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Register a new userA new collective phenomenon arising from spin anisotropic perturbations to a Heisenberg square lattice manifested in paramagnetic resonance experiments
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Added by
Ross David McDonald
Publication date
2009
fields
Physics
and research's language is
English
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We report unexpected behaviour in a family of Cu spin- 1/2 systems, in which an apparent gap in the low energy magneto-optical absorption spectrum opens at low temperature. This previously unreported collective phenomenon arises at temperatures where the energy of the dominant exchange interaction exceeds the thermal energy. Simulations of the observed shifts in electron paramagnetic resonance spectral weight, which include spin anisotropy, reproduce this behavior yielding the magnitude of the spin anisotropy in these compounds.
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We study the field dependence of the antiferromagnetic spin-1/2 Heisenberg model on the square lattice by means of exact diagonalizations. In a first part, we calculate the spin-wave velocity, the spin-stiffness, and the magnetic susceptibility and thus determine the microscopic parameters of the low-energy long-wavelength description. In a second part, we present a comprehensive study of dynamical spin correlation functions for magnetic fields ranging from zero up to saturation. We find that at low fields, magnons are well defined in the whole Brillouin zone, but the dispersion is substantially modified by quantum fluctuations compared to the classical spectrum. At higher fields, decay channels open and magnons become unstable with respect to multi-magnon scattering. Our results directly apply to inelastic neutron scattering experiments.
We study the quantum phase diagram and excitation spectrum of the frustrated $J_1$-$J_2$ spin-1/2 Heisenberg Hamiltonian. A hierarchical mean-field approach, at the heart of which lies the idea of identifying {it relevant} degrees of freedom, is developed. Thus, by performing educated, manifestly symmetry preserving mean-field approximations, we unveil fundamental properties of the system. We then compare various coverings of the square lattice with plaquettes, dimers and other degrees of freedom, and show that only the {it symmetric plaquette} covering, which reproduces the original Bravais lattice, leads to the known phase diagram. The intermediate quantum paramagnetic phase is shown to be a (singlet) {it plaquette crystal}, connected with the neighboring Neel phase by a continuous phase transition. We also introduce fluctuations around the hierarchical mean-field solutions, and demonstrate that in the paramagnetic phase the ground and first excited states are separated by a finite gap, which closes in the Neel and columnar phases. Our results suggest that the quantum phase transition between Neel and paramagnetic phases can be properly described within the Ginzburg-Landau-Wilson paradigm.
We report that a possible Z2 quantum spin liquid (QSL) can be observed in a new class of frustrated system: spinor bosons subject to a pi flux in a square lattice. We construct a new class of Ginsburg-Landau (GL) type of effective action to classify possible quantum or topological phases at any coupling strengths. It can be used to reproduce the frustrated SF with the 4 sublattice $ 90^{circ} $ coplanar spin structure plus its excitations in the weak coupling limit and the FM Mott plus its excitations in the strong coupling limit achieved in our previous work. It also establishes deep and intrinsic connections between the GL effective action and the order from quantum disorder (OFQD) phenomena in the weak coupling limit. Most importantly, it predicts two possible new phases at intermediate couplings: a FM SF phase or a frustrated magnetic Mott phase. We argue that the latter one is more likely and melts into a $ Z_2 $ quantum spin liquid (QSL) phase. If the heating issue can be under a reasonable control at intermediate couplings $ U/t sim 1 $, the topological order of the $ Z_2 $ QSL maybe uniquely probed by the current cold atom or photonic experimental techniques.
Cu(C$_8$H$_6$N$_2$)Cl$_2$, a strong-rung spin-1/2 Heisenberg ladder compound, is probed by means of electron spin resonance (ESR) spectroscopy in the field-induced gapless phase above $H_{c1}$. The temperature dependence of the ESR linewidth is analyzed in the quantum field theory framework, suggesting that the anisotropy of magnetic interactions plays a crucial role, determining the peculiar low-temperature ESR linewidth behavior. In particular, it is argued that the uniform Dzyaloshinskii-Moriya interaction (which is allowed on the bonds along the ladder legs) can be the source of this behavior in Cu(C$_8$H$_6$N$_2$)Cl$_2$.
We develop a simple and unbiased numerical method to obtain the uniform susceptibility of quantum many body systems. When a Hamiltonian is spatially deformed by multiplying it with a sine square function that smoothly decreases from the system center toward the edges, the size-scaling law of the excitation energy is drastically transformed to a rapidly converging one. Then, the local magnetization at the system center becomes nearly size independent; the one obtained for the deformed Hamiltonian of a system length as small as L=10 provides the value obtained for the original uniform Hamiltonian of L=100. This allows us to evaluate a bulk magnetic susceptibility by using the magnetization at the center by existing numerical solvers without any approximation, parameter tuning, or the size-scaling analysis. We demonstrate that the susceptibilities of the spin-1/2 antiferromagnetic Heisenberg chain and square lattice obtained by our scheme at L=10 agree within 10 to (-3) with exact analytical and numerical solutions for L=infinite down to temperature of 0.1 times the coupling constant. We apply this method to the spin-1/2 kagome lattice Heisenberg antiferromagnet which is of prime interest in the search of spin liquids.
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