Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userA structural evaluation of the tungsten isotopes via thermal neutron capture
365
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
Total radiative thermal neutron-capture $gamma$-ray cross sections for the $^{182,183,184,186}$W isotopes were measured using guided neutron beams from the Budapest Research Reactor to induce prompt and delayed $gamma$ rays from elemental and isotopically-enriched tungsten targets. These cross sections were determined from the sum of measured $gamma$-ray cross sections feeding the ground state from low-lying levels below a cutoff energy, E$_{rm crit}$, where the level scheme is completely known, and continuum $gamma$ rays from levels above E$_{rm crit}$, calculated using the Monte Carlo statistical-decay code DICEBOX. The new cross sections determined in this work for the tungsten nuclides are: $sigma_{0}(^{182}{rm W}) = 20.5(14)$ b and $sigma_{11/2^{+}}(^{183}{rm W}^{m}, 5.2 {rm s}) = 0.177(18)$ b; $sigma_{0}(^{183}{rm W}) = 9.37(38)$ b and $sigma_{5^{-}}(^{184}{rm W}^{m}, 8.33 mu{rm s}) = 0.0247(55)$ b; $sigma_{0}(^{184}{rm W}) = 1.43(10)$ b and $sigma_{11/2^{+}}(^{185}{rm W}^{m}, 1.67 {rm min}) = 0.0062(16)$ b; and, $sigma_{0}(^{186}{rm W}) = 33.33(62)$ b and $sigma_{9/2^{+}}(^{187}{rm W}^{m}, 1.38 mu{rm s}) = 0.400(16)$ b. These results are consistent with earlier measurements in the literature. The $^{186}$W cross section was also independently confirmed from an activation measurement, following the decay of $^{187}$W, yielding values for $sigma_{0}(^{186}{rm W})$ that are consistent with our prompt $gamma$-ray measurement. The cross-section measurements were found to be insensitive to choice of level density or photon strength model, and only weakly dependent on E$_{rm crit}$. Total radiative-capture widths calculated with DICEBOX showed much greater model dependence, however, the recommended values could be reproduced with selected model choices. The decay schemes for all tungsten isotopes were improved in these analyses.
rate research
Read More
The indication for the alpha decay of 180-W with a half-life T1/2=1.1+0.8-0.4(stat)+-0.3(syst)x10^18 yr has been observed for the first time with the help of the super-low background 116-CdWO_4 crystal scintillators. In conservative approach the lower limit on half-life of 180-W has been established as T1/2>0.7x10^18 yr at 90% C.L. Besides, new T1/2 bounds were set for alpha decay of 182-W, 183-W, 184-W and 186-W at the level of 10^20 yr.
50% of the heavy element abundances are produced via slow neutron capture reactions in different stellar scenarios. The underlying nucleosynthesis models need the input of neutron capture cross sections. One of the fundamental signatures for active nucleosynthesis in our galaxy is the observation of long-lived radioactive isotopes, such as $^{60}$Fe with a half-life of $2.60times10^6$ yr. To reproduce this $gamma$-activity in the universe, the nucleosynthesis of $^{60}$Fe has to be understood reliably. A $^{60}$Fe sample produced at the Paul-Scherrer-Institut was activated with thermal and epithermal neutrons at the research reactor at the Johannes Gutenberg-Universitat Mainz. The thermal neutron capture cross section has been measured for the first time to $sigma_{text{th}}=0.226 (^{+0.044}_{-0.049})$ b. An upper limit of $sigma_{text{RI}} < 0.50$ b could be determined for the resonance integral. An extrapolation towards the astrophysicaly interesting energy regime between $kT$=10 keV and 100 keV illustrates that the s-wave part of the direct capture component can be neglected.
We have measured the $gamma$-ray energy spectrum from the thermal neutron capture, ${}^{157}$Gd$(n,gamma){}^{158}$Gd, on an enriched $^{157}$Gd target (Gd$_{2}$O$_{3}$) in the energy range from 0.11 MeV up to about 8 MeV. The target was placed inside the germanium spectrometer of the ANNRI detector at J-PARC and exposed to a neutron beam from the Japan Spallation Neutron Source (JSNS). Radioactive sources ($^{60}$Co, $^{137}$Cs, and $^{152}$Eu) and the reaction $^{35}$Cl($n$,$gamma$) were used to determine the spectrometers detection efficiency for $gamma$ rays at energies from 0.3 to 8.5 MeV. Using a Geant4-based Monte Carlo simulation of the detector and based on our data, we have developed a model to describe the $gamma$-ray spectrum from the thermal ${}^{157}$Gd($n$,$gamma$) reaction. While we include the strength information of 15 prominent peaks above 5 MeV and associated peaks below 1.6 MeV from our data directly into the model, we rely on the theoretical inputs of nuclear level density and the photon strength function of ${}^{158}$Gd to describe the continuum $gamma$-ray spectrum from the ${}^{157}$Gd($n$,$gamma$) reaction. Our model combines these two components. The results of the comparison between the observed $gamma$-ray spectra from the reaction and the model are reported in detail.
An extended investigation of the low-spin structure of the $^{65}$Ni nucleus was performed at the Institut Laue-Langevin, Grenoble, via the neutron capture reaction $^{64}$Ni(n,$gamma$)$^{65}$Ni, using the FIPPS HPGe array. The level scheme of $^{65}$Ni was significantly expanded, with 2 new levels and 87 newly found transitions. Angular correlation analyses were also performed, allowing us to assign spins and parities for a number of states, and to determine multipolarity mixing ratios for selected $gamma$ transitions. The low-energy part of the experimental level scheme (up to about 1.4 MeV) was compared with Monte Carlo Shell Model calculations, which predict spherical shapes for all states, apart from the 9/2$^+$ and the second excited 1/2$^-$ states of oblate deformation.
Gamow-Teller (GT) strength distributions (B(GT)) in electron-capture (EC) daughters stemming from the parent ground state are computed with the shell-model in the full pf-shell space, with quasi-particle random-phase approximation (QRPA) in the formalism of Krumlinde and Moller and with an Approximate Method (AM) for assigning an effective B(GT). These are compared to data available from decay and charge-exchange (CE) experiments across titanium isotopes in the pf-shell from A=43 to A=62, the largest set available for any chain of isotopes in the pf-shell. The present study is the first to examine B(GT) and the associated EC rates across a particular chain of isotopes with the purpose of examining rate sensitivities as neutron number increases. EC rates are also computed for a wide variety of stellar electron densities and temperatures providing concise estimates of the relative size of rate sensitivities for particular astrophysical scenarios. This work underscores the astrophysical motivation for CE experiments in inverse kinematics for nuclei away from stability at the luminosities of future Radioactive Ion Beam Facilities.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
