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Register a new userIpopv2: Photoionization of Ni XIV -- a test case
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Several years ago, M. Asplund and coauthors (2004) proposed a revision of the Solar composition. The use of this new prescription for Solar abundances in standard stellar models generated a strong disagreement between the predictions and the observations of Solar observables. Many claimed that the Standard Solar Model (SSM) was faulty, and more specifically the opacities used in such models. As a result, activities around the stellar opacities were boosted. New experiments (J. Bailey at Sandia on Z-Pinch, The OPAC consortium at LULI200) to measure directly absorbtion coefficients have been realized or are underway. Several theoretical groups (CEA-OPAS, Los Alamos Nat. Lab., CEA-SCORCG, The Opacity Project - The Iron Project (IPOPv2)) have started new sets of calculations using different approaches and codes. While the new results seem to confirm the good quality of the opacities used in SSM, it remains important to improve and complement the data currently available. We present recent results in the case of the photoionization cross sections for Ni XIV (Ni13+ ) from IPOPv2 and possible implications on stellar modelling.
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We have used an electron beam ion trap to measure electron-density-diagnostic line-intensity ratios for extreme ultraviolet lines from F XII, XIII, and XIV at wavelengths of 185-205 255-276 Angstroms. These ratios can be used as density diagnostics for astrophysical spectra and are especially relevant to solar physics. We found that density diagnostics using the Fe XIII 196.53/202.04 and the Fe XIV 264.79/274.21 and 270.52A/274.21 line ratios are reliable using the atomic data calculated with the Flexible Atomic Code. On the other hand, we found a large discrepancy between the FAC theory and experiment for the commonly used Fe XII (186.85 + 186.88)/195.12 line ratio. These FAC theory calculations give similar results to the data tabulated in CHIANTI, which are commonly used to analyze solar observations. Our results suggest that the discrepancies seen between solar coronal density measurements using the Fe XII (186.85 + 186.88)/195.12 and Fe XIII 196.54/202.04 line ratios are likely due to issues with the atomic calculations for Fe XII.
Opacity is an important ingredient of the evolution of stars. The calculation of opacity coefficients is complicated by the fact that the plasma contains partially ionized heavy ions that contribute to opacity dominated by H and He. Up to now, the astrophysical community has greatly benefited from the work of the contributions of Los Alamos [1], Livermore [2] and the Opacity Project (OP) [3]. However unexplained differences of up to 50% in the radiative forces and Rosseland mean values for Fe have been noticed for conditions corresponding to stellar envelopes. Such uncertainty has a real impact on the understanding of pulsating stellar envelopes, on the excitation of modes, and on the identification of the mode frequencies. Temperature and density conditions equivalent to those found in stars can now be produced in laboratory experiments for various atomic species. Recently the photo-absorption spectra of nickel and iron plasmas have been measured during the LULI 2010 campaign, for temperatures between 15 and 40 eV and densities of ~3 mg/cm3. A large theoretical collaboration, the OPAC, has been formed to prepare these experiments. We present here the set of opacity calculations performed by eight different groups for conditions relevant to the LULI 2010 experiment and to astrophysical stellar envelope conditions.
A comprehensive study of high-accuracy photoionization cross sections is carried out using the relativistic Breit-Pauli R-matrix (BPRM) method for (hnu + Fe XVII --> Fe XVIII + e). Owing to its importance in high-temperature plasmas the calculations cover a large energy range, particularly the myriad photoexciation-of-core (PEC) resonances including the n = 3 levels not heretofore considered. The calculations employ a close coupling wave function expansion of 60 levels of the core ion Fe XVIII ranging over a wide energy range of nearly 900 eV between the n = 2 and n = 3 levels. Strong coupling effects due to dipole transition arrays 2p^5 --> 2p^4 (3s,3d) manifest themselves as large PEC resonances throughout this range, and enhance the effective photoionization cross sections orders of magnitude above the background. Comparisons with the erstwhile Opacity Project (OP) and other previous calculations shows that the currently available cross sections considerably underestimate the bound-free cross sections. A level-identification scheme is used for spectroscopic designation of the 454 bound fine structure levels of Fe XVII. Level-specific photoionization cross sections are computed for all levels. In addition, partial cross sections for leaving the core ion Fe XVII in the ground state are also obtained. These results should be relevant to modeling of astrophysical and laboratory plasma sources requiring (i) photoionization rates, (ii) extensive non-local-thermodynamic-equilibrium models, (iii) total unified electron-ion recombination rates including radiative and dielectronic recombination, and (iv) plasma opacities. We particularly examine PEC and non-PEC resonance strengths and emphasize their expanded role to incorporate inner-shell excitations for improved opacities, as shown by the computed monochromatic opacity of Fe XVII.
We demonstrate that the angular distribution of photoelectrons from a strongly polarizable target exposed to a laser field can deviate noticeably from the prediction of conventional theory. Even within the dipole-photon approximation the profile of distribution is modified due to the action of the field of alternating dipole moment induced at the residue by the laser field. This effect, being quite sensitive to the dynamic polarizability of the residue and to its geometry, depends also on the intensity and frequency of the laser field. Numerical results, presented for sodium cluster anions, demonstrate that dramatic changes to the profile occur for the photon energies in vicinities of the plasmon resonances, where the effect is enhanced due to the increase in the residue polarizability. Strong modifications of the characteristics of a single-photon ionization process can be achieved by applying laser fields of comparatively low intensities $I_0 sim10^{10}-10^{11}$ W/cm$^2$.
We consider three recent large-scale calculations for the radiative and electron-impact excitation data of N IV, carried out with different methods and codes. The scattering calculations employed the relativistic Dirac $R$-matrix (DARC) method, the intermediate coupling frame transformation (ICFT) $R$-matrix method, and the B-spline $R$-matrix (BSR) method. These are all large-scale scattering calculations with well-tested and sophisticated codes, which use the same set of target states. One concern raised in previous literature is related to the increasingly large discrepancies in the effective collision strengths between the three sets of calculations for increasingly weak and/or high-lying transitions. We have built three model ions and calculated the intensities of all the main spectral lines in this ion. We have found that, despite such large differences, excellent agreement (to within $pm$~20%) exists between all the spectroscopically-relevant line intensities. This provides confidence in the reliability of the calculations for plasma diagnostics. We have used the differences in the radiative and excitation rates amongst the three sets of calculations to obtain a measure of the uncertainty in each rate. Using a Monte Carlo approach, we have shown how these uncertainties affect the main theoretical ratios which are used to measure electron densities and temperatures.
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