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Register a new userNuclear masses, deformations and shell effects
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We show that the Liquid Drop Model is best suited to describe the masses of prolate deformed nuclei than of spherical nuclei. To this end three Liquid Drop Mass formulas are employed to describe nuclear masses of eight sets of nuclei with similar quadrupole deformations. It is shown that they are able to fit the measured masses of prolate deformed nuclei with an RMS smaller than 750 keV, while for the spherical nuclei the RMS is, in the three cases, larger than 2000 keV. The RMS of the best fit of the masses of semi-magic nuclei is also larger than 2000 keV. The parameters of the three models are studied, showing that the surface symmetry term is the one which varies the most from one group of nuclei to another. In one model, isospin dependent terms are also found to exhibit strong changes. The inclusion of shell effects allows for better fits, which continue to be better in the prolate deformed nuclei region
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We tabulate the atomic mass excesses and binding energies, ground-state shell-plus-pairing corrections, ground-state microscopic corrections, and nuclear ground-state deformations of 9318 nuclei ranging from $^{16}$O to $A=339$. The calculations are based on the finite-range droplet macroscopic model and the folded-Yukawa single-particle microscopic model. Relative to our FRDM(1992) mass table in {sc Atomic Data and Nuclear Data Tables} [{bf 59} 185 (1995)], the results are obtained in the same model, but with considerably improved treatment of deformation and fewer of the approximations that were necessary earlier, due to limitations in computer power. The more accurate execution of the model and the more extensive and more accurate experimental mass data base now available allows us to determine one additional macroscopic-model parameter, the density-symmetry coefficient $L$, which was not varied in the previous calculation, but set to zero. Because we now realize that the FRDM is inaccurate for some highly deformed shapes occurring in fission, because some effects are derived in terms of perturbations around a sphere, we only adjust its macroscopic parameters to ground-state masses. The values of ten constants are determined directly from an optimization to fit ground-state masses of 2149 nuclei ranging from $^{16}$O to $^{265}_{106}$Sg and $^{264}_{108}$Hs. The error of the mass model is 0.5595~MeV. We also provide masses in the FRLDM, which in the more accurate treatments now has an error of 0.6618 MeV. But in contrast to the FRDM, it is suitable for studies of fission and has been extensively so applied elsewhere, with FRLDM(2002) constants. The FRLDM(2012) fits 31 fission barrier heights from $^{70}$Se to $^{252}$Cf with a root-mean-square deviation of 1.052 MeV.
We analyze the ability of the three different Liquid Drop Mass (LDM) formulas to describe nuclear masses for nuclei in various deformation regions. Separating the 2149 measured nuclear species in eight sets with similar quadrupole deformations, we show that the masses of prolate deformed nuclei are better described than those of spherical ones. In fact, the prolate deformed nuclei are fitted with an RMS smaller than 750 keV, while for spherical and semi-magic species the RMS is always larger than 2000 keV. These results are found to be independent of pairing. The macroscopic sector of the Duflo-Zuker (DZ) mass model reproduces shell effects, while most of the deformation dependence is lost and the RMS is larger than in any LDM. Adding to the LDM the microscopically motivated DZ master terms introduces the shell effects, allowing for a significant reduction in the RMS of the fit but still exhibiting a better description of prolate deformed nuclei. The inclusion of shell effects following the Interacting Boson Models ideas produces similar results.
A unified theoretical model reproducing charge radii of known atomic nuclei plays an essential role to make extrapolations in the regions of unknown nuclear size. Recently developed new ansatz which phenomenally takes into account the neutron-proton short-range correlations (np-SRCs) can describe the discontinuity properties and odd-even staggering (OES) effect of charge radii along isotopic chains remarkably well. In this work, we further review the modified rms charge radii formula in the framework of relativistic mean field (RMF) theory. The charge radii are calculated along various isotopic chains that include the nuclei featuring the $N=50$ and $82$ magic shells. Our results suggest that RMF with and without considering correction term give almost similar trend of nuclear size for some isotopic chains with open proton shell, especially the shrink phenomena of charge radii at strong neutron closed shells and the OES behaviors. This suggests that the np-SRCs has almost no influence for some nuclei due to the strong coupling between different levels around Fermi surface. The weakening OES behavior of nuclear charge radii is observed generally at completely filled neutron shells and this may be proposed as a signature of magic indicator.
Precision mass spectrometry of neutron-rich nuclei is of great relevance for astrophysics. Masses of exotic nuclides impose constraints on models for the nuclear interaction and thus affect the description of the equation of state of nuclear matter, which can be extended to describe neutron-star matter. With knowledge of the masses of nuclides near shell closures, one can also derive the neutron-star crustal composition. The Penning-trap mass spectrometer ISOLTRAP at CERN-ISOLDE has recently achieved a breakthrough measuring the mass of 82Zn, which allowed constraining neutron-star crust composition to deeper layers (Wolf et al., PRL 110, 2013). We perform a more detailed study on the sequence of nuclei in the outer crust of neutron stars with input from different nuclear models to illustrate the sensitivity to masses and the robustness of neutron-star models. The dominant role of the N=50 and N=82 closed neutron shells for the crustal composition is confirmed.
The kernel ridge regression (KRR) approach is extended to include the odd-even effects in nuclear mass predictions by remodulating the kernel function without introducing new weight parameters and inputs in the training network. By taking the WS4 mass model as an example, the mass for each nucleus in the nuclear chart is predicted with the extended KRR network, which is trained with the mass model residuals, i.e., deviations between experimental and calculated masses, of other nuclei with known masses. The resultant root-mean-square mass deviation from the available experimental data for the 2353 nuclei with $Zge8$ and $Nge8$ can be reduced to 128 keV, which provides the most precise mass model from machine learning approaches so far. Moreover, the extended KRR approach can avoid the risk of worsening the mass predictions for nuclei at large extrapolation distances, and meanwhile, it provides a smooth extrapolation behavior with respect to the odd and even extrapolation distances.
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