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Register a new userFull control of spontaneous emission in confined Tamm plasmon structures
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We demonstrate strong confinement of the optical field by depositing a micron sized metallic disk on a planar interferential mirror. Zero dimensional Tamm plasmon modes are evidenced both experimentally and theoretically, with a lateral confinement limited to the disk area and strong coupling to TE polarized fields. Single quantum dots deterministically coupled to these modes are shown to experience acceleration of their spontaneous emission when spectrally resonant with the mode. For quantum dots spectrally detuned from the confined Tamm Plasmon mode, an inhibition of spontaneous emission by a factor 40 is observed, a record value in the optical domain.
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We investigate theoretically the non-Markovian dynamics of a degenerate V-type quantum emitter in the vicinity of a metallic nanosphere, a system that exhibits quantum interference in spontaneous emission due to the anisotropic Purcell effect. We calculate numerically the electromagnetic Greens tensor and employ the effective modes differential equation method for calculating the quantum dynamics of the emitter population, with respect to the resonance frequency and the initial state of the emitter, as well as its distance from the nanosphere. We find that the emitter population evolution varies between a gradually total decay and a partial decay combined with oscillatory population dynamics, depending strongly on the specific values of the above three parameters. Under strong coupling conditions, coherent population trapping can be observed in this system. We compare our exact results with results when the flat continuum approximation for the modified by the metallic nanosphere vacuum is applied. We conclude that the flat continuum approximation is an excellent approximation only when the spectral density of the system under study is characterized by non-overlapping plasmonic resonances.
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