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Register a new userObserving the intrinsic linewidth of a quantum-cascade laser: beyond the Schawlow-Townes limit
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A comprehensive investigation of the frequency-noise spectral density of a free-running mid-infrared quantum-cascade laser is presented for the first time. It provides direct evidence of the leveling of this noise down to a white noise plateau, corresponding to an intrinsic linewidth of a few hundred Hz. The experiment is in agreement with the most recent theory on the fundamental mechanism of line broadening in quantum-cascade lasers, which provides a new insight into the Schawlow-Townes formula and predicts a narrowing beyond the limit set by the radiative lifetime of the upper level.
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Due to their high coherence, Lasers are a ubiquitous tool in science. The standard quantum limit for the phase coherence time was first introduced by [A. Schawlow and C. Townes, Phys. Rev. 112, 1940 (1958)], who showed that the minimum possible laser linewidth is determined by the linewidth of the laser cavity divided by twice the number of photons in the cavity. Later, Wiseman showed theoretically that by using Susskind-Glogower (SG) operators to couple the gain medium to the laser cavity it is possible to eliminate pump noise, but not loss noise. This decreases the minimum laser linewidth, though only by a factor of two. In this article, we show that by engineering the coupling between the laser cavity and the output port it is possible to eliminate most of the loss noise as well and construct a laser that has a vastly narrower linewidth, narrower than the standard quantum limit by a factor equal to the number of photons in the laser cavity. We establish a roadmap for building such a device in the laboratory by using Josephson junctions and linear circuit elements to build coupling circuits that behave like SG operators for a range of cavity photon occupancies and using them to couple the laser cavity to both the gain medium and the output port. This device could be an ultra-coherent, cryogenic light source for microwave quantum information experiments. Further, our laser provides highly squeezed light and could be modified to provide designer quantum light which is an important resource for CV/linear optical quantum computing, readout of quantum states in superconducting quantum computers, quantum metrology, and quantum communication. Finally, our proposal relies on the tools and elements of superconducting quantum information, and thus is a clear example of how quantum engineering techniques can inspire us to re-imagine the limits of conventional quantum systems such as the laser.
We report the coherent phase-locking of a quantum cascade laser (QCL) at 10-$mu$m to the secondary frequency standard of this spectral region, a CO2 laser stabilized on a saturated absorption line of OsO4. The stability and accuracy of the standard are transferred to the QCL resulting in a line width of the order of 10 Hz, and leading to our knowledge to the narrowest QCL to date. The locked QCL is then used to perform absorption spectroscopy spanning 6 GHz of NH3 and methyltrioxorhenium, two species of interest for applications in precision measurements.
We propose a new light source based on having alkaline-earth atoms in an optical lattice collectively emit photons on an ultra-narrow clock transition into the mode of a high Q-resonator. The resultant optical radiation has an extremely narrow linewidth in the mHz range, even smaller than that of the clock transition itself due to collective effects. A power level of order $10^{-12}W$ is possible, sufficient for phase-locking a slave optical local oscillator. Realizing this light source has the potential to improve the stability of the best clocks by two orders of magnitude.
More and more applications require semiconductor lasers distinguished not only by large modulation bandwidths or high output powers, but also by small spectral linewidths. The theoretical understanding of the root causes limiting the linewidth is therefore of great practical relevance. In this paper, we derive a general expression for the calculation of the spectral linewidth step by step in a self-contained manner. We build on the linewidth theory developed in the 1980s and 1990s but look from a modern perspective, in the sense that we choose as our starting points the time-dependent coupled-wave equations for the forward and backward propagating fields and an expansion of the fields in terms of the stationary longitudinal modes of the open cavity. As a result, we obtain rather general expressions for the longitudinal excess factor of spontaneous emission ($K$-factor) and the effective $alpha$-factor including the effects of nonlinear gain (gain compression) and refractive index (Kerr effect), gain dispersion and longitudinal spatial hole burning in multi-section cavity structures. The effect of linewidth narrowing due to feedback from an external cavity often described by the so-called chirp reduction factor is also automatically included. We propose a new analytical formula for the dependence of the spontaneous emission on the carrier density avoiding the use of the population inversion factor. The presented theoretical framework is applied to a numerical study of a two-section distributed Bragg reflector laser.
Quantum cascade laser (QCL)-pumped molecular lasers (QPMLs) have recently been introduced as a new source of powerful (>1 mW), tunable (>1 THz), narrow-band (<10 kHz), continuous-wave terahertz radiation. The performance of these lasers depends critically on molecular collision physics, pump saturation, and on the design of the laser cavity. Using a validated three-level model that captures the essential collision and saturation behaviors of the QPML gas nitrous oxide (N2O),we explore how threshold pump power and output terahertz power depend on pump power, gas pressure, as well as on the diameter, length, and output-coupler transmissivity of a cylindrical cavity.The analysis indicates that maximum power occurs as pump saturation is minimized in a manner that depends much more sensitively on pressure than on cell diameter, length, or transmissivity. A near-optimal compact laser cavity can produce more than 10 mW of power tunable over frequencies above 1 THz when pumped by a multi-watt QCL.
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