No Arabic abstract
We present a comprehensive analysis of critical behavior in the driven-dissipative Bose condensation transition in three spatial dimensions. Starting point is a microscopic description of the system in terms of a many-body quantum master equation, where coherent and driven-dissipative dynamics occur on an equal footing. An equivalent Keldysh real time functional integral reformulation opens up the problem to a practical evaluation using the tools of quantum field theory. In particular, we develop a functional renormalization group approach to quantitatively explore the universality class of this stationary non-equilibrium system. Key results comprise the emergence of an asymptotic thermalization of the distribution function, while manifest non-equilibrium properties are witnessed in the response properties in terms of a new, independent critical exponent. Thus the driven-dissipative microscopic nature is seen to bear observable consequences on the largest length scales. The absence of two symmetries present in closed equilibrium systems - underlying particle number conservation and detailed balance, respectively - is identified as the root of this new non-equilibrium critical behavior. Our results are relevant for broad ranges of open quantum systems on the interface of quantum optics and many-body physics, from exciton-polariton condensates to cold atomic gases.
Solid state quantum condensates can differ from other condensates, such as Helium, ultracold atomic gases, and superconductors, in that the condensing quasiparticles have relatively short lifetimes, and so, as for lasers, external pumping is required to maintain a steady state. In this chapter we present a non-equilibrium path integral approach to condensation in a dissipative environment and apply it to microcavity polaritons, driven out of equilibrium by coupling to multiple baths, describing pumping and decay. Using this, we discuss the relation between non-equilibrium polariton condensation, lasing, and equilibrium condensation.
We investigate formation of Bose-Einstein condensates under non-equilibrium conditions using numerical simulations of the three-dimensional Gross-Pitaevskii equation. For this, we set initial random weakly nonlinear excitations and the forcing at high wave numbers, and study propagation of the turbulent spectrum toward the low wave numbers. Our primary goal is to compare the results for the evolving spectrum with the previous results obtained for the kinetic equation of weak wave turbulence. We demonstrate existence of a regime for which good agreement with the wave turbulence results is found in terms of the main features of the previously discussed self-similar solution. In particular, we find a reasonable agreement with the low-frequency and the high-frequency power-law asymptotics of the evolving solution, including the anomalous power-law exponent $x^* approx 1.24$ for the three-dimensional waveaction spectrum. We also study the regimes of very weak turbulence, when the evolution is affected by the discreteness of the Fourier space, and the strong turbulence regime when emerging condensate modifies the wave dynamics and leads to formation of strongly nonlinear filamentary vortices.
Coherence is a defining feature of quantum condensates. These condensates are inherently multimode phenomena and in the macroscopic limit it becomes extremely difficult to resolve populations of individual modes and the coherence between them. In this work we demonstrate non-equilibrium Bose-Einstein condensation (BEC) of photons in a sculpted dye-filled microcavity, where threshold is found for $8pm 2$ photons. With this nanocondensate we are able to measure occupancies and coherences of individual energy levels of the bosonic field. Coherence of individual modes generally increases with increasing photon number, but at the breakdown of thermal equilibrium we observe multimode-condensation phase transitions wherein coherence unexpectedly decreases with increasing population, suggesting that the photons show strong inter-mode phase or number correlations despite the absence of a direct nonlinearity. Experiments are well-matched to a detailed non-equilibrium model. We find that microlaser and Bose-Einstein statistics each describe complementary parts of our data and are limits of our model in appropriate regimes, which informs the debate on the differences between the two.
We report the formation of Bose-Einstein condensates into non-equilibrium states. Our condensates are much longer than equilibrium condensates with the same number of atoms, show strong phase fluctuations, and have a dynamical evolution similar to that of quadrupole shape oscillations of regular condensates. The condensates emerge in elongated traps as the result of local thermalization when the nucleation time is short compared to the axial oscillation time. We introduce condensate focusing as a powerful method to extract the phase-coherence length of Bose-Einstein condensates.
We derive a theoretical model which describes Bose-Einstein condensation in an open driven-dissipative system. It includes external pumping of a thermal reservoir, finite life time of the condensed particles and energy relaxation. The coupling between the reservoir and the condensate is described with semi-classical Boltzmann rates. This results in a dissipative term in the Gross-Pitaevskii equation for the condensate, which is proportional to the energy of the elementary excitations of the system. We analyse the main properties of a condensate described by this hybrid Boltzmann Gross-Pitaevskii model, namely, dispersion of the elementary excitations, bogolon distribution function, first order coherence, dynamic and energetic stability, drag force created by a disorder potential. We find that the dispersion of the elementary excitations of a condensed state fulfils the Landau criterion of superfluidity. The condensate is dynamically and energetically stable as longs it moves at a velocity smaller than the speed of excitations. First order spatial coherence of the condensate is found to decay exponentially in 1D and with a power law in 2D, similarly with the case of conservative systems. The coherence lengths are found to be longer due to the finite life time of the condensate excitations. We compare these properties with the ones of a condensate described by the popular diffusive models in which the dissipative term is proportional to the local condensate density. In the latter, the dispersion of excitations is diffusive which as soon as the condensate is put into motion implies finite mechanical friction and can lead to an energetic instability.