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Register a new userQuantum criticality near the upper critical field of Ce$_2$PdIn$_8$
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We report low-temperature specific heat measurements in magnetic fields up to 12 T applied parallel and perpendicular to the tetragonal c-axis of the heavy fermion superconductor Ce$_2$PdIn$_8$. In contrast to its quasi-two-dimensional (2D) relative CeCoIn$_5$, the system displays an almost isotropic upper critical field. While there is no indication for a FFLO phase in Ce$_2$PdIn$_8$, the data suggest a smeared weak first-order superconducting transition close to $H_{c2}approx 2$ T. The normal state electronic specific heat coefficient displays logarithmically divergent behavior, comparable to CeCoIn$_5$ and in agreement with 2D quantum criticality of spin-density-wave type.
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We report on single crystal growth and crystallographic parameters results of Ce$_2$PdIn$_8$, Ce$_3$PdIn$_{11}$, Ce$_2$PtIn$_8$ and Ce$_3$PtIn$_{11}$. The Pt-systems Ce$_2$PtIn$_8$ and Ce$_3$PtIn$_{11}$ are synthesized for the first time. All these compounds are member of the Ce$_n$T$_m$In$_{3n+2m}$ (n = 1, 2,..; m = 1, 2,.. and T = transition metal) to which the extensively studied heavy fermion superconductor CeCoIn$_5$ belongs. Single crystals have been grown by In self-flux method. Differential scanning calorimetry studies were used to derive optimal growth conditions. Evidently, the maximum growth conditions for these materials should not exceed 750 $^{circ}$C. Single crystal x-ray data show that Ce$_2$TIn$_8$ compounds crystallize in the tetragonal Ho$_2$CoGa$_8$ phase (space group P4/mmm) with lattice parameters a =4.6898(3) $AA$ and c =12.1490(8) $AA$ for the Pt-based one (Pd: a = 4.6881(4) $AA$ and c = 12.2031(8) AA). The Ce$_3$TIn$_{11}$ compounds adopt the Ce$_3$PdIn$_{11}$ structure with a = 4.6874(4) $AA$ and c = 16.8422(12) $AA$ for the Pt-based one (Pd: a = 4.6896 $AA$ and c = 16.891 AA). Specific heat experiments on Ce$_3$PtIn$_{11}$ and Ce$_3$PdIn$_{11}$ have revealed that both compounds undergo two successive magnetic transitions at T$_1$ ~ 2.2 K followed by T$_N$ ~ 2.0 K and T$_1$ ~ 1.7 K and T$_N$ ~ 1.5 K, respectively. Additionally, both compounds exhibit enhanced Sommerfeld coefficients yielding {gamma}$_{Pt}$ = 0.300 J/mol K$^2$ Ce ({gamma}$_{Pd}$ = 0.290 J/mol K$^2$ Ce), hence qualifying them as heavy fermion materials.
We present a detailed analysis of the upper critical field for CeCoIn5 under high pressure. We show that, consistently with other measurements, this system shows a decoupling between maximum of the superconducting transition temperature Tc and maximum pairing strength. This puts forward CeCoIn5 as an important paradigm for this class of unconventional, strongly correlated superconductors.
Systems with embedded magnetic ions that exhibit a competition between magnetic order and disorder down to absolute zero can display unusual low temperature behaviors of the resistivity, susceptibility, and specific heat. Moreover, the dynamic response of such a system can display hyperscaling behavior in which the relaxation back to equilibrium when an amount of energy E is given to the system at temperature T only depends on the ratio E/T. Ce(Fe$_{0.755}$Ru$_{0.245}$)$_2$Ge$_2$ is a system that displays these behaviors. We show that these complex behaviors are rooted in a fragmentation of the magnetic lattice upon cooling caused by a distribution of local Kondo screening temperatures, and that the hyperscaling behavior can be attributed to the flipping of the total magnetic moment of magnetic clusters that spontaneously form and order upon cooling. We present our arguments based on the review of two-decades worth of neutron scattering and transport data on this system, augmented with new polarized neutron scattering experiments.
The evolution of magnetism and superconductivity in Ce$_2$Rh$_{1-x}$Pd$_x$In$_8$ solid solutions has been studied within the entire concentration range by means of thermodynamic and magnetic measurements at ambient pressure and at temperatures between 0.35 K and room temperature. For this purpose, single crystals with Pd concentrations x = 0, 0.10, 0.15, 0.30, 0.45, 0.55, 0.85 and 1 have been grown from In self-flux and characterized by x-ray diffraction and microprobe analysis. Starting from the antiferromagnet Ce$_2$RhIn$_8$, the Neel temperature gradually decreases with increasing Pd concentration and the antiferromagnetism has disappeared for $x ge 0.45$. Superconductivity has been observed only for Ce$_2$PdIn$_8$.
Electric resistivity, specific heat, magnetic susceptibility, and inelastic neutron scattering experiments were performed on a single crystal of the heavy fermion compound Ce(Ni$_{0.935}$Pd$_{0.065}$)$_2$Ge$_2$ in order to study the spin fluctuations near an antiferromagnetic (AF) quantum critical point (QCP). The resistivity and the specific heat coefficient for $T leq$ 1 K exhibit the power law behavior expected for a 3D itinerant AF QCP ($rho(T) sim T^{3/2}$ and $gamma(T) sim gamma_0 - b T^{1/2}$). However, for 2 $leq T leq$ 10 K, the susceptibility and specific heat vary as $log T$ and the resistivity varies linearly with temperature. Furthermore, despite the fact that the resistivity and specific heat exhibit the non-Fermi liquid behavior expected at a QCP, the correlation length, correlation time, and staggered susceptibility of the spin fluctuations remain finite at low temperature. We suggest that these deviations from the divergent behavior expected for a QCP may result from alloy disorder.
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