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Register a new userSpin and density excitations in the triangular-lattice $t$-$J$ model with multiple-spin exchange interactions: $^3$He on graphite
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Using an exact diagonalization technique on small clusters, we study spin and density excitations of the triangular-lattice $t$-$J$ model with multiple-spin exchange interactions, whereby we consider anomalous properties observed in the doped Mott region of the two-dimensional liquid $^3$He adsorbed on a graphite surface. We find that the double-peak structure consistent with experiment appears in the calculated temperature dependence of the specific heat; the low-temperature sharp peak comes from the spin excitations reflecting the frustrated nature of the spin degrees of freedom and high-temperature broad peak comes from the density excitations extending over the entire band width. The clear separation in their energy scales is evident in the calculated spin and density excitation spectra. The calculated single-particle excitation spectra suggest the presence of fermionic quasiparticles dressed by the spin excitations, with an enhanced effective mass consistent with experiment.
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In our previous work [arXiv:1803.00999, Phys. Rev. Lett. 121, 046401 (2018)], we found a quantum spin liquid phase with a spinon Fermi surface in the two dimensional spin-1/2 Heisenberg model with four-spin ring exchange on a triangular lattice. In this work we dope the spinon Fermi surface phase by studying the $t$-$J$ model with four-spin ring exchange. We perform density matrix renormalization group calculations on four-leg cylinders of a triangular lattice and find that the dominant pair correlation function is that of a pair density wave; i.e., it is oscillatory while decaying with distance with a power law. The doping dependence of the period is studied. This is the first example where pair density wave is the dominant pairing in a generic strongly interacting system where the pair density wave cannot be explained as a composite order and no special symmetry is required.
Spin-spin relaxation time ($T_2$) and magnetic susceptibility ($chi$) of the second layer $^3$He adsorbed on Grafoil, exfoliated graphite, preplated with a monolayer $^4$He are studied by pulsed-NMR in a density range of $0.68 leq rho leq 5.28$ nm$^{-2}$. The temperature dependence of $chi(T)$ and $chi(T = 0)$ show Fermi fluid behaviour and no evidence of self-condensation are found even at the lowest density $rho = 0.68$ nm$^{-2}$. Density dependence of $T_2$ at $f = 5.5$ MHz shows a broad maximum of 5.7 ms around $rho = 3$ nm$^{-2}$. Since the decrease of $T_2$ in dilute side can not be expected in the ideal 2D fluid, it can be understood as the relaxation caused by a small amount of solid $^3$He at heterogeneity of the substrate. We also measured the Larmor frequency dependence of $T_2$ at $rho = 5.28$ nm$^{-2}$. $1/T_2$ has a $f$-linear dependence similarly to the earlier study on a first layer solid $^3$He. From a comparison between our result and the earlier one, this linearity is almost independent of the particle motion. Now, it could be caused by a microscopic magnetic field inhomogeneity arisen from the mosaic angle spread and diamagnetism of the graphite substrate.
We present a spin-rotation-invariant Green-function theory for the dynamic spin susceptibility in the spin-1/2 antiferromagnetic t-J Heisenberg model on the honeycomb lattice. Employing a generalized mean-field approximation for arbitrary temperatures and hole dopings, the electronic spectrum of excitations, the spin-excitation spectrum and thermodynamic quantities (two-spin correlation functions, staggered magnetization, magnetic susceptibility, correlation length) are calculated by solving a coupled system of self-consistency equations for the correlation functions. The temperature and doping dependence of the magnetic (uniform static) susceptibility is ascribed to antiferromagnetic short-range order. Our results on the doping dependencies of the magnetization and susceptibility are analyzed in comparison with previous results for the t_J model on the square lattice.
We study the effects of quantum fluctuations on a non-coplanar tetrahedral spin structure, which has a scalar chiral order, in the spin-1/2 multiple-spin exchange model with up to the six-spin exchange interactions on a triangular lattice. We find that, in the linear spin-wave approximation, the tetrahedral structure survives the quantum fluctuations because spin waves do not soften in the whole parameter region of the tetrahedral-structure phase evaluated for the classical system. In the quantum corrections to the ground-state energy, sublattice magnetization, and scalar chirality, the effects of the quantum fluctuations are small for the ferromagnetic nearest-neighbor interactions and for the strong five-spin interactions. The six-spin interactions have little effect on the quantum corrections in the tetrahedral-structure phase. This calculation also corrects an error in the previously reported value of scalar chirality for the spin-1/2 multiple-spin exchange model with up to the four-spin exchange interactions.
Starting from exact expression for the dynamical spin susceptibility in the time-dependent density functional theory a controversial issue about exchange interaction parameters and spin-wave excitation spectra of itinerant electron ferromagnets is reconsidered. It is shown that the original expressions for exchange integrals based on the magnetic force theorem (J. Phys. F14 L125 (1984)) are optimal for the calculations of the magnon spectrum whereas static response function is better described by the ``renormalized magnetic force theorem by P. Bruno (Phys. Rev. Lett. 90, 087205 (2003)). This conclusion is confirmed by the {it ab initio} calculations for Fe and Ni.
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