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Register a new userLow-temperature heat transport of the layered spin-dimer compound Ba_3Mn_2O_8
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We report the study on the low-temperature heat transport of Ba_3Mn_2O_8 single crystal, a layered spin-dimer compound exhibiting the magnetic-field-induced magnetic order or the magnon Bose-Einstein condensation. The thermal conductivities (kappa) along both the ab plane and the c axis show nearly isotropic dependence on magnetic field, that is, kappa is strongly suppressed with increasing field, particularly at the critical fields of magnetic phase transitions. These results indicate that the magnetic excitations play a role of scattering phonons and the scattering effect is enhanced when the magnetic field closes the gap in the spin spectrum. In addition, the magnons in the BEC state of this materials do not show notable ability of carrying heat.
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We report the magnetic-field dependence of thermal conductivity (kappa) of an insulating cuprate Nd_2CuO_4 at very low temperatures down to 0.3 K. It is found that apart from the paramagnetic moments scattering on phonons, the Nd^{3+} magnons can act as either heat carriers or phonon scatterers, which strongly depends on the long-range antiferromagnetic transition and the field-induced transitions of spin structure. In particular, the Nd^{3+} magnons can effectively transport heat in the spin-flopped state of the Nd^{3+} sublattice. However, both the magnon transport and the magnetic scattering are quenched at very high fields. The spin re-orientations under the in-plane field can be conjectured from the detailed field dependence of kappa.
We present results of magnetisation and electron paramagnetic resonance experiments on the spin-dimer system BaCuSi2O6. Evidence indicates that the origin of anisotropic terms in the spin Hamiltonian is from magnetic dipolar interactions. Axial symmetry-breaking is on a very small energy scale of ~11 mK, confirming Bose Einstein condensation critical scaling over an extended temperature range in the vicinity of the quantum critical point.
Heat capacity and magnetic torque measurements are used to probe the anisotropic temperature-field phase diagram of the frustrated spin dimer compound Ba3Mn2O8 in the field range from 0T to 18T. For fields oriented along the c axis a single magnetically ordered phase is found in this field range, whereas for fields oriented along the a axis two distinct phases are observed. The present measurements reveal a surprising non-monotonic evolution of the phase diagram as the magnetic field is rotated in the [001]-[100] plane. The angle dependence of the critical field (Hc1) that marks the closing of the spin gap can be quantitatively accounted for using a minimal spin Hamiltonian comprising superexchange between nearest and next nearest Mn ions, the Zeeman energy and single ion anisotropy. This Hamiltonian also predicts a non-monotonic evolution of the transition between the two ordered states as the field is rotated in the a-c plane. However, the observed effect is found to be significantly larger in magnitude, implying that either this minimal spin Hamiltonian is incomplete or that the magnetically ordered states have a slightly different structure than previously proposed.
Ba3Mn2O8 is a hexagonally coordinated Mn5+ S=1 spin dimer system with small uniaxial single-ion anisotropy. 135,137Ba NMR spectroscopy is used to establish the lower critical field Hc1 of distinct field-induced phases for H parallel to c,H perpendicular to c, and measure the longitudinal (Ml) and transverse (Mt) magnetizations in the vicinity of the quantum critical point (QCP). Ml_parallel (T, Hc1), Ml_perpendicular (T, Hc1) are reproduced by solving a low-energy model for a dilute gas of interacting bosons. Ml_parallel(T goes to 0, H = Hc1) (Ml_perpendicular(T goes to 0, H = Hc1)) follows the expectation for a BEC (Ising-like) QCP.
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