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Register a new userCoulomb-assisted cavity feeding in the non-resonant optical emission from a quantum dot
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Recent experiments have demonstrated that for a quantum dot in an optical resonator off-resonant cavity mode emission can occur even for detunings of the order of 10 meV. We show that Coulomb mediated Auger processes based on additional carriers in delocalized states can facilitate this far off-resonant emission. Using a novel theoretical approach for a non-perturbative treatment of the Auger-assisted quantum-dot carrier recombination, we present numerical calculations of the far off-resonant cavity feeding rate and cavity mean photon number confirming efficient coupling at higher densities of carriers in the delocalized states. In comparison to fast Auger-like intraband scattering processes, we find a reduced overall efficiency of Coulomb-mediated interband transitions due the required electron-hole correlations for the recombination processes.
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We demonstrate a method of tuning a semiconductor quantum dot (QD) onto resonance with a cavity mode all-optically. We use a system comprised of two evanescently coupled cavities containing a single QD. One resonance of the coupled cavity system is used to generate a cavity enhanced optical Stark shift, enabling the QD to be resonantly tuned to the other cavity mode. A twenty-seven fold increase in photon emission from the QD is measured when the off-resonant QD is Stark shifted into the cavity mode resonance, which is attributed to radiative enhancement of the QD. A maximum tuning of 0.06 nm is achieved for the QD at an incident power of 88 {mu}W.
We present a medium-dependent quantum optics approach to describe the influence of electron-acoustic phonon coupling on the emission spectra of a strongly coupled quantum-dot cavity system. Using a canonical Hamiltonian for light quantization and a photon Green function formalism, phonons are included to all orders through the dot polarizability function obtained within the independent Boson model. We derive simple user-friendly analytical expressions for the linear quantum light spectrum, including the influence from both exciton and cavity-emission decay channels. In the regime of semiconductor cavity-QED, we study cavity emission for various exciton-cavity detunings and demonstrate rich spectral asymmetries as well as cavity-mode suppression and enhancement effects. Our technique is nonperturbative, and non-Markovian, and can be applied to study photon emission from a wide range of semiconductor quantum dot structures, including waveguides and coupled cavity arrays. We compare our theory directly to recent and apparently puzzling experimental data for a single site-controlled quantum dot in a photonic crystal cavity and show good agreement as a function of cavity-dot detuning and as a function of temperature.
We present a theoretical model for the dynamics of an electron that gets trapped by means of decoherence and quantum interference in the central quantum dot (QD) of a semiconductor nanoring (NR) made of five QDs, between 100 K and 300 K. The electrons dynamics is described by a master equation with a Hamiltonian based on the tight-binding model, taking into account electron-LO phonon interaction (ELOPI). Based on this configuration, the probability to trap an electron with no decoherence is almost 27%. In contrast, the probability to trap an electron with decoherence is 70% at 100 K, 63% at 200 K and 58% at 300 K. Our model provides a novel method of trapping an electron at room temperature.
We experimentally investigate the non-resonant feeding of photons into the optical mode of a zero dimensional nanocavity by quantum dot multiexciton transitions. Power dependent photoluminescence measurements reveal a super-linear power dependence of the mode emission, indicating that the emission stems from multiexcitons. By monitoring the temporal evolution of the photoluminescence spectrum, we observe a clear anticorrelation of the mode and single exciton emission; the mode emission quenches as the population in the system reduces towards the single exciton level whilst the intensity of the mode emission tracks the multi-exciton transitions. Our results lend strong support to a recently proposed mechanism mediating the strongly non-resonant feeding of photons into the cavity mode.
We compare the photoluminescence spectrum of an indium arsenide (InAs) quantum dot (QD) that is strongly coupled to a photonic crystal cavity under above band excitation (ABE) and quasi-resonant excitation (QRE). We show that off-resonant cavity feeding, which manifests itself in a bare cavity emission peak at the strong coupling point, is suppressed by as much as 40% under QRE relative to ABE. We attribute this suppression to a reduced probability of QD charging because electrons and holes are created in pairs inside the QD. We investigate the pump power dependence of the cavity feeding and show that, below saturation, the ratio of the bare cavity emission to polariton emission for ABE is independent of pump power, while for QRE there is linear pump power dependence. These results suggest that the biexciton plays an important role in cavity feeding for QRE.
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