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Register a new userThe reversal of magnetization driven by the Dzyaloshinskii-Moriya interaction(DMI) in perovskite Bi2FeMnO6
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Hong-Jian Feng
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Ab initio calculations show that the coupling between antiferrodistortive(AFD) distortions and magnetization in perovskite Bi2FeMnO6 is prohibited to make magnetization rotate as on-site Coulomb interaction($U$) is larger than 2.7 eV, where anomalies in antiferromagnetic(AFM) vectors and band gap varying with on-site Coulomb interaction can be observed. This coupling is attributed to the antisymmetric Dzyaloshinskii-Moriya interaction(DMI) driven by the eg-eg states AFM interaction and charge redistribution with respect to different AFD distortions.
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Ab initio calculations show that the Dzyaloshinskii-Moriya interaction(DMI)and net magnetization per unit cell in BiFeO3 are reduced when U is increasing from 0 to 2.9 eV, and independent of $J$. Interestingly, the DMI is even destroyed as $U$ exceeds a critical value of 2.9 eV. We propose a simple model to explain this phenomenon and present the nature of the rotation of the magnetization corresponding to altered antiferrodistortive distortions under DMI in BiFeO3.
Brillouin light spectroscopy is a powerful and robust technique for measuring the interfacial Dzyaloshinskii-Moriya interaction in thin films with broken inversion symmetry. Here we show that the magnon visibility, i.e. the intensity of the inelastically scattered light, strongly depends on the thickness of the dielectric seed material - SiO$_2$. By using both, analytical thin-film optics and numerical calculations, we reproduce the experimental data. We therefore provide a guideline for the maximization of the signal by adapting the substrate properties to the geometry of the measurement. Such a boost-up of the signal eases the magnon visualization in ultrathin magnetic films, speeds-up the measurement and increases the reliability of the data.
The exchange bias effect in compensated IrMn3/Co(111) system is studied using multiscale modeling from ab initio to atomistic calculations. We evaluate numerically the out-of-plane hysteresis loops of the bi-layer for different thickness of the ferromagnetic layer. The results show the existence of a perpendicular exchange bias field and an enhancement of the coercivity of the system. In order to elucidate the possible origin of the exchange bias, we analyze the hysteresis loops of a selected bi-layer by tuning the different contributions to the exchange interactions across the interface. Our results indicate that the exchange bias is primarily induced by the Dzyaloshinskii-Moriya interactions, while the coercivity is increased mainly due to a spin-flop mechanism.
Chiral spin textures at the interface between ferromagnetic and heavy nonmagnetic metals, such as Neel-type domain walls and skyrmions, have been studied intensively because of their great potential for future nanomagnetic devices. The Dyzaloshinskii-Moriya interaction (DMI) is an essential phenomenon for the formation of such chiral spin textures. In spite of recent theoretical progress aiming at understanding the microscopic origin of the DMI, an experimental investigation unravelling the physics at stake is still required. Here, we experimentally demonstrate the close correlation of the DMI with the anisotropy of the orbital magnetic moment and with the magnetic dipole moment of the ferromagnetic metal. The density functional theory and the tight-binding model calculations reveal that asymmetric electron occupation in orbitals gives rise to this correlation.
The interface between a ferromagnet (FM) or antiferromagnet (AFM) and a heavy metal (HM) results in an antisymmetric exchange interaction known as the interfacial Dzyaloshinskii-Moriya interaction (iDMI) which favors non-collinear spin configurations. The iDMI is responsible for stabilizing noncollinear spin textures such as skyrmions in materials with bulk inversion symmetry. Interfacial DMI values have been previously determined theoretically and experimentally for FM/HM interfaces, and, in this work, values are calculated for the metallic AFM MnPt and the insulating AFM NiO. The heavy metals considered are W, Re, and Au. The effects of the AFM and HM thicknesses are determined. The iDMI values of the MnPt heterolayers are comparable to those of the common FM materials, and those of NiO are lower.
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