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Water deuterium fractionation in the low-mass protostar NGC1333-IRAS2A

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 Added by Fang-Chun Liu
 Publication date 2011
  fields Physics
and research's language is English




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Although deuterium enrichment of water may provide an essential piece of information in the understanding of the formation of comets and protoplanetary systems, only a few studies up to now have aimed at deriving the HDO/H2O ratio in low-mass star forming regions. Previous studies of the molecular deuteration toward the solar-type class 0 protostar, IRAS 16293-2422, have shown that the D/H ratio of water is significantly lower than other grain-surface-formed molecules. It is not clear if this property is general or particular to this source. In order to see if the results toward IRAS 16293-2422 are particular, we aimed at studying water deuterium fractionation in a second low-mass solar-type protostar, NGC1333-IRAS2A. Using the 1-D radiative transfer code RATRAN, we analyzed five HDO transitions observed with the IRAM 30m, JCMT, and APEX telescopes. We assumed that the abundance profile of HDO in the envelope is a step function, with two different values in the inner warm (T>100 K) and outer cold (T<100 K) regions of the protostellar envelope. The inner and outer abundance of HDO is found to be well constrained at the 3 sigma level. The obtained HDO inner and outer fractional abundances are x_in=6.6e-8 - 1e-7 and x_out=9e-11 - 1.8e-9 (3 sigma). These values are close to those in IRAS 16293-2422, which suggests that HDO may be formed by the same mechanisms in these two solar-type protostars. Taking into account the (rather poorly constrained) H2O abundance profile deduced from Herschel observations, the derived HDO/H2O in the inner envelope is larger than 1% and in the outer envelope it is 0.9%-18%. These values are more than one order of magnitude higher than what is measured in comets. If the same ratios apply to the protosolar nebula, this would imply that there is some efficient reprocessing of the material between the protostellar and cometary phases. The H2O inner fractional [...]



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92 - Ruud Visser 2013
Evaporation of water ice above 100 K in the inner few 100 AU of low-mass embedded protostars (the so-called hot core) should produce quiescent water vapor abundances of ~10^-4 relative to H2. Observational evidence so far points at abundances of only a few 10^-6. However, these values are based on spherical models, which are known from interferometric studies to be inaccurate on the relevant spatial scales. Are hot cores really that much drier than expected, or are the low abundances an artifact of the inaccurate physical models? We present deep velocity-resolved Herschel-HIFI spectra of the 3(12)-3(03) lines of H2-16O and H2-18O (1097 GHz, Eup/k = 249 K) in the low-mass Class 0 protostar NGC1333 IRAS2A. A spherical radiative transfer model with a power-law density profile is unable to reproduce both the HIFI data and existing interferometric data on the H2-18O 3(13)-2(20) line (203 GHz, Eup/k = 204 K). Instead, the HIFI spectra likely show optically thick emission from a hot core with a radius of about 100 AU. The mass of the hot core is estimated from the C18O J=9-8 and 10-9 lines. We derive a lower limit to the hot water abundance of 2x10^-5, consistent with the theoretical predictions of ~10^-4. The revised HDO/H2O abundance ratio is 1x10^-3, an order of magnitude lower than previously estimated.
Water plays a crucial role both in the interstellar medium and on Earth. To constrain its formation mechanisms and its evolution through the star formation process, the determination of the water deuterium fractionation ratios is particularly suitable. Previous studies derived HDO/H$_2$O ratios in the warm inner regions of low-mass protostars. We here report a detection of the D$_2$O 1$_{1,0}$-1$_{0,1}$ transition toward the low-mass protostar NGC1333 IRAS2A with the Plateau de Bure interferometer: this represents the first interferometric detection of D$_2$O - and only the second solar-type protostar for which this isotopologue is detected. Using the observations of the HDO 5$_{4,2}$-6$_{3,3}$ transition simultaneously detected and three other HDO lines previously observed, we show that the HDO line fluxes are well reproduced with a single excitation temperature of 218$pm$21 K and a source size of $sim$0.5 arcsec. The D$_2$O/HDO ratio is $sim$(1.2$pm$0.5) $times$ 10$^{-2}$, while the use of previous H$_2^{18}$O observations give an HDO/H$_2$O ratio of $sim$(1.7$pm$0.8) $times$ 10$^{-3}$, i.e. a factor of 7 lower than the D$_2$O/HDO ratio. These results contradict the predictions of current grain surface chemical models and indicate that either the surface deuteration processes are poorly understood or that both sublimation of grain mantles and water formation at high temperatures ($gtrsim$230 K) take place in the inner regions of this source. In the second scenario, the thermal desorption of the grain mantles would explain the high D$_2$O/HDO ratio, while water formation at high temperature would explain significant extra production of H$_2$O leading to a decrease of the HDO/H$_2$O ratio.
The [HDO]/[H2O] ratio is a crucial parameter for probing the history of water formation. So far, it has been measured for only three solar type protostars and yielded different results, possibly pointing to a substantially different history in their formation. In the present work, we report new interferometric observations of the HDO 4 2,2 - 4 2,3 line for two solar type protostars, IRAS2A and IRAS4A, located in the NGC1333 region. In both sources, the detected HDO emission originates from a central compact unresolved region. Comparison with previously published interferometric observations of the H218$O 3 1,3 - 2 2,0 line shows that the HDO and H$_2$O lines mostly come from the same region. A non-LTE LVG analysis of the HDO and H218$O line emissions, combined with published observations, provides a [HDO]/[H2O] ratio of 0.3 - 8 % in IRAS2A and 0.5 - 3 % in IRAS4A. First, the water fractionation is lower than that of other molecules such as formaldehyde and methanol in the same sources. Second, it is similar to that measured in the solar type protostar prototype, IRAS16293-2422, and, surprisingly enough, larger than that measured in NGC1333 IRAS4B. {The comparison of the measured values towards IRAS2A and IRAS4A with the predictions of our gas-grain model GRAINOBLE gives similar conclusions to those for IRAS 16293, arguing that these protostars {share} a similar chemical history, although they are located in different clouds.
The HDO/H2O ratio is a powerful diagnostic to understand the evolution of water from the first stages of star formation to the formation of planets and comets. Our aim is to determine precisely the abundance distribution of HDO towards the low-mass protostar IRAS16293-2422 and learn more about the water formation mechanisms by determining the HDO/H2O abundance ratio. A spectral survey of the source IRAS16293-2422 was carried out in the framework of the CHESS Herschel Key program with the HIFI instrument, allowing the detection of numerous HDO lines. Other transitions have been observed previously with ground-based telescopes. The spherical Monte Carlo radiative transfer code RATRAN was used to reproduce the observed line profiles of HDO by assuming an abundance jump. To determine the H2O abundance throughout the envelope, a similar study was made of the H2-18O observed lines, as the H2O main isotope lines are contaminated by the outflows. We derive an inner HDO abundance of 1.7e-7 and an outer HDO abundance of 8e-11. To reproduce the HDO absorption lines, it is necessary to add an absorbing layer in front of the envelope. It may correspond to a water-rich layer created by the photodesorption of the ices at the edges of the molecular cloud. The HDO/H2O ratio is ~1.4-5.8% in the hot corino whereas it is ~0.2-2.2% in the outer envelope. It is estimated at ~4.8% in the added absorbing layer. Although it is clearly higher than the cosmic D/H abundance, the HDO/H2O ratio remains lower than the D/H ratio derived for other deuterated molecules observed in the same source. The similarity of the ratios derived in the hot corino and in the added absorbing layer suggests that water formed before the gravitational collapse of the protostar, contrary to formaldehyde and methanol, which formed later once the CO molecules had depleted on the grains.
The low mass protostar IRAS 16293$-$2422 is a well-known young stellar system that is observed in the L1689N molecular cloud in the constellation of Ophiuchus. In the interstellar medium and solar system bodies, water is a necessary species for the formation of life. We present the spectroscopic detection of the rotational emission line of water (H$_{2}$O) vapour from the low mass protostar IRAS 16293$-$2422 using the Atacama Large Millimeter/submillimeter Array (ALMA) band 5 observation. The emission line of H$_{2}$O is detected at frequency $ u$ = 183.310 GHz with transition J=3$_{1,3}$$-$2$_{2,2}$. The statistical column density of the emission line of water vapour is $N$(H$_{2}$O) = 4.2$times$10$^{16}$ cm$^{-2}$ with excitation temperature ($T_{ex}$) = 124$pm$10 K. The fractional abundance of H$_{2}$O with respect to H$_{2}$ is 1.44$times$10$^{-7}$ where $N$(H$_{2}$) = 2.9$times$10$^{23}$ cm$^{-2}$.
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