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Register a new userCross-Section Measurements of the 86Kr(g,n) Reaction to Probe the s-Process Branching at 85Kr
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We have carried out photodisintegration cross-section measurements on 86Kr using monoenergetic photon beams ranging from the neutron separation energy, S_n = 9.86 MeV, to 13 MeV. We combine our experimental 86Kr(g,n)85Kr cross section with results from our recent 86Kr(g,g) measurement below the neutron separation energy to obtain the complete nuclear dipole response of 86Kr. The new experimental information is used to predict the neutron capture cross section of 85Kr, an important branching point nucleus on the abundance flow path during s-process nucleosynthesis. Our new and more precise 85Kr(n,g)86Kr cross section allows to produce more precise predictions of the 86Kr abundance from s-process models. In particular, we find that the models of the s-process in asymptotic giant branch stars of mass < 1.5 Msun, where the 13C neutron source burns convectively rather than radiatively, represent a possible solution for the highest 86Kr/82Kr ratios observed in meteoritic stardust SiC grains.
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An experimental method to determine the (n,g) cross section of short-living s-process branching points using data of the inverse (g,n) reaction is presented. The method was used to observe the branching point nucleus 95Zr because the elemental abundance patterns corresponding to this branching point cannot be reproduced by full stellar models and a possible error source is the neutron capture cross section of 95Zr. The analysis of the experiment is still under progress, we will outline the current status in this manuscript.
The doubly-magic nucleus $^{16}$O has a small neutron capture cross section of just a few tens of microbarn in the astrophysical energy region. Despite of this, $^{16}$O plays an important role as neutron poison in the astrophysical slow neutron capture ($s$) process due to its high abundance. We present in this paper a re-evaluation of the available experimental data for $^{16}$O($n,gamma$)$^{17}$O and derive a new recommendation for the Maxwellian-averaged cross sections (MACS) between $kT$= 5$-$100 keV. Our new recommendations are lower up to $kT$= 60 keV compared to the previously recommended values but up to 14% higher at $kT$= 100 keV. We explore the impact of this different energy dependence on the weak $s$-process during core helium- ($kT$= 26 keV) and shell carbon burning ($kT$= 90 keV) in massive stars where $^{16}$O is the most abundant isotope.
The neutron capture cross section of 14C is of relevance for several nucleosynthesis scenarios such as inhomogeneous Big Bang models, neutron induced CNO cycles, and neutrino driven wind models for the r process. The 14C(n,g) reaction is also important for the validation of the Coulomb dissociation method, where the (n,g) cross section can be indirectly obtained via the time-reversed process. So far, the example of 14C is the only case with neutrons where both, direct measurement and indirect Coulomb dissociation, have been applied. Unfortunately, the interpretation is obscured by discrepancies between several experiments and theory. Therefore, we report on new direct measurements of the 14C(n,g) reaction with neutron energies ranging from 20 to 800 keV.
We present a new measurement of the $alpha$-spectroscopic factor ($S_alpha$) and the asymptotic normalization coefficient (ANC) for the 6.356 MeV 1/2$^+$ subthreshold state of $^{17}$O through the $^{13}$C($^{11}$B, $^{7}$Li)$^{17}$O transfer reaction and we determine the $alpha$-width of this state. This is believed to have a strong effect on the rate of the $^{13}$C($alpha$, $n$)$^{16}$O reaction, the main neutron source for {it slow} neutron captures (the $s$-process) in asymptotic giant branch (AGB) stars. Based on the new width we derive the astrophysical S-factor and the stellar rate of the $^{13}$C($alpha$, $n$)$^{16}$O reaction. At a temperature of 100 MK our rate is roughly two times larger than that by citet{cau88} and two times smaller than that recommended by the NACRE compilation. We use the new rate and different rates available in the literature as input in simulations of AGB stars to study their influence on the abundances of selected $s$-process elements and isotopic ratios. There are no changes in the final results using the different rates for the $^{13}$C($alpha$, $n$)$^{16}$O reaction when the $^{13}$C burns completely in radiative conditions. When the $^{13}$C burns in convective conditions, as in stars of initial mass lower than $sim$2 $M_sun$ and in post-AGB stars, some changes are to be expected, e.g., of up to 25% for Pb in our models. These variations will have to be carefully analyzed when more accurate stellar mixing models and more precise observational constraints are available.
At the n_TOF experiment at CERN a dedicated single-crystal chemical vapor deposition (sCVD) Diamond Mosaic-Detector has been developed for (n,$alpha$) cross-section measurements. The detector, characterized by an excellent time and energy resolution, consists of an array of 9 sCVD diamond diodes. The detector has been characterized and a cross-section measurement has been performed for the $^{59}$Ni(n,$alpha$)$^{56}$Fe reaction in 2012. The characteristics of the detector, its performance and the promising preliminary results of the experiment are presented.
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