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Register a new userEvidence for Dirac Nodes from Quantum Oscillations in SrFe$_2$As$_2$
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We present a detailed study of quantum oscillations in the antiferromagnetically ordered pnictide compound SrFe$_2$As$_2$ as the angle between the applied magnetic field and crystalline axes is varied. Our measurements were performed on high quality single crystals in a superconducting magnet, and in pulsed magnetic fields up to 60 T, allowing us to observe orbits from several small Fermi surface pockets. We extract the cyclotron effective mass $m^{star}$ and frequency $F$ for these orbits and track their values as the field is rotated away from the c-axis. While a constant ratio of $m^{star}/F$ is observed for one orbit as expected for a parabolic band, a clear deviation is observed for another. We conclude that this deviation points to an orbit derived from a band with Dirac dispersion near the Fermi level.
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A detailed elastic neutron scattering study of the structural and magnetic phase transitions in single-crystal SrFe$_2$As$_2$ reveals that the orthorhombic (O)-tetragonal (T) and the antiferromagnetic transitions coincide at $T_texttt{O}$ = $T_texttt{N}$ = (201.5 $pm$ 0.25) K. The observation of coexisting O-T phases over a finite temperature range at the transition and the sudden onset of the O distortion provide strong evidences that the structural transition is first order. The simultaneous appearance and disappearance within 0.5 K upon cooling and within 0.25 K upon warming, respectively, indicate that the magnetic and structural transitions are intimately coupled. We find that the hysteresis in the transition temperature extends over a 1-2 K range. Based on the observation of a remnant orthorhombic phase at temperatures higher than emph{T}$_texttt{O}$, we suggest that the T-O transition may be an order-disorder transition.
Neutron diffraction measurements have been carried out to investigate the magnetic form factor of the parent SrFe2As2 system of the iron-based superconductors. The general feature is that the form factor is approximately isotropic in wave vector, indicating that multiple d-orbitals of the iron atoms are occupied as expected based on band theory. Inversion of the diffraction data suggests that there is some elongation of the spin density toward the As atoms. We have also extended the diffraction measurements to investigate a possible jump in the c-axis lattice parameter at the structural phase transition, but find no detectable change within the experimental uncertainties.
An instrumentation problem with the signal acquisition at high frequencies was discovered and we no longer believe that the experimental data presented in the manuscript, showing a frequency enhancement of the elastoresistivity, are correct. After correcting the problem, the elastoresistivity data is frequency independent in the range investigated. Therefore, the authors have withdrawn this submission. We would like to thank Alex Hristov, Johanna Palmstrom, Josh Straquadine and Ian Fisher (Stanford) for the kind discussions and assistance we received which helped us identify these problems.
In order to investigate whether magnetism and superconductivity coexist in Co-doped SrFe$_2$As$_2$, we have prepared single crystals of SrFe$_{2-x}$Co$_x$As$_2$, $x$ = 0 and 0.4, and characterized them via X-ray diffraction, electrical resistivity in zero and applied field up to 9 T as well as at ambient and applied pressure up to 1.6 GPa, and magnetic susceptibility. At $x$ = 0.4, there is both magnetic and resistive evidence for a spin density wave transition at 120 K, while $T_c$ = 19.5 K - indicating coexistent magnetism and superconductivity. A discussion of how these results compare with reported results, both in SrFe$_{2-x}$Co$_x$As$_2$ and in other doped 122 compounds, is given.
We present a study of the Fermi surface of KFe$_2$As$_2$ single crystals. Quantum oscillations were observed in magnetostriction measured down to 50 mK and in magnetic fields $H$ up to 14 T. For $H parallel c$, the calculated effective masses are in agreement with recent de Haas-van Alphen and ARPES experiments, showing enhanced values with respect to the ones obtained from previous band calculations. For $H parallel a$, we observed a small orbit at a cyclotron frequency of 64 T, characterized by an effective mass of $sim 0.8 m_e$, supporting the presence of a three-dimensional pocket at the Z-point.
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