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Register a new userOptomechanics of liquid crystals for dynamical optical response of photonic structures
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Added by
Andrey Miroshnichenko
Publication date
2010
fields
Physics
and research's language is
English
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We show that the mechanical effect of light on the orientational ordering of the crystalline axis of a mesophase can be used to control the dynamics of the optical response of liquid crystal infiltrated photonic structures. The demonstration is made using a one-dimensional periodic structure whose periodicity is broken by the presence of a nematic liquid crystal defect layer. In this study we report on output light polarization and/or intensity dynamics that depends on the initial molecular ordering and incident light wavelength and intensity.
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Starting from a microscopic definition of an alignment vector proportional to the polarization, we discuss the hydrodynamics of polar liquid crystals with local $C_{infty v}$-symmetry. The free energy for polar liquid crystals differs from that of nematic liquid crystals ($D_{infty h}$) in that it contains terms violating the ${bf{n}}to -{bf{n}}$ symmetry. First we show that these $mathcal{Z}_2$-odd terms induce a general splay instability of a uniform polarized state in a range of parameters. Next we use the general Poisson-bracket formalism to derive the hydrodynamic equations of the system in the polarized state. The structure of the linear hydrodynamic modes confirms the existence of the splay instability.
We model a cholesteric liquid crystal as a planar uniaxial multilayer system, where the orientation of each layer differs slightly from that of the adjacent one. This allows us to analytically simplify the otherwise acutely complicated calculation of the Casimir-Lifshitz torque. Numerical results differ appreciably from the case of nematic liquid crystals, which can be treated like bloc birefringent media. In particular, we find that the torque deviates considerably from its usual sinusoidal behavior as a function of the misalignment angle. In the case of a birefringent crystal faced with a cholesteric liquid one, the Casimir-Lifshitz torque decreases more slowly as a function of distance than in the nematic case. In the case of two cholesteric liquid crystals, either in the homochiral or in the heterochiral configuration, the angular dependence changes qualitatively as a function of distance. In all considered cases, finite pitch length effects are most pronounced at distances of about 10 nm.
The multidimensional energy surface of a cholesteric liquid crystal in a planar cell is investigated as a function of spherical coordinates determining the director orientation. Minima on the energy surface correspond to the stable states with particular director distribution. External electric and magnetic fields deform the energy surface and positions of minima. It can lead to the transitions between states, known as the Fr{e}edericksz effect. Transitions can be continuous or discontinuous depending on parameters of the liquid crystal which determine an energy surface. In a case of discontinuous transition when a barrier between stable states is comparable with the thermal energy, the activation transitions may occur and it leads to the modification of characteristics of the Fr{e}edericksz effect with temperature without explicit temperature dependencies of liquid crystal parameters. Minimum energy path between stable states on the energy surface for the Fr{e}edericksz transition is found using geodesic nudged elastic band method. Knowledge of this path, which has maximal statistical weight among all other paths, gives the information about a barrier between stable states and configuration of director orientation during the transition. It also allows one to estimate the stability of states with respect to the thermal fluctuations and their lifetime when the system is close to the Fr{e}edericksz transition.
The physics of nematic liquid crystals has been subject of intensive research since the late 19th century. However, because of the limitations of chemistry the focus has been centered around uni- and biaxial nematics associated with constituents bearing a $D_{infty h}$ or $D_{2h}$ symmetry respectively. In view of general symmetries, however, these are singularly special since nematic order can in principle involve any point group symmetry. Given the progress in tailoring nano particles with particular shapes and interactions, this vast family of generalized nematics might become accessible in the laboratory. Little is known since the order parameter theories associated with the highly symmetric point groups are remarkably complicated, involving tensor order parameters of high rank. Here we show that the generic features of the statistical physics of such systems can be studied in a highly flexible and efficient fashion using a mathematical tool borrowed from high energy physics: discrete non-Abelian gauge theory. Explicitly, we construct a family of lattice gauge models encapsulating nematic ordering of general three dimensional point group symmetries. We find that the most symmetrical generalized nematics are subjected to thermal fluctuations of unprecedented severity. As a result, novel forms of fluctuation phenomena become possible. In particular, we demonstrate that a vestigial phase carrying no more than chiral order becomes ubiquitous departing from high point group symmetry chiral building blocks, such as $I$, $O$ and $T$ symmetric matter.
Quadrupole topological phases, exhibiting protected boundary states that are themselves topological insulators of lower dimensions, have recently been of great interest. Extensions of these ideas from current tight binding models to continuum theories for realistic materials require the identification of quantized invariants describing the bulk quadrupole order. Here we identify the analog of quadrupole order in Maxwells equations for a photonic crystal (PhC) and identify quadrupole topological photonic crystals formed through a band inversion process. Unlike prior studies relying on threaded flux, our quadrupole moment is quantized purely by crystalline symmetries, which we confirm using three independent methods: analysis of symmetry eigenvalues, numerical calculations of the nested Wannier bands, and the expectation value of the quadrupole operator. Furthermore, through the bulk-edge correspondence of Wannier bands, we reveal the boundary manifestations of nontrivial quadrupole phases as quantized polarizations at edges and bound states at corners. Finally, we relate the nontrivial corner states to the emergent phenomena of quantized fractional corner charges and a filling anomaly as first predicted in electronic systems. Our work paves the way to further explore higher-order topological phases in nanophotonic systems and our method of inducing quadrupole phase transitions is also applicable to other wave systems, such as electrons, phonons and polaritons.
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