No Arabic abstract
High resolution angle-resolved photoemission measurements are carried out to systematically investigate the effect of cleaving temperature on the electronic structure and Fermi surface of Sr$_2$RuO$_4$. Different from previous reports that high cleaving temperature can suppress surface Fermi surface, we find that the surface Fermi surface remains obvious and strong in Sr$_2$RuO$_4$ cleaved at high temperature, even at room temperature. This indicates that cleaving temperature is not a key effective factor in suppressing the surface bands. On the other hand, in the aged surface of Sr$_2$RuO$_4$ that is cleaved and held for a long time, the bulk bands can be enhanced. We have also carried out laser ARPES measurements on Sr$_2$RuO$_4$ by using vacuum ultra-violet laser (photon energy at 6.994 eV) and found an obvious enhancement of bulk bands even for samples cleaved at low temperature. These information are important in realizing an effective approach in manipulating and detecting the surface and bulk electronic structure of Sr$_2$RuO$_4$. In particular, the enhancement of bulk sensitivity, together with its super-high instrumental resolution of VUV laser ARPES, will be advantageous in investigating fine electronic structure and superconducting properties of Sr$_2$RuO$_4$ in the future.
We study the normal state electronic excitations probed by angle resolved photoemission spectroscopy (ARPES) in Bi2201 and Bi2212. Our main goal is to establish explicit criteria for determining the Fermi surface from ARPES data on strongly interacting systems where sharply defined quasiparticles do not exist and the dispersion is very weak in parts of the Brillouin zone. Additional complications arise from strong matrix element variations within the zone. We present detailed results as a function of incident photon energy, and show simple experimental tests to distinguish between an intensity drop due to matrix element effects and spectral weight loss due to a Fermi crossing. We reiterate the use of polarization selection rules in disentangling the effect of umklapps due to the BiO superlattice in Bi2212. We conclude that, despite all the complications, the Fermi surface can be determined unambiguously: it is a single large hole barrel centered about (pi,pi) in both materials.
The electronic structure of LaOFeAs, a parent compound of iron-arsenic superconductors, is studied by angleresolved photoemission spectroscopy. By examining its dependence on photon energy, polarization, sodium dosing and the counting of Fermi surface volume, both the bulk and the surface contributions are identified. We find that a bulk band moves toward high binding energies below structural transition, and shifts smoothly across the spin density wave transition by about 25 meV. Our data suggest the band reconstruction may play a crucial role in the spin density wave transition, and the structural transition is driven by the short range magnetic order. For the surface states, both the LaO-terminated and FeAs-terminated components are revealed. Certain small band shifts are verified for the FeAs-terminated surface states in the spin density wave state, which is a reflection of the bulk electronic structure reconstruction. Moreover, sharp quasiparticle peaks quickly rise at low temperatures, indicating of drastic reduction of the scattering rate. A kink structure in one of the surface band is shown to be possibly related to the electron-phonon interactions.
Here we apply high resolution angle-resolved photoemission spectroscopy (ARPES) using a wide excitation energy range to probe the electronic structure and the Fermi surface topology of the Ba1-xKxFe2As2 (Tc = 32 K) superconductor. We find significant deviations in the low energy band structure from that predicted in calculations. A set of Fermi surface sheets with unexpected topology is detected at the Brillouin zone boundary. At the X-symmetry point the Fermi surface is formed by a shallow electron-like pocket surrounded by four hole-like pockets elongated in G-X and G-Y directions.
The (Ca,R)FeAs2 (R=La,Pr and etc.) superconductors with a signature of superconductivity transition above 40 K possess a new kind of block layers that consist of zig-zag As chains. In this paper, we report the electronic structure of the new (Ca,La)FeAs2 superconductor investigated by both band structure calculations and high resolution angle-resolved photoemission spectroscopy measurements. Band structure calculations indicate that there are four hole-like bands around the zone center $Gamma$(0,0) and two electron-like bands near the zone corner M(pi,pi) in CaFeAs2. In our angle-resolved photoemission measurements on (Ca0.9La0.1})FeAs2, we have observed three hole-like bands around the Gamma point and one electron-like Fermi surface near the M(pi,pi) point. These results provide important information to compare and contrast with the electronic structure of other iron-based compounds in understanding the superconductivity mechanism in the iron-based superconductors.
In order to determine the orbital characters on the various Fermi surface pockets of the Fe-based superconductors Ba$_{0.6}$K$_{0.4}$Fe$_{2}$As$_{2}$ and FeSe$_{0.45}$Te$_{0.55}$, we introduce a method to calculate photoemission matrix elements. We compare our simulations to experimental data obtained with various experimental configurations of beam orientation and light polarization. We show that the photoemission intensity patterns revealed from angle-resolved photoemission spectroscopy measurements of Fermi surface mappings and energy-momentum plots along high-symmetry lines exhibit asymmetries carrying precious information on the nature of the states probed, information that is destroyed after the data symmetrization process often performed in the analysis of angle-resolved photoemission spectroscopy data. Our simulations are consistent with Fermi surfaces originating mainly from the $d_{xy}$, $d_{xz}$ and $d_{yz}$ orbitals in these materials.