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Register a new userMagnetism and superconductivity driven by identical 4$f$ states in a heavy-fermion metal
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The apparently inimical relationship between magnetism and superconductivity has come under increasing scrutiny in a wide range of material classes, where the free energy landscape conspires to bring them in close proximity to each other. This is particularly the case when these phases microscopically interpenetrate, though the manner in which this can be accomplished remains to be fully comprehended. Here, we present combined measurements of elastic neutron scattering, magnetotransport, and heat capacity on a prototypical heavy fermion system, in which antiferromagnetism and superconductivity are observed. Monitoring the response of these states to the presence of the other, as well as to external thermal and magnetic perturbations, points to the possibility that they emerge from different parts of the Fermi surface. This enables a single 4$f$ state to be both localized and itinerant, thus accounting for the coexistence of magnetism and superconductivity.
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The interplay of magnetism and unconventional superconductivity (d singlet wave or p triplet wave) in strongly correlated electronic system (SCES) is discussed with recent examples found in heavy fermion compounds. A short presentation is given on the formation of the heavy quasiparticle with the two sources of a local and intersite enhancement for the effective mass. Two cases of the coexistence or repulsion of antiferromagnetism and superconductivity are given with CeIn3 and CeCoIn5. A spectacular example is the emergence of superconductivity in relatively strong itinerant ferromagnets UGe2 and URhGe. The impact of heavy fermion matter among other SCES as organic conductor or high Tc oxide is briefly pointed out.
In this document, I present a personal view on the heavy-fermion problem, within a phenomenological approach guided by experiments. This review presents a set of historical works which established the ground bases of the thematic during the last decades. An exhaustive and systematic approach is privileged. After a general presentation in Chapter 2, the properties of heavy-fermion paramagnets, antiferromagnets, and ferromagnets are considered in Chapters 3, 4, and 5, respectively. Chapters 6 and 7 are dedicated to two specific compounds, URu$_2$Si$_2$ for which a hidden-order phase constitutes a more-than-thirty-years-old unsolved mystery, and UTe$_2$, where multiple superconducting phases have been discovered in the last two years. Experiments performed using a panel of techniques ranging from microscopic (neutron scattering, NMR, etc.) to thermodynamic (specific heat, magnetization, etc.) and transport (electrical resistivity, etc.) probes, under extreme conditions of low temperatures, intense magnetic fields and high pressures, are reviewed. They show that magnetism plays a central role in the quantum critical properties of heavy-fermion systems. An emphasis is given to the intersite magnetic fluctuations, presented as the driving force for a heavy Fermi liquid, precursor of quantum magnetic criticality ending in magnetically-ordered phases. They are also suspected to drive an unconventional mechanism for superconductivity, which develops in the vicinity of quantum magnetic phase transitions induced under pressure or magnetic field. The appearance of magnetic fluctuations and ultimately magnetic order in heavy-fermion compounds occurs in a nearly-integer-valence regime, in which $f$ electrons have a dual itinerant-localized character. Fermi-surface and valence studies, which give complementary information about this duality, are also considered.
We review magnetic, superconducting and non-Fermi-liquid properties of the structurally layered heavy-fermion compounds Ce$_n$M$_m$In$_{3n+2m}$ (M=Co, Rh, Ir). These properties suggest d-wave superconductivity and proximity to an antiferromagetic quantum-critical point.
This article reviews recent results of magnetotransport and magnetization measurements performed on highly oriented pyrolitic graphite (HOPG) and single crystalline Kish graphite samples. Both metal-insulator and insulator-metal transitions driven by magnetic field applied perpendicular to the basal planes of graphite were found and discussed in the light of relevant theories. The results provide evidence for the existence of localized superconducting domains in HOPG even at room temperature, as well as an interplay between superconducting and ferromagnetic correlations. We also present experimental evidence for the superconductivity occurrence in graphite-sulfur composites.
We grew single crystals of the recently discovered heavy fermion superconductor UTe2, and measured the resistivity, specific heat and magnetoresistance. Superconductivity (SC) was clearly detected at Tsc=1.65K as sharp drop of the resistivity in a high quality sample of RRR=35. The specific heat shows a large jump at Tsc indicating strong coupling. The large Sommerfeld coefficient, 117mJ K-2mol-1 extrapolated in the normal state and the temperature dependence of C/T below Tsc are the signature of unconventional SC. The discrepancy in the entropy balance at Tsc between SC and normal states points out that hidden features must occur. Surprisingly, a large residual value of the Sommerfeld coefficient seems quite robust (gamma_0/gamma ~ 0.5). The large upper critical field Hc2 along the three principal axes favors spin-triplet SC. For H // b-axis, our experiments do not reproduce the huge upturn of Hc2 reported previously. This discrepancy may reflect that Hc2 is very sensitive to the sample quality. A new perspective in UTe2 is the proximity of a Kondo semiconducting phase predicted by the LDA band structure calculations.
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