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Carbon isotope measurements in the Solar System

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 Added by Paul Woods
 Publication date 2009
  fields Physics
and research's language is English




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I make publicly available my literature study into carbon isotope ratios in the Solar System, which formed a part of Woods & Willacy (2009). As far as I know, I have included here all measurements of 12C/13C in Solar System objects (excluding those of Earth) up to and including 1 February 2010. Full references are given. If you use the any of the information here, please reference the paper Woods & Willacy (2009) and this publication.



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Previous determinations of the oxygen isotopic ratios in AGB carbon stars were at odds with the existing theoretical predictions. We aim to redetermine the oxygen ratios in these stars using new spectral analysis tools and further develop discussions on the carbon and nitrogen isotopic ratios in order to elucidate this problem. Oxygen isotopic ratios were derived from spectra in the K-band in a sample of galactic AGB carbon stars of different spectral types and near solar metallicity. Synthetic spectra calculated in LTE with spherical carbon-rich atmosphere models and updated molecular line lists were used. The CNO isotope ratios derived in a homogeneous way, were compared with theoretical predictions for low-mass (1.5-3 M_o) AGB stars computed with the FUNS code assuming extra mixing both during the RGB and AGB phases. For most of the stars the 16O/17O/18O ratios derived are in good agreement with theoretical predictions confirming that, for AGB stars, are established using the values reached after the FDU according to the initial stellar mass. This fact, as far as the oxygen isotopic ratios are concerned, leaves little space for the operation of any extra mixing mechanism during the AGB phase. Nevertheless, for a few stars with large 16O/17O/18O, the operation of such a mechanism might be required, although their observed 12C/13C and 14N/15N ratios would be difficult to reconcile within this scenario. Furthermore, J-type stars tend to have lower 16O/17O ratios than the normal carbon stars, as already indicated in previous studies. Excluding these peculiar stars, AGB carbon stars occupy the same region as pre-solar type I oxide grains in a 17O/16O vs. 18O/16O diagram, showing little spread. This reinforces the idea that these grains were probably formed in low-mass stars during the previous O-rich phases.
Dust measurements in the outer solar system are reviewed. Only the plasma wave instrument on board Voyagers 1 and 2 recorded impacts in the Edgeworth-Kuiper belt (EKB). Pioneers 10 and 11 measured a constant dust flux of 10-micron-sized particles out to 20 AU. Dust detectors on board Ulysses and Galileo uniquely identified micron-sized interstellar grains passing through the planetary system. Impacts of interstellar dust grains onto big EKB objects generate at least about a ton per second of micron-sized secondaries that are dispersed by Poynting-Robertson effect and Lorentz force. We conclude that impacts of interstellar particles are also responsible for the loss of dust grains at the inner edge of the EKB. While new dust measurements in the EKB are in an early planning stage, several missions (Cassini and STARDUST) are en route to analyze interstellar dust in much more detail.
We investigate the gas-phase and grain-surface chemistry in the inner 30 AU of a typical protoplanetary disk using a new model which calculates the gas temperature by solving the gas heating and cooling balance and which has an improved treatment of the UV radiation field. We discuss inner-disk chemistry in general, obtaining excellent agreement with recent observations which have probed the material in the inner regions of protoplanetary disks. We also apply our model to study the isotopic fractionation of carbon. Results show that the fractionation ratio, 12C/13C, of the system varies with radius and height in the disk. Different behaviour is seen in the fractionation of different species. We compare our results with 12C/13C ratios in the Solar System comets, and find a stark contrast, indicative of reprocessing.
We report on single-wall carbon nanotube (SWCNT) specific $^{13}$C isotope enrichment. The high temperature annealing of isotope enriched fullerenes encapsulated in SWCNTs yields double-wall carbon nanotubes (DWCNTs) with a high isotope enrichment of the inner wall. The vibrational spectra evidences that no carbon exchange occurs between the two walls. The method facilitates the identification of the Raman signal of the outer and inner tubes. Nuclear magnetic resonance proves the significant contrast of the isotope enriched SWCNTs as compared to other carbon phases, and provides information on the electronic properties of the small diameter inner tubes of the DWCNTs.
In the present work we study evolution of magnetic helicity in the solar corona. We compare the rate of change of a quantity related to the magnetic helicity in the corona to the flux of magnetic helicity through the photosphere and find that the two rates are similar. This gives observational evidence that helicity flux across the photosphere is indeed what drives helicity changes in solar corona during emergence. For the purposes of estimating coronal helicity we neither assume a strictly linear force-free field, nor attempt to construct a non-linear force-free field. For each coronal loop evident in Extreme Ultraviolet (EUV) we find a best-matching line of a linear force-free field and allow the twist parameter alpha to be different for each line. This method was introduced and its applicability was discussed in Malanushenko et. al. (2009). The object of the study is emerging and rapidly rotating AR 9004 over about 80 hours. As a proxy for coronal helicity we use the quantity <alpha_i*L_i/2> averaged over many reconstructed lines of magnetic field. We argue that it is approximately proportional to flux-normalized helicity H/Phi^2, where H is helicity and Phi is total enclosed magnetic flux of the active region. The time rate of change of such quantity in the corona is found to be about 0.021 rad/hr, which is compatible with the estimates for the same region obtained using other methods Longcope et. al. (2007), who estimated the flux of normalized helicity of about 0.016 rad/hr.
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