by varying the constraints on a classical spin system. This leads to pair creation, and coalescence, of topological defects of an underlying vector field. The latter makes higher-rank spin liquids, of recent interest in the context of fracton theories, with attendant multi-fold pinch points in the structure factor, appear naturally. New Coulomb liquids with an abundance of pinch points also arise. We thus establish a new and general route to uncovering exotic Coulomb liquids, via the manipulation of topological defects in momentum space.