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Register a new userPressure-induced quenching of the charge-density-wave state observed by x-ray diffraction
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We report an x-ray diffraction study on the charge-density-wave (CDW) LaTe$_3$ and CeTe$_3$ compounds as a function of pressure. We extract the lattice constants and the CDW modulation wave-vector, and provide direct evidence for a pressure-induced quenching of the CDW phase. We observe subtle differences between the chemical and mechanical compression of the lattice. We account for these with a scenario where the effective dimensionality in these CDW systems is dependent on the type of lattice compression and has a direct impact on the degree of Fermi surface nesting and on the strength of fluctuation effects.
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We investigate the thermal-driven charge density wave (CDW) transition of two cubic superconducting intermetallic systems Lu(Pt1-xPdx)2In and (Sr1-xCax)3Ir4Sn13 by means of x-ray diffraction technique. A detailed analysis of the CDW modulation superlattice peaks as function of temperature is performed for both systems as the CDW transition temperature T_CDW is suppressed to zero by an non-thermal control parameter. Our results indicate an interesting crossover of the classical thermal-driven CDW order parameter critical exponent from a three-dimensional universality class to a mean-field tendency, as T_CDW vanishes. Such behavior might be associated with presence of quantum fluctuations which influences the classical second-order phase transition, strongly suggesting the presence of a quantum critical point (QCP) at T_CDW = 0. This also provides experimental evidence that the effective dimensionality exceeds its upper critical dimension due to a quantum phase transition.
Incommensurate charge density waves (CDW) have the extraordinary ability to display non-Ohmic behavior when submitted to an external field. The mechanism leading to this non trivial dynamics is still not well understood, although recent experimental studies tend to prove that it is due to solitonic transport. Solitons could come from the relaxation of the strained CDW within an elastic-to-plastic transition. However, the nucleation process and the transport of these charged topological objects have never been observed at the local scale until now. In this letter, we use in-situ scanning x-ray micro-diffraction with micrometer resolution of a NbSe$_3$ sample designed to have sliding and non-sliding areas. Direct imaging of the charge density wave deformation is obtained using an analytical approach based on the phase gradient to disentangle the transverse from the longitudinal components over a large surface of a hundred microns size. We show that the CDW dissociates itself from the host lattice in the sliding regime and displays a large transverse deformation, ten times larger than the longitudinal one and strongly dependent on the amplitude and the direction of the applied currents. This deformation continuously extends across the macroscopic sample dimensions, over a distance 10 000 times greater than the CDW wavelength despite the presence of strong defects while remaining strongly pinned by the lateral surfaces. This 2D quantitative study highlights the prominent role of shear effect that should play a significant role in the nucleation of solitons.
We report on the study of a magnetic dislocation in pure chromium. Coherent x-ray diffraction profiles obtained on the incommensurate Spin Density Wave (SDW) reflection are consistent with the presence of a dislocation of the magnetic order, embedded at a few micrometers from the surface of the sample. Beyond the specific case of magnetic dislocations in chromium, this work may open up a new method for the study of magnetic defects embedded in the bulk.
We investigated the effect of application of hydrostatic pressure on the charge-density wave (CDW) state in Lu(Pt$_{1-x}$Pd$_x$)$_2$In by electrical-resistivity measurements. In Lu(Pt$_{0.7}$Pd$_{0.3}$)$_{2}$In we find an increase of the CDW transition temperature upon application of pressure, which is not expected based on simple volume arguments, but in line with results of a theoretical work by Kim et al. [Phys. Rev. Lett. 125, 157001 (2020).]. Combining experimental and theoretical results suggests the existence of a CDW quantum critical point in stoichiometric LuPd$_2$In around $papprox20$ GPa.
We report pressure evolution of charge density wave (CDW) order and emergence of superconductivity (SC) in 1T-VSe2 single crystal by studying resistance and magnetoresistance behavior under high pressure. With increasing quasi-hydrostatic pressure the CDW order enhances with increase ofthe ordering temperature up to 240K at 12 GPa. Upon further increase of pressure, the resistance anomaly due to CDW order gets suppressed drastically and superconductivity emerges at ~15 GPa, with the onset critical temperature (Tc) ~ 4K. The pressure dependence of Tc is found negligible, different from the significant increase or a dome-shape seen in iso-structural layered diselenide superconductors. The high pressure magnetoresistance and Hall measurements suggest successive electronic structural changes with Fermi surface modifications at 6 GPa and 12GPa. From the observed negative magnetoresistance in this pressure range and absence of coexisting CDW and SC phases, we propose that intra-layer spin-fluctuation can play a role in the emergence of superconductivity in the high pressure phase.
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