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Register a new userSemi-classical model for the dephasing of a two-electron spin qubit coupled to a coherently evolving nuclear spin bath
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We study electron spin decoherence in a two-electron double quantum dot due to the hyperfine interaction, under spin-echo conditions as studied in recent experiments. We develop a semi-classical model for the interaction between the electron and nuclear spins, in which the time-dependent Overhauser fields induced by the nuclear spins are treated as classical vector variables. Comparison of the model with experimentally-obtained echo signals allows us to quantify the contributions of various processes such as coherent Larmor precession and spin diffusion to the nuclear spin evolution.
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The quantum coherence and gate fidelity of electron spin qubits in semiconductors is often limited by noise arising from coupling to a bath of nuclear spins. Isotopic enrichment of spin-zero nuclei such as $^{28}$Si has led to spectacular improvements of the dephasing time $T_2^*$ which, surprisingly, can extend two orders of magnitude beyond theoretical expectations. Using a single-atom $^{31}$P qubit in enriched $^{28}$Si, we show that the abnormally long $T_2^*$ is due to the controllable freezing of the dynamics of the residual $^{29}$Si nuclei close to the donor. Our conclusions are supported by a nearly parameter-free modeling of the $^{29}$Si nuclear spin dynamics, which reveals the degree of back-action provided by the electron spin as it interacts with the nuclear bath. This study clarifies the limits of ergodic assumptions in analyzing many-body spin-problems under conditions of strong, frequent measurement, and provides novel strategies for maximizing coherence and gate fidelity of spin qubits in semiconductors.
The main source of decoherence for an electron spin confined to a quantum dot is the hyperfine interaction with nuclear spins. To analyze this process theoretically we diagonalize the central spin Hamiltonian in the high magnetic B-field limit. Then we project the eigenstates onto an unpolarized state of the nuclear bath and find that the resulting density of states has Gaussian tails. The level spacing of the nuclear sublevels is exponentially small in the middle of each of the two electron Zeeman levels but increases super-exponentially away from the center. This suggests to select states from the wings of the distribution when the system is projected on a single eigenstate by a measurement to reduce the noise of the nuclear spin bath. This theory is valid when the external magnetic field is larger than a typical Overhauser field at high nuclear spin temperature.
The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond the ubiquitous spin 1/2 approximation for nuclear spins and present a comprehensive theoretical framework for an optically driven electron spin in a self-assembled quantum dot coupled to a nuclear spin bath of arbitrary spin. Using a dynamical mean-field approach, we compute the nuclear spin polarization distribution with and without the quadrupolar coupling. We find that while hyperfine interactions drive dynamic nuclear polarization and mode-locking, quadrupolar couplings counteract these effects. The tension between these mechanisms is imprinted on the steady-state electron spin evolution, providing a way to measure the importance of quadrupolar interactions in a quantum dot. Our results show that higher-spin effects such as quadrupolar interactions can have a significant impact on the generation of dynamic nuclear polarization and how it influences the electron spin evolution.
We apply the time-convolutionless (TCL) projection operator technique to the model of a central spin which is coupled to a spin bath via nonuniform Heisenberg interaction. The second-order results of the TCL method for the coherences and populations of the central spin are determined analytically and compared with numerical simulations of the full von Neumann equation of the total system. The TCL approach is found to yield an excellent approximation in the strong field regime for the description of both the short-time dynamics and the long time behavior.
Coherent spin states in semiconductor quantum dots offer promise as electrically controllable quantum bits (qubits) with scalable fabrication. For few-electron quantum dots made from gallium arsenide (GaAs), fluctuating nuclear spins in the host lattice are the dominant source of spin decoherence. We report a method of preparing the nuclear spin environment that suppresses the relevant component of nuclear spin fluctuations below its equilibrium value by a factor of ~ 70, extending the inhomogeneous dephasing time for the two-electron spin state beyond 1 microsecond. The nuclear state can be readily prepared by electrical gate manipulation and persists for > 10 seconds.
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