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Register a new userPhoton correlations from ultra-strong optical nonlinearities
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We study the full field and frequency filtered output photon statistics of a resonator in thermal equilibrium with a bath and containing an arbitrarily large quartic nonlinearity. According to the general theory of photodetection, we derive general input-output relations valid for the ultra-anharmonic regime, where the nonlinearity becomes comparable to the energy of the resonator, and show how the emission properties are modified as compared to the generally assumed simple anharmonic regime. We analyse the impact of the nonlinearity on the full statistics of the emission and its spectral properties. In particular we derive a semi-analytical expression for the frequency resolved two-photon correlations or two-photon spectrum of the system in terms of the master equation coefficients and density matrix. This provides a very clear insight into the level structure and emission possibilities of the system.
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We propose a cavity QED scheme to enable cross-phase modulation between two arbitrarily weak classical fields in the optical domain, using organic molecular photoswitches as a disordered intracavity nonlinear medium. We show that a long-lived vibrational Raman coherence between the $cis$ and $trans$ isomer states of the photoswitch can be exploited to establish the phenomenon of vacuum-induced transparency (VIT) in high-quality microcavities. We exploit this result to derive an expression for the cross-phase modulation signal and demonstrate that it is possible to surpass the detection limit imposed by absorption losses, even in the presence of strong natural energetic and orientational disorder in the medium. Possible applications of the scheme include the development of organic nanophotonic devices for all-optical switching with low photon numbers.
Strong and ultra-strong light-matter coupling are remarkable phenomena of quantum electrodynamics occurring when the interaction between a matter excitation and the electromagnetic field cannot be described by usual perturbation theory. This is generally achieved by coupling an excitation with large oscillator strength to the confined electromagnetic mode of an optical microcavity. In this work we demonstrate that strong/ultra-strong coupling can also take place in the absence of optical confinement. We have studied the non-perturbative spontaneous emission of collective excitations in a dense two-dimensional electron gas that superradiantly decays into free space. By using a quantum model based on the input-output formalism, we have derived the linear optical properties of the coupled system and demonstrated that its eigenstates are mixed light-matter particles, like in any system displaying strong or ultra-strong light-matter interaction. Moreover, we have shown that in the ultra-strong coupling regime, i.e. when the radiative broadening is comparable to the matter excitation energy, the commonly used rotating-wave and Markov approximations yield unphysical results. Finally, the input-output formalism has allowed us to prove that Kirchhoffs law, describing thermal emission properties, applies to our system in all the light-matter coupling regimes considered in this work.
We propose a superconducting circuit comprising a dc-SQUID with mechanically compliant arm embedded in a coplanar microwave cavity that realizes an optomechanical system with a degenerate or non-degenerate parametric interaction generated via the dynamical Casimir effect. For experimentally feasible parameters, this setup is capable of reaching the single-photon, ultra-strong coupling regime, while simultaneously possessing a parametric coupling strength approaching the renormalized cavity frequency. This opens up the possibility of observing the interplay between these two fundamental nonlinearities at the single-photon level.
With the introduction of superconducting circuits into the field of quantum optics, many novel experimental demonstrations of the quantum physics of an artificial atom coupled to a single-mode light field have been realized. Engineering such quantum systems offers the opportunity to explore extreme regimes of light-matter interaction that are inaccessible with natural systems. For instance the coupling strength $g$ can be increased until it is comparable with the atomic or mode frequency $omega_{a,m}$ and the atom can be coupled to multiple modes which has always challenged our understanding of light-matter interaction. Here, we experimentally realize the first Transmon qubit in the ultra-strong coupling regime, reaching coupling ratios of $g/omega_{m}=0.19$ and we measure multi-mode interactions through a hybridization of the qubit up to the fifth mode of the resonator. This is enabled by a qubit with 88% of its capacitance formed by a vacuum-gap capacitance with the center conductor of a coplanar waveguide resonator. In addition to potential applications in quantum information technologies due to its small size and localization of electric fields in vacuum, this new architecture offers the potential to further explore the novel regime of multi-mode ultra-strong coupling.
We present and analyze a method where parametric (two-photon) driving of a cavity is used to exponentially enhance the light-matter coupling in a generic cavity QED setup, with time-dependent control. Our method allows one to enhance weak-coupling systems, such that they enter the strong coupling regime (where the coupling exceeds dissipative rates) and even the ultra-strong coupling regime (where the coupling is comparable to the cavity frequency). As an example, we show how the scheme allows one to use a weak-coupling system to adiabatically prepare the highly entangled ground state of the ultra-strong coupling system. The resulting state could be used for remote entanglement applications.
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