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Laser frequency stabilization to highly excited state transitions using electromagnetically induced transparency in a cascade system

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 Added by Richard Abel
 Publication date 2009
  fields Physics
and research's language is English




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We demonstrate laser frequency stabilization to excited state transitions using cascade electromagnetically induced transparency (EIT). Using a room temperature Rb vapor cell as a reference, we stabilize a first diode laser to the D2 transition and a second laser to a transition from the intermediate state to a Rydberg state with principal quantum number n=19 - 70. A combined laser linewidth of 280 kHz over a 0.1 ms time period is achieved. This method may be applied generally to any cascade system and allows laser stabilization to an atomic reference in the absence of strong optical transitions.



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We propose a sub-Doppler laser cooling mechanism that takes advantage of the unique spectral features and extreme dispersion generated by the phenomenon of electromagnetically induced transparency (EIT). EIT is a destructive quantum interference phenomenon experienced by atoms with multiple internal quantum states when illuminated by laser fields with appropriate frequencies. By detuning the lasers slightly from the dark resonance, we observe that, within the transparency window, atoms can be subject to a strong viscous force, while being only slightly heated by the diffusion caused by spontaneous photon scattering. In contrast to other laser cooling schemes, such as polarization gradient cooling or EIT-sideband cooling, no external magnetic field or strong external confining potential is required. Using a semiclassical approximation, we derive analytically quantitative expressions for the steady-state temperature, which is confirmed by full quantum mechanical numerical simulations. We find that the lowest achievable temperatures approach the single-photon recoil energy. In addition to dissipative forces, the atoms are subject to a stationary conservative potential, leading to the possibility of spatial confinement. We find that under typical experimental parameters this effect is weak and stable trapping is not possible.
Electromagnetically induced transparency (EIT) is a well-known phenomenon due in part to its applicability to quantum devices such as quantum memories and quantum gates. EIT is commonly modeled with a three-level lambda system due to the simplicity of the calculations. However, this simplified model does not capture all the physics of EIT experiments with real atoms. We present a theoretical study of the effect of two closely-spaced excited states on EIT and off-resonance Raman transitions. We find that the coherent interaction of the fields with two excited states whose separation is smaller than their Doppler broadened linewidth can enhance the EIT transmission and broaden the width of the EIT peak. However, a shift of the two-photon resonance frequency for systems with transitions of unequal dipole strengths leads to a reduction of the maximum transparency that can be achieved when Doppler broadening is taken into account even under ideal conditions of no decoherence. As a result, complete transparency cannot be achieved in a vapor cell. Only when the separation between the two excited states is of the order of the Doppler width or larger can complete transparency be recovered. In addition, we show that off-resonance Raman absorption is enhanced and its resonance frequency is shifted. Finally, we present experimental EIT measurements on the D1 line of $^{85}$Rb that agree with the theoretical predictions when the interaction of the fields with the four levels is taken into account.
119 - O.S. Mishina 2011
Electromagnetically induced transparency (EIT) has mainly been modelled for three-level systems. In particular, a considerable interest has been dedicated to the Lambda-configuration, with two ground states and one excited state. However, in the alkali-metal atoms, which are commonly used, hyperfine interaction in the excited state introduces several levels which simultaneously participate in the scattering process. When the Doppler broadening is comparable with the hyperfine splitting in the upper state, the three-level Lambda model does not reproduce the experimental results. Here we theoretically investigate the EIT in a hot vapor of alkali-metal atoms and demonstrate that it can be strongly reduced due to the presence of multiple excited levels. Given this model, we also show that a well-designed optical pumping enables to significantly recover the transparency.
The broadband parametric fluorescence pulse (probe light) with center frequency resonant on 87Rb D1 line was injected into a cold atomic ensemble with coherent light (control light). Due to the low gain in the parametric down conversion process, the probe light was in a highly bunched photon-pair state. By switching off the control light, the probe light within the electromagnetically induced transparency window was mapped on the atoms. When the control light was switched on, the probe light was retrieved and frequency filtered storage was confirmed from the superbunching effect and an increase of the coherence time of the retrieved light.
We report on the all-optical detection of Rydberg states in a effusive atomic beam of strontium atoms using electromagnetically induced transparency (EIT). Using narrow-linewidth CW lasers we obtain an EIT linewidth of 5 MHz. To illustrate the high spectroscopic resolution offered by this method, we have measured isotope shifts of the 5s18d ^1D_2 and 5s19s ^1S_0 Rydberg states. This technique could be applied to high-resolution, non-destructive measurements of ultra-cold Rydberg gases and plasmas.
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