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Register a new userUnravelling the glue and the competing order in superconducting cuprates
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We present Raman scattering experiments in ${rm La_{2-x}Sr_xCuO_4}$ single crystals at various doping levels x and compare the results with theoretical predictions obtained assuming an interaction mediated by spin and charge fluctuations. The light-scattering selection rules allow us to disentangle their respective contributions. We find that the glue spectral function is spin-dominated at low doping while the contribution of charge fluctuations becomes dominant around optimal doping. This indicates that the fluctuations of a nearly ordered state with coexisting spin and charge order support the superconducting pairing.
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A grand challenge in many-body quantum physics is to explain the apparent connection between quantum criticality and high-temperature superconductivity in the cuprates and similar systems, such as the iron pnictides and chalcogenides. Here we argue that the quantum-critical regime plays an essential role in activating a strong-pairing mechanism: although pairing bosons create a symmetry-breaking instability which suppresses pairing, the combination of these broken-symmetry states within the critical regime can restore this symmetry for the paired quasiparticles. This condition is shown to be met within a large-U ansatz. A hidden quantum phase transition then arises between a Fermi-liquid and a non-Fermi-liquid broken-symmetry striped state, and a critical regime in which the broken-symmetry states are combined.
We have studied the momentum dependence of the energy gap of Bi2(Sr,R)2CuOy by angleresolved photoemission spectroscopy (ARPES), particularly focusing on the difference between R=La and Eu. By comparing the gap function and characteristic temperatures between the two sets of samples, we show that there exist three distinct energy scales, {Delta}pg, {Delta}sc0, and {Delta}eff sc0, which correspond to T* (pseudogap temperature), Tonset (onset temperature of fluctuating superconductivity), and Tc (critical temperature of coherent superconductivity). The results not only support the existence of a pseudogap state below T* that competes with superconductivity but also the duality of competition and superconducting fluctuation at momenta around the antinode below Tonset.
Along with some other researches we have realised that the true origin of high-temperature superconductivity should be found in the strong Coulomb repulsion combined with a significant electronphonon interaction. Both interactions are strong (on the order of 1 eV) compared with the low Fermi energy of doped carries which makes the conventional BCS-Eliashberg theory inapplicable in cuprates and related doped insulators. Based on our recent analytical and numerical results I argue that high-temperature superconductivity from repulsion is impossible for any strength of the Coulomb interaction. Major steps of our alternative polaronic theory are outlined starting from the generic Hamiltonian with the unscreened (bare) Coulomb and electron-phonon interactions accounting for critical temperatures of high-temperature superconductors without any adjustable parameters.
Angle-dependent studies of the gap function provide evidence for the coexistence of two distinct gaps in hole doped cuprates, where the gap near the nodal direction scales with the superconducting transition temperature $T_c$, while that in the antinodal direction scales with the pseudogap temperature. We present model calculations which show that most of the characteristic features observed in the recent angle-resolved photoemission spectroscopy (ARPES) as well as scanning tunneling microscopy (STM) two-gap studies are consistent with a scenario in which the pseudogap has a non-superconducting origin in a competing phase. Our analysis indicates that, near optimal doping, superconductivity can quench the competing order at low temperatures, and that some of the key differences observed between the STM and ARPES results can give insight into the superlattice symmetry of the competing order.
In strongly correlated materials the electronic and optical properties are significantly affected by the coupling of fermionic quasiparticles to different degrees of freedom, such as lattice vibrations and bosonic excitations of electronic origin. Broadband ultrafast spectroscopy is emerging as the premier technique to unravel the subtle interplay between quasiparticles and electronic or phononic collective excitations, by their different characteristic timescales and spectral responses. By investigating the femtosecond dynamics of the optical properties of Y-Bi2212 crystals over the 0.5-2 eV energy range, we disentangle the electronic and phononic contributions to the generalized electron-boson Eliashberg function, showing that the spectral distribution of the electronic excitations, such as spin fluctuations and current loops, and the strength of their interaction with quasiparticles can account for the high critical temperature of the superconducting phase transition. Finally, we discuss how the use of this technique can be extended to the underdoped region of the phase diagram of cuprates, in which a pseudogap in the quasiparticle density of states opens. The microscopic modeling of the interaction of ultrashort light pulses with unconventional superconductors will be one of the key challenges of the next-years materials science, eventually leading to the full understanding of the role of the electronic correlations in controlling the dynamics on the femtosecond timescale.
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