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Magnetization Process and Adiabatic Demagnetization of the Antiferromagnetic Spin-1/2 Heisenberg Cubic Cluster

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 Added by Strecka Jozef
 Publication date 2013
  fields Physics
and research's language is English




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A full energy spectrum of the spin-1/2 Heisenberg cubic cluster is used to investigate a low-temperature magnetization process and adiabatic demagnetization of this zero-dimensional 2x2x2 quantum spin system. It is shown that the antiferromagnetic spin-1/2 Heisenberg cube exhibits at low enough temperatures a stepwise magnetization curve with four intermediate plateaux at zero, one quarter, one half, and three quarters of the saturation magnetization. We have also found the enhanced magnetocaloric effect close to level-crossing fields that determine transitions between the intermediate plateaux.



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A full energy spectrum, magnetization and susceptibility of a spin-1/2 Heisenberg model on two edge-shared tetrahedra are exactly calculated by assuming two different coupling constants. It is shown that a ground state in zero field is either a singlet or a triplet state depending on a relative strength of both coupling constants. Low-temperature magnetization curves may exhibit three different sequences of intermediate plateaux at the following fractional values of the saturation magnetization: 1/3-2/3-1, 0-1/3-2/3-1 or 0-2/3-1. The inverse susceptibility displays a marked temperature dependence significantly influenced by a character of the zero-field ground state. The obtained theoretical results are confronted with recent high-field magnetization data of the mineral crystal fedotovite K2Cu3(SO4)3.
The frustrated spin-1/2 Ising-Heisenberg ladder with Heisenberg intra-rung and Ising inter-rung interactions is exactly solved in a longitudinal magnetic field by taking advantage of the local conservation of the total spin on each rung and the transfer-matrix method. We have rigorously calculated the ground-state phase diagram, magnetization process, magnetocaloric effect and basic thermodynamic quantities for the model, which can be alternatively viewed as an Ising-Heisenberg tetrahedral chain. It is demonstrated that a stepwise magnetization curve with an intermediate plateau at a half of the saturation magnetization is also reflected in respective stepwise changes of the concurrence serving as a measure of bipartite entanglement. The ground-state phase diagram and zero-temperature magnetization curves of the Ising-Heisenberg tetrahedral chain are contrasted with the analogous results of the purely quantum Heisenberg tetrahedral chain, which have been obtained through density-matrix renormalization group (DMRG) calculations. While both ground-state phase diagrams fully coincide in the regime of weak inter-rung interaction, the purely quantum Heisenberg tetrahedral chain develops Luttinger spin-liquid and Haldane phases for strongly coupled rungs which are absent in the Ising-Heisenberg counterpart model.
The ground state and zero-temperature magnetization process of the spin-1/2 Ising-Heisenberg model on two-dimensional triangles-in-triangles lattices is exactly calculated using eigenstates of the smallest commuting spin clusters. Our ground-state analysis of the investigated classical--quantum spin model reveals three unconventional dimerized or trimerized quantum ground states besides two classical ground states. It is demonstrated that the spin frustration is responsible for a variety of magnetization scenarios with up to three or four intermediate magnetization plateaus of either quantum or classical nature. The exact analytical results for the Ising-Heisenberg model are confronted with the corresponding results for the purely quantum Heisenberg model, which were obtained by numerical exact diagonalizations based on the Lanczos algorithm for finite-size spin clusters of 24 and 21 sites, respectively. It is shown that the zero-temperature magnetization process of both models is quite reminiscent and hence, one may obtain some insight into the ground states of the quantum Heisenberg model from the rigorous results for the Ising-Heisenberg model even though exact ground states for the Ising-Heisenberg model do not represent true ground states for the pure quantum Heisenberg model.
Using density matrix renormalization group calculations, ground state properties of the spin-1 Heisenberg chain with exchange and single-ion anisotropies in an external field are studied. Our findings confirm and refine recent results by Sengupta and Batista, Physical Review Letters 99, 217205 (2007) (2007), on the same model applying Monte Carlo techniques. In particular, we present evidence for two types of biconical (or supersolid) and for two types of spin-flop (or superfluid) structures. Basic features of the quantum phase diagram may be interpreted qualitatively in the framework of classical spin models.
Ground states of the frustrated spin-1 Ising-Heisenberg two-leg ladder with Heisenberg intra-rung coupling and only Ising interaction along legs and diagonals are rigorously found by taking advantage of local conservation of the total spin on each rung. The constructed ground-state phase diagram of the frustrated spin-1 Ising-Heisenberg ladder is then compared with the analogous phase diagram of the fully quantum spin-1 Heisenberg two-leg ladder obtained by density matrix renormalization group (DMRG) calculations. It is demonstrated that both investigated spin models exhibit quite similar magnetization scenarios, which involve intermediate plateaux at one-quarter, one-half and three-quarters of the saturation magnetization.
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