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Register a new userLiquid Xenon Detectors for Positron Emission Tomography
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PET is a functional imaging technique based on detection of annihilation photons following beta decay producing positrons. In this paper, we present the concept of a new PET system for preclinical applications consisting of a ring of twelve time projection chambers filled with liquid xenon viewed by avalanche photodiodes. Simultaneous measurement of ionization charge and scintillation light leads to a significant improvement to spatial resolution, image quality, and sensitivity. Simulated performance shows that an energy resolution of <10% (FWHM) and a sensitivity of 15% are achievable. First tests with a prototype TPC indicate position resolution <1 mm (FWHM).
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The interaction of radiation with liquid xenon, inducing both scintillation and ionization signals, is of particular interest for Compton-sequences reconstruction. We report on the development and recent results of a liquid-xenon time-projection chamber, dedicated to a novel nuclear imaging technique named 3 gamma imaging. In a first prototype, the scintillation is detected by a vacuum photomultiplier tube and the charges are collected with a MICROMEGAS structure; both are fully immersed in liquid xenon. In view of the final large-area detector, and with the aim of minimizing dead-zones, we are investigating a gaseous photomultiplier for recording the UV scintillation photons. The prototype concept is presented as well as preliminary results in liquid xenon. We also present soft x-rays test results of a gaseous photomultiplier prototype made of a double Thick Gaseous Electron Multiplier (THGEM) at normal temperature and pressure conditions.
The fast scintillation decay time and the high scintillation yield of liquid xenon makes it an appropriate material for nuclear medicine. Moreover, being a continuous medium with a uniform response, liquid xenon allows one to avoid most of the geometrical distortions of conventional detectors based on scintillating crystals. In this paper, we describe how these properties have motivated the development of a novel concept for positron emission tomography scanners with Time-Of-Flight measurement, which uses liquid xenon as a scintillating material and silicon photomultipliers as sensors. Monte Carlo studies have indicated that this technology would provide a very good intrinsic time resolution, of around 70 ps. Moreover, being liquid xenon transparent to UV and blue wavelengths, both scintillation and Cherenkov light can be exploited. While the former can be used for energy measurements, the latter is a prompt signal (of a few picoseconds), which provides a very precise time measurement. Monte Carlo simulations point to a time resolution of 30-50 ps obtained using Cherenkov light. A first prototype is being built to demonstrate the high energy, spatial and time resolution of this concept, using a ring of around 30 cm of internal diameter and a depth of 3 cm instrumented with VUV--sensitive silicon photomultipliers.
This article reviews the progress made over the last 20 years in the development and applications of liquid xenon detectors in particle physics, astrophysics and medical imaging experiments. We begin with a summary of the fundamental properties of liquid xenon as radiation detection medium, in light of the most current theoretical and experimental information. After a brief introduction of the different type of liquid xenon detectors, we continue with a review of past, current and future experiments using liquid xenon to search for rare processes and to image radiation in space and in medicine. We will introduce each application with a brief survey of the underlying scientific motivation and experimental requirements, before reviewing the basic characteristics and expected performance of each experiment. Within this decade it appears likely that large volume liquid xenon detectors operated in different modes will contribute to answering some of the most fundamental questions in particle physics, astrophysics and cosmology, fulfilling the most demanding detection challenges. From experiments like MEG, currently the largest liquid xenon scintillation detector in operation, dedicated to the rare mu -> e + gamma decay, to the future XMASS which also exploits only liquid xenon scintillation to address an ambitious program of rare event searches, to the class of time projection chambers like XENON and EXO which exploit both scintillation and ionization of liquid xenon for dark matter and neutrinoless double beta decay, respectively, we anticipate unrivaled performance and important contributions to physics in the next few years.
Results are presented from radioactivity screening of two models of photomultiplier tubes designed for use in current and future liquid xenon experiments. The Hamamatsu 5.6 cm diameter R8778 PMT, used in the LUX dark matter experiment, has yielded a positive detection of four common radioactive isotopes: 238U, 232Th, 40K, and 60Co. Screening of LUX materials has rendered backgrounds from other detector materials subdominant to the R8778 contribution. A prototype Hamamatsu 7.6 cm diameter R11410 MOD PMT has also been screened, with benchmark isotope counts measured at <0.4 238U / <0.3 232Th / <8.3 40K / 2.0+-0.2 60Co mBq/PMT. This represents a large reduction, equal to a change of times 1/24 238U / times 1/9 232Th / times 1/8 40K per PMT, between R8778 and R11410 MOD, concurrent with a doubling of the photocathode surface area (4.5 cm to 6.4 cm diameter). 60Co measurements are comparable between the PMTs, but can be significantly reduced in future R11410 MOD units through further material selection. Assuming PMT activity equal to the measured 90% upper limits, Monte Carlo estimates indicate that replacement of R8778 PMTs with R11410 MOD PMTs will change LUX PMT electron recoil background contributions by a factor of times1/25 after further material selection for 60Co reduction, and nuclear recoil backgrounds by a factor of times 1/36. The strong reduction in backgrounds below the measured R8778 levels makes the R11410 MOD a very competitive technology for use in large-scale liquid xenon detectors.
We successfully developed a new photomultiplier tube (PMT) with a three-inch diameter, convex-shaped photocathode, R13111. Its prominent features include good performance and ultra-low radioactivity. The convex-shaped photocathode realized a large photon acceptance and good timing resolution. Low radioactivity was achieved by three factors: (1) the glass material was synthesized using low-radioactive-contamination material; (2) the photocathode was produced with $^{39}$K-enriched potassium; and (3) the purest grade of aluminum material was used for the vacuum seal. As a result each R13111 PMT contains only about 0.4 mBq of $^{226}$Ra, less than 2 mBq of $^{238}$U, 0.3 mBq of $^{228}$Ra, 2 mBq of $^{40}$K and 0.2 mBq of $^{60}$Co. We also examined and resolved the intrinsic leakage of Xe gas into PMTs that was observed in several older models. We thus succeeded in developing a PMT that has low background, large angular acceptance with high collection efficiency, good timing resolution, and long-term stable operation. These features are highly desirable for experiments searching for rare events beyond the standard model, such as dark matter particle interactions and neutrinoless double beta decay events.
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