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Register a new userExtremely Large and Anisotropic Upper Critical Field and the Ferromagnetic Instability in UCoGe
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Magnetoresistivity measurements with fine tuning of the field direction on high quality single crystals of the ferromagnetic superconductor UCoGe show anomalous anisotropy of the upper critical field H_c2. H_c2 for H // b-axis (H_c2^b) in the orthorhombic crystal structure is strongly enhanced with decreasing temperature with an S-shape and reaches nearly 20 T at 0 K. The temperature dependence of H_c2^a shows upward curvature with a low temperature value exceeding 30 T, while H_c2^c at 0 K is very small (~ 0.6 T). Contrary to conventional ferromagnets, the decrease of the Curie temperature with increasing field for H // b-axis marked by an enhancement of the effective mass of the conduction electrons appears to be the origin of the S-shaped H_c2^b curve. These results indicate that the field-induced ferromagnetic instability or magnetic quantum criticality reinforces superconductivity.
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We review our recent studies on ferromagnetic superconductors, UGe2, URhGe and UCoGe, where the spin-triplet state with the so-called equal spin pairing is realized. We focus on experimental results of URhGe and UCoGe in which the superconductivity occurs already at ambient pressure. The huge upper critical field Hc2 on UCoGe for the field along the hard magnetization axis (b-axis) is confirmed by the AC susceptibility measurements by the fine tuning of field angle. Contrary to the huge Hc2 along the hard-magnetization axis, Hc2 along the easy-magnetization axis (c-axis) is relatively small in value. However, the initial slope of Hc2, namely dHc2/dT (H -> 0) both in UCoGe and in URhGe indicates the large value, which can be explained by the magnetic domain effect detected in the magnetization measurements. The specific heat measurements using a high quality single crystal of UCoGe demonstrate the bulk superconductivity, which is extended under magnetic field for the field along c-axis.
We grew single crystals of U6Co by the self-flux method and measured the magnetic susceptibility, resistivity, and specific heat. The magnetic susceptibility shows very small anisotropy and weak temperature dependence, indicating small spin-susceptibility. Superconductivity was clearly observed in the resistivity, susceptibility, and specific heat at Tc~2.3K. The upper critical field was remarkably large, 7.9 and 6.6T for H || [001] and [110], respectively, in the tetragonal structure, indicating that the ellipsoidal Fermi surface is slightly suppressed along the [001] direction according to the effective mass model. The specific heat shows a large jump at Tc with Delta C/gamma Tc = 1.58, and the field dependence of the specific heat at low temperatures shows an almost linear increase. These experimental results are well explained by the BCS model in the dirty limit condition. U6Co is most likely a conventional s-wave superconductor with a full superconducting gap.
A $^{59}$Co nuclear quadrupole resonance (NQR) was performed on a single-crystalline ferromagnetic (FM) superconductor UCoGe under pressure. The FM phase vanished at a critical pressure $P_c$, and the NQR spectrum just below $P_c$ showed phase separation of the FM and paramagnetic (PM) phases below Curie temperature $T_{textrm{Curie}}$, suggesting first-order FM quantum phase transition (QPT). We found that the internal field was absent above $P_c$, but the superconductivity is almost unchanged. This result suggests the existence of the nonunitary to unitary transition of the superconductivity around $P_c$. Nuclear spin-lattice relaxation rate $1/T_1$ showed the FM critical fluctuations around $P_c$, which persist above $P_c$ and are clearly related to superconductivity in the PM phase. This FM QPT is understood to be a weak first order with critical fluctuations. $1/T_1$ sharply decreased in the superconducting (SC) state above $P_c$ with a single component, in contrast to the two-component $1/T_1$ in the FM SC state, indicating that the inhomogeneous SC state is a characteristic feature of the FM SC state in UCoGe.
We present a detailed analysis of the upper critical field for CeCoIn5 under high pressure. We show that, consistently with other measurements, this system shows a decoupling between maximum of the superconducting transition temperature Tc and maximum pairing strength. This puts forward CeCoIn5 as an important paradigm for this class of unconventional, strongly correlated superconductors.
We performed AC calorimetry and magnetoresistance measurements under pressure for H || a-axis (easy-magnetization axis) in the novel heavy-fermion superconductor UTe2. Thanks to the thermodynamic information, multiple superconducting phases have been revealed under pressure and magnetic field. The (H,T) phase diagram of superconductivity under pressure displays an abrupt increase of the upper critical field (Hc2) at low temperature and in the high field region, and a strong convex curvature of Hc2 at high temperature. This behavior of Hc2 and the multiple superconducting phases require a state for the superconducting order parameter more complex than a spin-triplet equal spin pairing. Above the superconducting critical pressure, Pc, we find strong indications that the possible magnetic order is closer to antiferromagnetism than to ferromagnetism.
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