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Register a new userLow-threshold whispering-gallery-mode microlasers fabricated in a Nd: glass substrate by three-dimensional femtosecond laser micromachining
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We report on fabrication of whispering-gallery-mode microlasers in a Nd:glass chip by femtosecond laser three-dimensional (3D) micromachining. Main fabrication procedures include the fabrication of freestanding microdisks supported by thin pillars by femtosecond laser ablation of the glass substrate immersed in water, followed by CO2 laser annealing for surface smoothing. Lasing is observed at a pump threshold as low as ~69 {mu}W at room temperature with a continuous-wave laser diode operating at 780nm. This technique allows for fabrication of microcavities of high quality factors in various dielectric materials such as glasses and crystals.
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Titanium doped sapphire (Ti:sapphire) is a laser gain material with broad gain bandwidth benefiting from the material stability of sapphire. These favorable characteristics of Ti:sapphire have given rise to femtosecond lasers and optical frequency combs. Shaping a single Ti:sapphire crystal into a millimeter sized high quality whispering gallery mode resonator ($Qsim10^8$) reduces the lasing threshold to 14.2 mW and increases the laser slope efficiency to 34%. The observed lasing can be both multi-mode and single-mode. This is the first demonstration of a Ti:sapphire whispering-gallery laser. Furthermore, a novel method of evaluating the gain in Ti:sapphire in the near infrared region is demonstrated by introducing a probe laser with a central wavelength of 795 nm. This method results in decreasing linewidth of the modes excited with the probe laser, consequently increasing their $Q$. These findings open avenues for the usage of whispering gallery mode resonators as cavities for the implementation of compact Ti:sapphire lasers. Moreover, Ti:sapphire can also be utilized as an amplifier inside its gain bandwidth by implementing a pump-probe configuration.
Cuboid-shaped organic microcavities containing a pyrromethene laser dye and supported upon a photonic crystal have been investigated as an approach to reducing the lasing threshold of the cavities. Multiphoton lithography facilitated fabrication of the cuboid cavities directly on the substrate or on the decoupling structure, while similar structures were fabricated on the substrate by UV lithography for comparison. Significant reduction of the lasing threshold by a factor of ~30 has been observed for cavities supported by the photonic crystal relative to those fabricated on the substrate. The lasing mode spectra of the cuboid microresonators provide strong evidence showing that the lasing modes are localized in the horizontal plane, with the shape of an inscribed diamond.
A fiber laser is stabilized using a Calcium Fluoride (CaF2) whispering-gallery-mode resonator. It is set up using a semiconductor optical amplifier as a gain medium. The resonator is critically coupled through prisms, and used as a filtering element to suppress the laser linewidth. Using the self-heterodyne beat technique the linewidth is determined to be 13 kHz. This implies an enhancement factor of 10^3 with respect to the passive cavity linewidth. The three-cornered hat method shows a stability of 10^(-11) after 10 mu s.
Detection and characterization of individual nano-scale particles, virions, and pathogens are of paramount importance to human health, homeland security, diagnostic and environmental monitoring[1]. There is a strong demand for high-resolution, portable, and cost-effective systems to make label-free detection and measurement of individual nanoparticles, molecules, and viruses [2-6]. Here, we report an easily accessible, real-time and label-free detection method with single nanoparticle resolution that surpasses detection limit of existing micro- and nano-photonic devices. This is achieved by using an ultra-narrow linewidth whispering gallery microlaser, whose lasing line undergoes frequency splitting upon the binding of individual nano-objects. We demonstrate detection of polystyrene and gold nanoparticles as small as 15 nm and 10 nm in radius, respectively, and Influenza A virions by monitoring changes in self-heterodyning beat note of the split lasing modes. Experiments are performed in both air and aqueous environment. The built-in self-heterodyne interferometric method achieved in a microlaser provides a self-reference scheme with extraordinary sensitivity [7,8], and paves the way for detection and spectroscopy of nano-scale objects using micro- and nano-lasers.
Recently optical whispering-gallery-mode resonators (WGMRs) have emerged as promising platforms to achieve label-free detection of nanoscale objects and to reach single molecule sensitivity. The ultimate detection performance of WGMRs are limited by energy dissipation in the material they are fabricated from. Up to date, to improve detection limit, either rare-earth ions are doped into the WGMR to compensate losses or plasmonic resonances are exploited for their superior field confinement. Here, we demonstrate, for the first time, enhanced detection of single-nanoparticle induced mode-splitting in a silica WGMR via Raman-gain assisted loss-compensation and WGM Raman lasing. Notably, we detected and counted individual dielectric nanoparticles down to a record low radius of 10 nm by monitoring a beatnote signal generated when split Raman lasing lines are heterodyne-mixed at a photodetector. This dopant-free scheme retains the inherited biocompatibility of silica, and could find widespread use for sensing in biological media. It also opens the possibility of using intrinsic Raman or parametric gain in other systems, where dissipation hinders the progress of the field and limits applications.
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