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Register a new userAn efficient biologically-inspired photocell enhanced by quantum coherence
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Artificially reproducing the biological light reactions responsible for the remarkably efficient photon-to-charge conversion in photosynthetic complexes represents a new direction for the future development of photovoltaic devices. Here, we develop such a paradigm and present a model photocell based on the nanoscale architecture of photosynthetic reaction centres that explicitly harnesses the quantum mechanical effects recently discovered in photosynthetic complexes. Quantum interference of photon absorption/emission induced by the dipole-dipole interaction between molecular excited states guarantees an enhanced light-to-current conversion and power generation for a wide range of realistic parameters, opening a promising new route for designing artificial light-harvesting devices inspired by biological photosynthesis and quantum technologies.
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We investigate surface plasmon amplification in a silver nanoparticle coupled to an externally driven three-level gain medium, and show that quantum coherence significantly enhances the generation of surface plasmons. Surface plasmon amplification by stimulated emission of radiation is achieved in the absence of population inversion on the spasing transition, which reduces the pump requirements. The coherent drive allows us to control the dynamics, and holds promise for quantum control of nanoplasmonic devices.
The understanding of the nanoscale physical properties of biomolecules and biomaterials will ultimately promote the research in the biological sciences. In this review, we focused on theory, simulation, and experiments involving nanoscale materials inspired by biological systems. Specifically, self-assembly in living and synthetic materials, bio-functionalized nanomaterials and probing techniques that use nanomaterials are discussed.
Quantum coherence, a basic feature of quantum mechanics residing in superpositions of quantum states, is a resource for quantum information processing. Coherence emerges in a fundamentally different way for nonidentical and identical particles, in that for the latter a unique contribution exists linked to indistinguishability which cannot occur for nonidentical particles. We experimentally demonstrate by an optical setup this additional contribution to quantum coherence, showing that its amount directly depends on the degree of indistinguishability and exploiting it to run a quantum phase discrimination protocol. Furthermore, the designed setup allows for simulating Fermionic particles with photons, thus assessing the role of particle statistics (Bosons or Fermions) in coherence generation and utilization. Our experiment proves that independent indistinguishable particles can supply a controllable resource of coherence for quantum metrology.
The quantum computation of electronic energies can break the curse of dimensionality that plagues many-particle quantum mechanics. It is for this reason that a universal quantum computer has the potential to fundamentally change computational chemistry and materials science, areas in which strong electron correlations present severe hurdles for traditional electronic structure methods. Here, we present a state-of-the-art analysis of accurate energy measurements on a quantum computer for computational catalysis, using improved quantum algorithms with more than an order of magnitude improvement over the best previous algorithms. As a prototypical example of local catalytic chemical reactivity we consider the case of a ruthenium catalyst that can bind, activate, and transform carbon dioxide to the high-value chemical methanol. We aim at accurate resource estimates for the quantum computing steps required for assessing the electronic energy of key intermediates and transition states of its catalytic cycle. In particular, we present new quantum algorithms for double-factorized representations of the four-index integrals that can significantly reduce the computational cost over previous algorithms, and we discuss the challenges of increasing active space sizes to accurately deal with dynamical correlations. We address the requirements for future quantum hardware in order to make a universal quantum computer a successful and reliable tool for quantum computing enhanced computational materials science and chemistry, and identify open questions for further research.
We propose a quantum metrology scheme in a cavity QED setup to achieve the Heisenberg limit. In our scheme, a series of identical two-level atoms randomly pass through and interact with a dissipative single-mode cavity. Different from the entanglement based Heisenberg limit metrology scheme, we do not need to prepare the atomic entangled states before they enter into the cavity. We show that the initial atomic coherence will induce an effective driving to the cavity field, whose steady state is an incoherent superposition of orthogonal states, with the superposition probabilities being dependent on the atom-cavity coupling strength. By measuring the average photon number of the cavity in the steady state, we demonstrate that the root-mean-square of the fluctuation of the atom-cavity coupling strength is proportional to $1/N_c^2$ ($N_c$ is the effective atom number interacting with the photon in the cavity during its lifetime). It implies that we have achieved the Heisenberg limit in our quantum metrology process. We also discuss the experimental feasibility of our theoretical proposal. Our findings may find potential applications in quantum metrology technology.
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