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Register a new userAccessing the transport properties of graphene and its multi-layers at high carrier density
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We present a comparative study of high carrier density transport in mono-, bi-, and trilayer graphene using electric-double-layer transistors to continuously tune the carrier density up to values exceeding 10^{14} cm^{-2}. Whereas in monolayer the conductivity saturates, in bi- and trilayer flling of the higher energy bands is observed to cause a non-monotonic behavior of the conductivity, and a large increase in the quantum capacitance. These systematic trends not only show how the intrinsic high-density transport properties of graphene can be accessed by field-effect, but also demonstrate the robustness of ion-gated graphene, which is crucial for possible future applications.
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We report a multiband transport study of bilayer graphene at high carrier densities. Employing a poly(ethylene)oxide-CsClO$_4$ solid polymer electrolyte gate we demonstrate the filling of the high energy subbands in bilayer graphene samples at carrier densities $|n|geq2.4times 10^{13}$ cm$^{-2}$. We observe a sudden increase of resistance and the onset of a second family of Shubnikov de Haas (SdH) oscillations as these high energy subbands are populated. From simultaneous Hall and magnetoresistance measurements together with SdH oscillations in the multiband conduction regime, we deduce the carrier densities and mobilities for the higher energy bands separately and find the mobilities to be at least a factor of two higher than those in the low energy bands.
Variable-field Hall measurements were performed on epitaxial graphene grown on Si-face and C-face SiC. The carrier transport involves essentially a single-type of carrier in few-layer graphene, regardless of SiC face. However, in multi-layer graphene (MLG) grown on C-face SiC, the Hall measurements indicated the existence of several groups of carriers with distinct mobilities. Electrical transport in MLG can be properly described by invoking three independent conduction channels in parallel. Two of these are n- and p-type, while the third involves nearly intrinsic graphene. The carriers in this lightly doped channel have significantly higher mobilities than the other two.
Chiral symmetry, fundamental in the physics of graphene, guarantees the existence of topologically stable doubled Dirac cones and anomalous behaviors of the zero-energy Landau level in magnetic fields. The crucial role is inherited in the optical responses and many-body physics in graphene, which are explained in this paper. We also give an overview of multilayer graphene from the viewpoint of the optical properties and their relation with the chiral symmetry.
One of the enduring challenges in graphene research and applications is the extreme sensitivity of its charge carriers to external perturbations, especially those introduced by the substrate. The best available substrates to date, graphite and hBN, still pose limitations: graphite being metallic does not allow gating, while both hBN and graphite having lattice structures closely matched to that of graphene, may cause significant band structure reconstruction. Here we show that the atomically smooth surface of exfoliated MoS2 provides access to the intrinsic electronic structure of graphene without these drawbacks. Using scanning tunneling microscopy and Landau-level spectroscopy in a device configuration which allows tuning the carrier concentration, we find that graphene on MoS2 is ultra-flat producing long mean free paths, while avoiding band structure reconstruction. Importantly, the screening of the MoS2 substrate can be tuned by changing the position of the Fermi energy with relatively low gate voltages. We show that shifting the Fermi energy from the gap to the edge of the conduction band gives rise to enhanced screening and to a substantial increase in the mean-free-path and quasiparticle lifetime. MoS2 substrates thus provide unique opportunities to access the intrinsic electronic properties of graphene and to study in situ the effects of screening on electron-electron interactions and transport.
The specific band structure of graphene, with its unique valley structure and Dirac neutrality point separating hole states from electron states has led to the observation of new electronic transport phenomena such as anomalously quantized Hall effects, absence of weak localization and the existence of a minimum conductivity. In addition to dissipative transport also supercurrent transport has already been observed. It has also been suggested that graphene might be a promising material for spintronics and related applications, such as the realization of spin qubits, due to the low intrinsic spin orbit interaction, as well as the low hyperfine interaction of the electron spins with the carbon nuclei. As a first step in the direction of graphene spintronics and spin qubits we report the observation of spin transport, as well as Larmor spin precession over micrometer long distances using single graphene layer based field effect transistors. The non-local spin valve geometry was used, employing four terminal contact geometries with ferromagnetic cobalt electrodes, which make contact to the graphene sheet through a thin oxide layer. We observe clear bipolar (changing from positive to negative sign) spin signals which reflect the magnetization direction of all 4 electrodes, indicating that spin coherence extends underneath all 4 contacts. No significant changes in the spin signals occur between 4.2K, 77K and room temperature. From Hanle type spin precession measurements we extract a spin relaxation length between 1.5 and 2 micron at room temperature, only weakly dependent on charge density, which is varied from n~0 at the Dirac neutrality point to n = 3.6 10^16/m^2. The spin polarization of the ferromagnetic contacts is calculated from the measurements to be around 10%.
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