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Register a new userAttosecond probing of instantaneous AC Stark shifts in helium atoms
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Based on numerical solutions of the time-dependent Schrodinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a single tunable attosecond pulse to probe excited states of the perturbed atom. The ionization probability in the combined fields depends on both, the frequency of the attosecond pulse and the time delay between both pulses, since the IR field shifts excited energy levels into and out of resonance with the attosecond probe pulse. We show that this method (i) allows the detection of instantaneous atomic energy gaps with sub-laser-cycle time resolution and (ii) can be applied as an ultrafast gate for more complex processes such as non-sequential double-ionization.
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A strong, far-detuned laser can shift the energy levels of an optically active quantum system via the AC Stark effect. We demonstrate that the polarization of the laser results in a spin-selective modification to the energy structure of a charged quantum dot, shifting one spin manifold but not the other. An additional shift occurs due to the Overhauser field of the nuclear spins, which are pumped into a partially polarized state. This mechanism offers a potentially rapid, reversible, and coherent control of the energy structure and polarization selection rules of a charged quantum dot.
The burgeoning fields of quantum computing and quantum key distribution have created a demand for a quantum memory. The gradient echo memory scheme is a quantum memory candidate for light storage that can boast efficiencies approaching unity, as well as the flexibility to work with either two or three level atoms. The key to this scheme is the frequency gradient that is placed across the memory. Currently the three level implementation uses a Zeeman gradient and warm atoms. In this paper we model a new gradient creation mechanism - the ac Stark effect - to provide an improvement in the flexibility of gradient creation and field switching times. We propose this scheme in concert with a move to cold atoms (~1 mK). These temperatures would increase the storage times possible, and the small ensemble volumes would enable large ac Stark shifts with reasonable laser power. We find that memory bandwidths on the order of MHz can be produced with experimentally achievable laser powers and trapping volumes, with high precision in gradient creation and switching times on the order of nanoseconds possible. By looking at the different decoherence mechanisms present in this system we determine that coherence times on the order of 10s of milliseconds are possible, as are delay-bandwidth products of approximately 50 and efficiencies over 90%.
The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion in Helium by using an XUV attosecond pulse train to prepare a coherent superposition of excited states and a delayed femtosecond IR pulse to ionize them. Quantum beat signals observed in the high resolution photoelectron spectrogram allow us to follow the field-free evolution of the bound electron wavepacket and determine the time-dependent ionization dynamics of the low-lying 2p state.
We describe a numerical method that simulates the interaction of the helium atom with sequences of femtosecond and attosecond light pulses. The method, which is based on the close-coupling expansion of the electronic configuration space in a B-spline bipolar spherical harmonic basis, can accurately reproduce the excitation and single ionization of the atom, within the electrostatic approximation. The time dependent Schrodinger equation is integrated with a sequence of second-order split-exponential unitary propagators. The asymptotic channel-, energy- and angularly-resolved photoelectron distributions are computed by projecting the wavepacket at the end of the simulation on the multichannel scattering states of the atom, which are separately computed within the same close-coupling basis. This method is applied to simulate the pump-probe ionization of helium in the vicinity of the $2s/2p$ excitation threshold of the He$^+$ ion. This work confirms the qualitative conclusions of one of our earliest publications [L Argenti and E Lindroth, Phys. Rev. Lett. {bf 105}, 53002 (2010)], in which we demonstrated the control of the $2s/2p$ ionization branching-ratio. Here, we take those calculations to convergence and show how correlation brings the periodic modulation of the branching ratios in almost phase opposition. The residual total ionization probability to the $2s+2p$ channels is dominated by the beating between the $sp_{2,3}^+$ and the $sp_{2,4}^+$ doubly excited states, which is consistent with the modulation of the complementary signal in the $1s$ channel, measured in 2010 by Chang and co-workers~[S Gilbertson~emph{et al.}, Phys. Rev. Lett. {bf 105}, 263003 (2010)].
We study the dynamic behavior of ultracold neutral atoms in a macroscopic ac electric trap. Confinement in such a trap is achieved by switching between two saddle-point configurations of the electric field. The gradual formation of a stably trapped cloud is observed and the trap performance is studied versus the switching frequency and the symmetry of the switching cycle. Additionally, the electric field in the trap is mapped out by imaging the atom cloud while the fields are still on. Finally, the phase-space acceptance of the trap is probed by introducing a modified switching cycle. The experimental results are reproduced using full three-dimensional trajectory calculations.
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