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Register a new userHigh resolution photoassociation spectroscopy of the $^{6}$Li$_2$ $A(1^1Sigma_u^+)$ state
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We present spectroscopic measurements of seven vibrational levels $v=29-35$ of the $A(1^1Sigma_u^+)$ excited state of Li$_2$ molecules by the photoassociation of a degenerate Fermi gas of $^6$Li atoms. The absolute uncertainty of our measurements is $pm 0.00002$ cm$^{-1}$ ($pm 600$ kHz) and we use these new data to further refine an analytic potential for this state. This work provides high accuracy photo-association resonance locations essential for the eventual high resolution mapping of the $X(1^1Sigma_g^+)$ state enabling further improvements to the s-wave scattering length determination of Li and enabling the eventual creation of ultra-cold ground state $^6$Li$_2$ molecules.
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We present experimental observations of seven vibrational levels $v=20-26$ of the $1^{3}Sigma_{g}^{+}$ excited state of Li$_2$ molecules by the photoassociation (PA) of a degenerate Fermi gas of $^6$Li atoms. For each vibrational level, we resolve the rotational structure using a Feshbach resonance to enhance the PA rates from p-wave collisions. We also, for the first time, determine the spin-spin and spin-rotation interaction constants for this state. The absolute uncertainty of our measurements is $pm 0.00002$ cm$^{-1}$ ($pm 600$ kHz). We use these new data to further refine an analytic potential for this state.
Using new experimental measurements of photoassociation resonances near the $^1mathrm{S}_0 rightarrow phantom{ }^3mathrm{P}_1$ intercombination transition in $^{84}$Sr and $^{86}$Sr, we present an updated study into the mass-scaling behavior of bosonic strontium dimers. A previous mass-scaling model [Borkowski et al., Phys. Rev. A 90, 032713 (2014)] was able to incorporate a large number of photoassociation resonances for $^{88}$Sr, but at the time only a handful of resonances close to the dissociation limit were known for $^{84}$Sr and $^{86}$Sr. In this work, we perform a more thorough measurement of $^{84}$Sr and $^{86}$Sr bound states, identifying multiple new resonances at deeper binding energies out to $E/h=-5$ GHz. We also identify several previously measured resonances that cannot be experimentally reproduced and provide alternative binding energies instead. With this improved spectrum, we develop a mass-scaled model that reproduces the observed binding energies of $^{86}$Sr and $^{88}$Sr to within 1 MHz. In order to accurately reproduce the deeper bound states, our model includes a second $1_u$ channel and more faithfully reproduces the depth of the potential. As determined by the previous mass-scaling study, $^{84}$Sr $0_u^+$ levels are strongly perturbed by the avoided crossing between the $^1mathrm{S}_0 + phantom{ }^3mathrm{P}_1$ $0_u^+$ $(^3Pi_u)$ and $^1mathrm{S}_0 + phantom{ }^1mathrm{D}_2$ $0_u^+$ $(^1Sigma_u^+)$ potential curves and therefore are not included in this mass-scaled model, but are accurately reproduced using an isotope-specific model with slightly different quantum defect parameters. In addition, the optical lengths of the $^{84}$Sr $0_u^+, u=-2$ to $ u=-5$ states are measured and compared to numerical estimates to characterize their use as optical Feshbach resonances.
We theoretically evaluate the feasibility to form magnetically-tunable Feshbach molecules in collisions between fermionic $^6$Li atoms and bosonic metastable $^{174}$Yb($^3$P$_2$) atoms. In contrast to the well-studied alkali-metal atom collisions, collisions with meta-stable atoms are highly anisotropic. Our first-principle coupled-channel calculation of these collisions reveals the existence of broad Feshbach resonances due to the combined effect of anisotropic-molecular and atomic-hyperfine interactions. In order to fit our predictions to the specific positions of experimentally-observed broad resonance structures cite{Deep2015} we optimized the shape of the short-range potentials by direct least-square fitting. This allowed us to identify the dominant resonance by its leading angular momentum quantum numbers and describe the role of collisional anisotropy in the creation and broadening of this and other resonances.
We perform photoassociation spectroscopy in an ultracold $^{23}$Na-$^6$Li mixture to study the $c^3Sigma^+$ excited triplet molecular potential. We observe 50 vibrational states and their substructure to an accuracy of 20 MHz, and provide line strength data from photoassociation loss measurements. An analysis of the vibrational line positions using near-dissociation expansions and a full potential fit is presented. This is the first observation of the $c^3Sigma^+$ potential, as well as photoassociation in the NaLi system.
We report the high resolution photoassociation (PA) spectroscopy of a $^{87}Rb$ Bose-Einstein condensate (BEC) to excited molecular states near the dissociation limit of $5P_{1/2} +5S_{1/2}$ by optical Bragg scattering. Since the detection of optical Bragg scattering in BEC has a high signal-noise ratio, we obtain the high resolution PA spectrum of excited molecular states in the range of $pm1$ GHz near the dissociation limit of $5P_{1/2} +5S_{1/2}$. We compare the results with the conventional method of trap loss and show that the results agree each other very well. Many interesting phenomena of excited molecular states are observed, such as light-induced frequency shift and the anomalous strong bound molecular lines at the atomic transition from $|F=1rangle$ to $|F^{prime}=2rangle$. The observed excited molecular states in the range of $pm1$ GHz near the dissociation limit of $5P_{1/2} +5S_{1/2}$ are never reported before, which will help to further improve the long range bound state models near the dissociation limit.
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