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Performance of ZnMoO4 crystal as cryogenic scintillating bolometer to search for double beta decay of molybdenum

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 Added by Stefano Pirro
 Publication date 2010
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and research's language is English




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Zinc molybdate (ZnMoO4) single crystals were grown for the first time by the Czochralski method and their luminescence was measured under X ray excitation in the temperature range 85-400 K. Properties of ZnMoO4 crystal as cryogenic low temperature scintillator were checked for the first time. Radioactive contamination of the ZnMoO4 crystal was estimated as <0.3 mBq/kg (228-Th) and 8 mBq/kg (226-Ra). Thanks to the simultaneous measurement of the scintillation light and the phonon signal, the alpha particles can be discriminated from the gamma/beta interactions, making this compound extremely promising for the search of neutrinoless Double Beta Decay of 100-Mo. We also report on the ability to discriminate the alpha-induced background without the light measurement, thanks to a different shape of the thermal signal that characterizes gamma/beta and alpha particle interactions.



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Bolometers are ideal devices in the search for neutrinoless Double Beta Decay. Enlarging the mass of individual detectors would simplify the construction of a large experiment, but would also decrease the background per unit mass induced by alpha-emitters located close to the surfaces and background arising from external and internal gammas. We present the very promising results obtained with a 2.13 kg TeO2 crystal. This bolometer, cooled down to a temperature of 10.5 mK in a dilution refrigerator located deep underground in the Gran Sasso National Laboratories, represents the largest thermal detector ever operated. The detector exhibited an energy resolution spanning a range from 3.9 keV (at 145 keV) to 7.8 keV (at the 2615 gamma-line of 208Tl) FWHM. We discuss the decrease in the background per unit mass that can be achieved increasing the mass of a bolometer.
We present the performances of a 330 g zinc molybdate (ZnMoO4) crystal working as scintillating bolometer as a possible candidate for a next generation experiment to search for neutrinoless double beta decay of 100Mo. The energy resolution, evaluated at the 2615 keV gamma-line of 208Tl, is 6.3 keV FWHM. The internal radioactive contaminations of the ZnMoO4 were evaluated as <6 microBq/kg (228Th) and 27pm6 microBq/kg (226Ra). We also present the results of the alpha vs beta/gamma discrimination, obtained through the scintillation light as well as through the study of the shape of the thermal signal alone.
We investigate the performances of two ZnMoO4 scintillating crystals operated as bolometers, in view of a next generation experiment to search the neutrinoless double beta decay of Mo-100. We present the results of the alpha vs beta/gamma discrimination, obtained through the scintillation light as well as through the study of the shape of the thermal signal alone. The discrimination capability obtained at the 2615 keV line of Tl-208 is 8 sigma, using the heat-light scatter plot, while it exceeds 20 sigma using the shape of the thermal pulse alone. The achieved FWHM energy resolution ranges from 2.4 keV (at 238 keV) to 5.7 keV (at 2615 keV). The internal radioactive contaminations of the ZnMoO4 crystals were evaluated through a 407 hours background measurement. The obtained limit is < 32 microBq/kg for Th-228 and Ra-226. These values were used for a Monte Carlo simulation aimed at evaluating the achievable background level of a possible, future array of enriched ZnMoO4 crystals.
We present the results obtained in the development of scintillating Double Beta Decay bolometers. Several Mo and Cd based crystals were tested with the bolometric technique. The scintillation light was measured through a second independent bolometer. A 140 g CdWO_4 crystal was run in a 417 h live time measurement. Thanks to the scintillation light, the alpha background is easily discriminated resulting in zero counts above the 2615 keV gamma line of Thallium 208. These results, combined with an extremely easy light detector operation, represent the first tangible proof demonstrating the feasibility of this kind of technique.
We report the performances of a 0.51 kg CdWO4 scintillating bolometer to be used for future Double Beta Decay Experiments. The simultaneous read-out of the heat and the scintillation light allows to discriminate between different interacting particles aiming at the disentanglement and the reduction of background contribution, key issue for next generation experiments. We will describe the observed anticorrelation between the heat and the light signal and we will show how this feature can be used in order to increase the energy resolution of the bolometer over the entire energy spectrum, improving up to a factor 2.6 on the 2615 keV line of 208Tl. The detector was tested in a 433 h background measurement that permitted to estimate extremely low internal trace contaminations of 232Th and 238U. The light yield of gamma/beta, alpha and neutrons is presented. Furthermore we developed a method in order to correctly evaluate the absolute thermal quenching factor of alpha particles in scintillating bolometers.
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