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Register a new userSuppression of critical temperature in Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ with point defects introduced by proton irradiation
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We report the effect of 3 MeV proton irradiation on the suppression of the critical temperature $T_{c}$ in Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ single crystals at under-, optimal-, and over-doping levels. We find that $T_{c}$ decreases and residual resistivity increases monotonically with increasing dose. We also find no upturn in low-temperature resistivity in contrast with the $yen alpha$-particle irradiated NdFeAs(O,F), which suggests that defects induced by the proton irradiation behave as nonmagnetic scattering centers. The critical scattering rate for all samples estimated by three different ways is much higher than that expected in $s_{yen pm}$-pairing scenario based on inter-band scattering due to antiferro-magnetic spin fluctuation.
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We report the first realization of columnar defects in Co-doped BaFe$_{2}$As$_{2}$ single crystals by heavy-iron irradiation. The columnar defects are confirmed by transmission electron microscopy and their density is about 40 % of the irradiation dose. Magneto-optical imaging and bulk magnetization measurements reveal that the critical current density is strongly enhanced in the irradiated region. We also find that vortex creep rates are strongly suppressed by the columnar defects. We compare the effect of heavy-ion irradiation into Co-doped BaFe$_{2}$As$_{2}$ and cuprate superconductors.
We observed the anisotropic superconducting-gap (SC-gap) structure of a slightly overdoped superconductor, Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ ($x=0.1$), using three-dimensional (3D) angle-resolved photoemission spectroscopy. Two hole Fermi surfaces (FSs) observed at the Brillouin zone center and an inner electron FS at the zone corner showed a nearly isotropic SC gap in 3D momentum space. However, the outer electron FS showed an anisotropic SC gap with nodes or gap minima around the M and A points. The different anisotropies obtained the SC gap between the outer and inner electron FSs cannot be expected from all theoretical predictions with spin fluctuation, orbital fluctuation, and both competition. Our results provide a new insight into the SC mechanisms of iron pnictide superconductors.
By means of infrared spectroscopy we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$. The Fano parameter $1/q^2$, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic/structural orderings at low temperatures. More strikingly, at elevated temperatures in the paramagnetic/tetragonal state we find a linear correlation between $1/q^2$ and the superconducting critical temperature $T_c$. Based on theoretical calculations and symmetry considerations, we identify the relevant interband transitions that are coupled to the Fe-As mode. In particular, we show that a sizable $xy$ orbital component at the Fermi level is fundamental for the Fano effect and possibly also for the superconducting pairing.
We investigate magnetic ordering in metallic Ba[Fe(1-x)Mn(x)](2)As(2) and discuss the unusual magnetic phase, which was recently discovered for Mn concentrations x > 10%. We argue that it can be understood as a Griffiths-type phase that forms above the quantum critical point associated with the suppression of the stripe-antiferromagnetic spin-density-wave (SDW) order in BaFe2As2 by the randomly introduced localized Mn moments acting as strong magnetic impurities. While the SDW transition at x = 0, 2.5% and 5% remains equally sharp, in the x = 12% sample we observe an abrupt smearing of the antiferromagnetic transition in temperature and a considerable suppression of the spin gap in the magnetic excitation spectrum. According to our muon-spin-relaxation, nuclear magnetic resonance and neutron-scattering data, antiferromagnetically ordered rare regions start forming in the x = 12% sample significantly above the Neel temperature of the parent compound. Upon cooling, their volume grows continuously, leading to an increase in the magnetic Bragg intensity and to the gradual opening of a partial spin gap in the magnetic excitation spectrum. Using neutron Larmor diffraction, we also demonstrate that the magnetically ordered volume is characterized by a finite orthorhombic distortion, which could not be resolved in previous diffraction studies most probably due to its coexistence with the tetragonal phase and a microstrain-induced broadening of the Bragg reflections. We argue that Ba[Fe(1-x)Mn(x)](2)As(2) could represent an interesting model spin-glass system, in which localized magnetic moments are randomly embedded into a SDW metal with Fermi surface nesting.
We used angle-resolved photoemission spectroscopy (ARPES) and density functional theory calculations to study the electronic structure of Ba(Fe1-x-yCoxMny)2As2 for x=0.06 and 0<=y <=0.07. From ARPES we derive that the substitution of Fe by Mn does not lead to hole doping, indicating a localization of the induced holes. An evaluation of the measured spectral function does not indicate a diverging effective mass or scattering rate near optimal doping. Thus the present ARPES results indicate a continuous evolution of the quasiparticle interaction and therefore question previous quantum critical scenarios.
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