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Stark effect and generalized Bloch-Siegert shift in a strongly driven two-level system

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 Added by Mika Sillanpaa
 Publication date 2010
  fields Physics
and research's language is English




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A superconducting qubit was driven in an ultrastrong fashion by an oscillatory microwave field, which was created by coupling via the nonlinear Josephson energy. The observed Stark shifts of the `atomic levels are so pronounced that corrections even beyond the lowest-order Bloch-Siegert shift are needed to properly explain the measurements. The quasienergies of the dressed two-level system were probed by resonant absorption via a cavity, and the results are in agreement with a calculation based on the Floquet approach.



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We measure the dispersive energy-level shift of an $LC$ resonator magnetically coupled to a superconducting qubit, which clearly shows that our system operates in the ultrastrong coupling regime. The large mutual kinetic inductance provides a coupling energy of $approx0.82$~GHz, requiring the addition of counter-rotating-wave terms in the description of the Jaynes-Cummings model. We find a 50~MHz Bloch-Siegert shift when the qubit is in its symmetry point, fully consistent with our analytical model.
Coherent light-matter interaction can be used to manipulate the energy levels of atoms, molecules and solids. When light with frequency {omega} is detuned away from a resonance {omega}o, repulsion between the photon-dressed (Floquet) states can lead to a shift of energy resonance. The dominant effect is the optical Stark shift (1/({omega}0-{omega})), but there is an additional contribution from the so-called Bloch-Siegert shift (1/({omega}o+{omega})). Although it is common in atoms and molecules, the observation of Bloch-Siegert shift in solids has so far been limited only to artificial atoms since the shifts were small (<1 {mu}eV) and inseparable from the optical Stark shift. Here we observe an exceptionally large Bloch-Siegert shift (~10 meV) in monolayer WS2 under infrared optical driving by virtue of the strong light-matter interaction in this system. Moreover, we can disentangle the Bloch-Siegert shift entirely from the optical Stark shift, because the two effects are found to obey opposite selection rules at different valleys. By controlling the light helicity, we can confine the Bloch-Siegert shift to occur only at one valley, and the optical Stark shift at the other valley. Such a valley-exclusive Bloch-Siegert shift allows for enhanced control over the valleytronic properties in two-dimensional materials, and offers a new avenue to explore quantum optics in solids.
We study the coherent dynamics of a qubit excited by an amplitude-modulated electromagnetic field under the Rabi resonance when the frequency of the low-frequency modulation field matches the Rabi frequency in the high-frequency field. Due to destructive interference of multiple photon processes at the ultrastrong coupling between the qubit and the low-frequency driving field, Rabi oscillations result exclusively from the Bloch-Siegert effect. It is directly observed in the time-resolved coherent dynamics as the Bloch-Siegert oscillation. In this case, triplets in Fourier spectra of the coherent response are transformed into doublets with the splitting between the lines equal to twice the Bloch-Siegert shift. These unusual properties are demonstrated in conditions of experiments with a nitrogen vacancy center in diamond.
We have performed spectroscopic measurements of a superconducting qubit dispersively coupled to a nonlinear resonator driven by a pump microwave field. Measurements of the qubit frequency shift provide a sensitive probe of the intracavity field, yielding a precise characterization of the resonator nonlinearity. The qubit linewidth has a complex dependence on the pump frequency and amplitude, which is correlated with the gain of the nonlinear resonator operated as a small-signal amplifier. The corresponding dephasing rate is found to be close to the quantum limit in the low-gain limit of the amplifier.
We present a detailed theoretical analysis of a multi-level quantum system coupled to two radiation fields and subject to decoherence. We concentrate on an effect known from quantum optics as the Autler-Townes splitting, which has been recently demonstrated experimentally [M. A. Sillanpaa et al., Phys. Rev. Lett. 103, 193601 (2009)] in a superconducting phase qubit. In the three-level approximation, we derive analytical solutions and describe how they can be used to extract the decoherence rates and to account for the measurement data. Better agreement with the experiment can be obtained by extending this model to five levels. Finally, we investigate the stationary states created in the experiment and show that their structure is close to that of dark states.
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