No Arabic abstract
We study numerically the deformation of sessile dielectric drops immersed in a second fluid when submitted to the optical radiation pressure of a continuous Gaussian laser wave. Both drop stretching and drop squeezing are investigated at steady state where capillary effects balance the optical radiation pressure. A boundary integral method is implemented to solve the axisymmetric Stokes flow in the two fluids. In the stretching case, we find that the drop shape goes from prolate to near-conical for increasing optical radiation pressure whatever the drop to beam radius ratio and the refractive index contrast between the two fluids. The semi-angle of the cone at equilibrium decreases with the drop to beam radius ratio and is weakly influenced by the index contrast. Above a threshold value of the radiation pressure, these optical cones become unstable and a disruption is observed. Conversely, when optically squeezed, the drop shifts from an oblate to a concave shape leading to the formation of a stable optical torus. These findings extend the electrohydrodynamics approach of drop deformation to the much less investigated optical domain and reveal the openings offered by laser waves to actively manipulate droplets at the micrometer scale.
The sliding of non-Newtonian drops down planar surfaces results in a complex, entangled balance between interfacial forces and non linear viscous dissipation, which has been scarcely inspected. In particular, a detailed understanding of the role played by the polymer flexibility and the resulting elasticity of the polymer solution is still lacking. To this aim, we have considered polyacrylamide (PAA) solutions of different molecular weights, suspended either in water or glycerol/water mixtures. In contrast to drops with stiff polymers, drops with flexible polymers exhibit a remarkable elongation in steady sliding. This difference is most likely attributed to different viscous bending as a consequence of different shear thinning. Moreover, an optimal elasticity of the polymer seems to be required for this drop elongation to be visible. We have complemented experimental results with numerical simulations of a viscoelastic FENE-P drop. This has been a decisive step to unravel how a change of the elastic parameters (e.g. polymer relaxation time, maximum extensibility) affects the dimensionless sliding velocity.
Sessile drops of soft hydrogels were vibrated vertically by subjecting them to a mechanically induced Gaussian white noise. Power spectra of the surface fluctuation of the gel allowed identification of its resonant frequency that decreases with their mass, but increases with its shear modulus. The principal resonant frequencies of the spheroidal modes of the gel of shear moduli ranging from 55 Pa to 290 Pa were closest to the lowest Rayleigh mode of vibration of a drop of pure water. These observations coupled with the fact that the resonance frequency varies inversely as the square root of the mass in all cases suggest that they primarily correspond to the capillary (or a pseudo-capillary) mode of drop vibration. The contact angles of the gel drops also increase with the modulus of the gel. When the resonance frequencies are corrected for the wetting angles, and plotted against the fundamental frequency scale (gamma/mu)^0.5, all the data collapse nicely on a single plot provided that the latter is shifted by a shear modulus dependent factor (1+mu.L/gamma). A length scale L, independent of both the modulus and the mass of the drop emerges from such a fit.
The force of electromagnetic radiation on a dielectric medium may be derived by a direct application of the Lorentz law of classical electrodynamics. While the lights electric field acts upon the (induced) bound charges in the medium, its magnetic field exerts a force on the bound currents. We use the example of a wedge-shaped solid dielectric, immersed in a transparent liquid and illuminated at Brewsters angle, to demonstrate that the linear momentum of the electromagnetic field within dielectrics has neither the Minkowski nor the Abraham form; rather, the correct expression for momentum density has equal contributions from both. The time rate of change of the incident momentum thus expressed is equal to the force exerted on the wedge plus that experienced by the surrounding liquid.
We unveil the generation of universal morphologies of fluid interfaces by radiation pressure whatever is the nature of the wave, acoustic or optical. Experimental observations reveal interface deformations endowed with step-like features that are shown to result from the interplay between the wave propagation and the shape of the interface. The results are supported by numerical simulations and a quantitative interpretation based on the waveguiding properties of the field is provided.
Using the Finite-Difference-Time-Domain (FDTD) method, we compute the electromagnetic field distribution in and around dielectric media of various shapes and optical properties. With the aid of the constitutive relations, we proceed to compute the bound charge and bound current densities, then employ the Lorentz law of force to determine the distribution of force-density within the regions of interest. For a few simple cases where analytical solutions exist, these solutions are found to be in complete agreement with our numerical results. We also analyze the distribution of fields and forces in more complex systems, and discuss the relevance of our findings to experimental observations. In particular, we demonstrate the single-beam trapping of a dielectric micro-sphere immersed in a liquid under conditions that are typical of optical tweezers.