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Register a new userHybrid resonant phenomenon in a metamaterial structure with integrated resonant magnetic material
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We explore the hybridization of fundamental material resonances with the artificial resonances of metamaterials. A hybrid structure is presented in the waveguide environment that consists of a resonant magnetic material with a characteristic tuneable gyromagnetic response that is integrated into a complementary split ring resonator (CSRR) metamaterial structure. The combined structure exhibits a distinct hybrid resonance in which each natural resonance of the CSRR is split into a lower and upper resonance that straddle the frequency for which the magnetic materials permeability is zero. We provide an analytical understanding of this hybrid resonance and define an effective medium theory for the combined structure that demonstrates good agreement with numerical electromagnetic simulations. The designed structure demonstrates the potential for using a ferrimagnetic or ferromagnetic material as a means of creating a tunable metamaterial structure.
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The Raman effect -- inelastic scattering of light by lattice vibrations (phonons) -- produces an optical response closely tied to a materials crystal structure. Here we show that resonant optical excitation of IR and Raman phonons gives rise to a Raman scattering effect that can induce giant shifts to the refractive index and induce new optical constants that are forbidden in the equilibrium crystal structure. We complete the description of light-matter interactions mediated by coupled IR and Raman phonons in crystalline insulators -- currently the focus of numerous experiments aiming to dynamically control material properties -- by including a forgotten pathway through the nonlinear lattice polarizability. Our work expands the toolset for control and development of new optical technologies by revealing that the absorption of light within the terahertz gap can enable control of optical properties of materials over a broad frequency range.
We present a new class of artificial materials which exhibit a tailored response to the electrical component of electromagnetic radiation. These electric metamaterials (EM-MMs) are investigated theoretically, computationally, and experimentally using terahertz time-domain spectroscopy. These structures display a resonant response including regions of negative permittivity (epsilon < 0) ranging from ~500 GHz to 1 THz. Conventional electric media such as distributed wires are difficult to incorporate into metamaterials. In contrast, these new localized structures will simplify the construction of future metamaterials - including those with negative index of refraction - and will enhance the design and fabrication of functional THz devices.
We propose herein a method of material-structure integrated design for broadband absorption of dielectric metamaterial, which is achieved by combination of genetic algorithm and simulation platform. A multi-layered metamaterial absorber with an ultra-broadband absorption from 5.3 to 18 GHz (a relative bandwidth of as high as 109%) is realized numerically and experimentally. In addition, simulated results demonstrate the proposed metamaterial exhibits good incident angle and polarization tolerance, which also are significant criteria for practical applications. By investigating the working principle with theoretical calculation and numerical simulation, it can be found that merging of multiple resonance modes encompassing quarter-wavelength interference cancellation, spoof surface plasmon polariton mode, dielectric resonance mode and grating mode is responsible for a remarkable ultra-broadband absorption. Analysis of respective contribution of material and structure indicates that either of them plays an indispensable role in activating different resonance modes, and symphony of material and structure is essential to afford desirable target performance. The material-structure integrated design philosophy highlights the superiority of coupling material and structure and provides an effective comprehensive optimization strategy for dielectric metamaterials.
We validate that off-resonant electron transport across {it ultra-short} oligomer molecular junctions is characterised by a conductance which decays exponentially with length, and we discuss a method to determine the damping factor via the energy spectrum of a periodic structure as a function of complex wavevector. An exact mapping to the complex wavevector is demonstrated by first-principle-based calculations of: a) the conductance of molecular junctions of phenyl-ethynylene wires covalently bonded to graphitic ribbons as a function of the bridge length, and b) the complex-band structure of poly-phenyl-ethynylene.
Resonant Raman spectra (RRS) of O-H and O-D vibration and libration modes, their combinations and higher harmonics have been observed in LiTaO3 polycrystalline thin films. RRS peaks are superimposed on photoluminescence (PL) spectrum. Monochromatic light from a xenon lamp is used as excitation source. PL spectrum shows two broad peaks, first near the band gap in UV (4.4-4.8eV) and another in the sub band gap region (< 4.0 eV). Band gap PL along with RRS peaks are reported for the first time. Photoluminescence excitation spectrum (PLE) shows a peak at 4.8 eV. Peak positions and full width at half maximum (FWHM) of RRS peaks depend upon the excitation energy. Dispersions of the fundamental and the third harmonic of the stretching mode of O-H with excitation energy are about 800 cm-1/eV and 2000 cm-1/eV respectively. This dispersion is much higher than reported in any other material.
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