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We show that Rydberg states in an ultra-cold gas can be excited with strongly preferred nearest-neighbor distance if densities are well below saturation. The scheme makes use of an echo sequence in which the first half of a laser pulse excites Rydberg states while the second half returns atoms to the ground state, as in the experiment of Raitzsch et al. [Phys. Rev. Lett. 100 (2008) 013002]. Near to the end of the echo sequence, almost any remaining Rydberg atom is separated from its next-neighbor Rydberg atom by a distance slightly larger than the instantaneous blockade radius half-way through the pulse. These correlations lead to large deviations of the atom counting statistics from a Poissonian distribution. Our results are based on the exact quantum evolution of samples with small numbers of atoms. We finally demonstrate the utility of the omega-expansion for the approximate description of correlation dynamics through an echo sequence.
We manipulate correlations between Rydberg excitations in cold atom samples using a rotary-echo technique. The correlations are due to interactions between the Rydberg atoms. In the rotary-echo excitation sequence, the phase of the excitation pulse is flipped at a selected time during the pulse. We measure the resultant change in the spatial pair correlation function of the excitations via direct position-sensitive atom imaging. For zero detuning of the lasers from the interaction-free Rydberg-excitation resonance, the pair-correlation value at the most likely nearest-neighbor Rydberg-atom distance is substantially enhanced when the phase is flipped at the middle of the excitation pulse. In this case, the rotary echo eliminates most uncorrelated (un-paired) atoms, leaving an abundance of correlated atom pairs at the end of the sequence. In off-resonant cases, a complementary behavior is observed. We further characterize the effect of the rotary-echo excitation sequence on the excitation-number statistics of the atom sample.
We report the creation of an interacting cold Rydberg gas of strontium atoms. We show that the excitation spectrum of the inner valence electron is sensitive to the interactions in the Rydberg gas, even though they are mediated by the outer Rydberg electron. By studying the evolution of this spectrum we observe density-dependent population transfer to a state of higher angular momentum l. We determine the fraction of Rydberg atoms transferred, and identify the dominant transfer mechanism to be l-changing electron-Rydberg collisions associated with the formation of a cold plasma.
One of the most striking features of the strong interactions between Rydberg atoms is the dipole blockade effect, which allows only a single excitation to the Rydberg state within the volume of the blockade sphere. Here we present a method that spatially visualizes this phenomenon in an inhomogeneous gas of ultra-cold rubidium atoms. In our experiment we scan the position of one of the excitation lasers across the cold cloud and determine the number of Rydberg excitations detected as a function of position. Comparing this distribution to the one obtained for the number of ions created by a two-photon ionization process via the intermediate 5P level, we demonstrate that the blockade effect modifies the width of the Rydberg excitation profile. Furthermore, we study the dynamics of the Rydberg excitation and find that the timescale for the excitation depends on the atomic density at the beam position.
In this paper we study the density noise correlations of the two component Fermi gas in optical lattices. Three different type of phases, the BCS-state (Bardeen, Cooper, and Schieffer), the FFLO-state (Fulde, Ferrel, Larkin, and Ovchinnikov), and BP (breach pair) state, are considered. We show how these states differ in their noise correlations. The noise correlations are calculated not only at zero temperature, but also at non-zero temperatures paying particular attention to how much the finite temperature effects might complicate the detection of different phases. Since one-dimensional systems have been shown to be very promising candidates to observe FFLO states, we apply our results also to the computation of correlation signals in a one-dimensional lattice. We find that the density noise correlations reveal important information about the structure of the underlying order parameter as well as about the quasiparticle dispersions.
In the laser excitation of ultracold atoms to Rydberg states, we observe a dramatic suppression caused by van der Waals interactions. This behavior is interpreted as a local excitation blockade: Rydberg atoms strongly inhibit excitation of their neighbors. We measure suppression, relative to isolated atom excitation, by up to a factor of 6.4. The dependence of this suppression on both laser irradiance and atomic density are in good agreement with a mean-field model. These results are an important step towards using ultracold Rydberg atoms in quantum information processing.