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Nonclassical Radiation from Thermal Cavities in the Ultrastrong Coupling Regime

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 Added by Michael Hartmann Dr
 Publication date 2012
  fields Physics
and research's language is English




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Thermal or chaotic light sources emit radiation characterized by a slightly enhanced probability of emitting photons in bunches, described by a zero-delay second-order correlation function $g^{(2)}(0) = 2$. Here we explore photon-coincidence counting statistics of thermal cavities in the ultrastrong coupling regime, where the atom-cavity coupling rate becomes comparable to the cavity resonance frequency. We find that, depending on the system temperature and coupling rate, thermal photons escaping the cavity can display very different statistical behaviors, characterised by second-order correlation functions approaching zero or greatly exceeding two.

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We explore photon coincidence counting statistics in the ultrastrong-coupling regime where the atom-cavity coupling rate becomes comparable to the cavity resonance frequency. In this regime usual normal order correlation functions fail to describe the output photon statistics. By expressing the electric-field operator in the cavity-emitter dressed basis we are able to propose correlation functions that are valid for arbitrary degrees of light-matter interaction. Our results show that the standard photon blockade scenario is significantly modified for ultrastrong coupling. We observe parametric processes even for two-level emitters and temporal oscillations of intensity correlation functions at a frequency given by the ultrastrong photon emitter coupling. These effects can be traced back to the presence of two-photon cascade decays induced by counter-rotating interaction terms.
The interaction among the components of a hybrid quantum system is often neglected when considering the coupling of these components to an environment. However, if the interaction strength is large, this approximation leads to unphysical predictions, as has been shown for cavity-QED and optomechanical systems in the ultrastrong-coupling regime. To deal with these cases, master equations with dissipators retaining the interaction between these components have been derived for the quantum Rabi model and for the standard optomechanical Hamiltonian. In this article, we go beyond these previous derivations and present a general master equation approach for arbitrary hybrid quantum systems interacting with thermal reservoirs. Specifically, our approach can be applied to describe the dynamics of open hybrid systems with harmonic, quasi-harmonic, and anharmonic transitions. We apply our approach to study the influence of temperature on multiphoton vacuum Rabi oscillations in circuit QED. We also analyze the influence of temperature on the conversion of mechanical energy into photon pairs in an optomechanical system, which has been recently described at zero temperature. We compare our results with previous approaches, finding that these sometimes overestimate decoherence rates and understimate excited-state populations.
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We investigate the output generation of squeezed radiation of a cavity photon mode coupled to another off-resonant bosonic excitation. By modulating in time their linear interaction, we predict high degree of output squeezing when the dispersive ultrastrong coupling regime is achieved, i.e., when the interaction rate becomes comparable to the frequency of the lowest energy mode. Our work paves the way to squeezed light generation in frequency domains where the ultrastrong coupling is obtained, e.g., solid-state resonators in the GHz, THz and mid-IR spectral range.
The interaction between an atom and the electromagnetic field inside a cavity has played a crucial role in the historical development of our understanding of light-matter interaction and is a central part of various quantum technologies, such as lasers and many quantum computing architectures. The emergence of superconducting qubits has allowed the realization of strong and ultrastrong coupling between artificial atoms and cavities. If the coupling strength $g$ becomes as large as the atomic and cavity frequencies ($Delta$ and $omega_{rm o}$ respectively), the energy eigenstates including the ground state are predicted to be highly entangled. This qualitatively new regime can be called the deep strong-coupling regime, and there has been an ongoing debate over whether it is fundamentally possible to realize this regime in realistic physical systems. By inductively coupling a flux qubit and an LC oscillator via Josephson junctions, we have realized circuits with $g/omega_{rm o}$ ranging from 0.72 to 1.34 and $g/Deltagg 1$. Using spectroscopy measurements, we have observed unconventional transition spectra, with patterns resembling masquerade masks, that are characteristic of this new regime. Our results provide a basis for ground-state-based entangled-pair generation and open a new direction of research on strongly correlated light-matter states in circuit-quantum electrodynamics.
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