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Distillation of Liquid Xenon to Remove Krypton

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 Added by Masayuki Nakahata
 Publication date 2009
  fields Physics
and research's language is English




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A high performance distillation system to remove krypton from xenon was constructed, and a purity level of Kr/Xe = $sim 3 times 10^{-12}$ was achieved. This development is crucial in facilitating high sensitivity low background experiments such as the search for dark matter in the universe.



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The XENON1T experiment aims for the direct detection of dark matter in a cryostat filled with 3.3 tons of liquid xenon. In order to achieve the desired sensitivity, the background induced by radioactive decays inside the detector has to be sufficiently low. One major contributor is the $beta$-emitter $^{85}$Kr which is an intrinsic contamination of the xenon. For the XENON1T experiment a concentration of natural krypton in xenon $rm{^{nat}}$Kr/Xe < 200 ppq (parts per quadrillion, 1 ppq = 10$^{-15}$ mol/mol) is required. In this work, the design of a novel cryogenic distillation column using the common McCabe-Thiele approach is described. The system demonstrated a krypton reduction factor of 6.4$cdot$10$^5$ with thermodynamic stability at process speeds above 3 kg/h. The resulting concentration of $rm{^{nat}}$Kr/Xe < 26 ppq is the lowest ever achieved, almost one order of magnitude below the requirements for XENON1T and even sufficient for future dark matter experiments using liquid xenon, such as XENONnT and DARWIN.
71 - Rui Yan , Zhou Wang , Xiangyi Cui 2021
An efficient cryogenic distillation system was designed and constructed for PandaX-4T dark matter detector based on the McCabe-Thiele (M-T) method and the conservation of mass and energy. This distillation system is designed to reduce the concentration of krypton in commercial xenon from 5X$10^{-7}$ mol/mol to $10^{-14}$ mol/mol with 99% xenon collection efficiency at a maximum flow rate of 10 kg/h. The offline distillation operation has been completed and 5.75 tons of ultra-high purity xenon was produced, which is used as the detection medium in PandaX-4T detector. The krypton concentration of the product xenon is measured with an upper limit of 8.0 ppt. The stability and purification performance of the cryogenic distillation system are studied by analyzing the experimental data, which is important for theoretical research and distillation operation optimization.
154 - K. Ni , R. Hasty , T. M. Wongjirad 2007
We report the preparation of neutron-activated xenon for the calibration of liquid xenon (LXe) detectors. Gamma rays from the decay of xenon metastable states, produced by fast neutron activation, were detected and their activities measured in a LXe scintillation detector. Following a five-day activation of natural xenon gas with a Cf-252 (4 x 10^5 n/s) source, the activities of two gamma ray lines at 164 keV and 236 keV, from Xe-131m and Xe-129m metastable states, were measured at about 95 and 130 Bq/kg, respectively. We also observed three additional lines at 35 keV, 100 keV and 275 keV, which decay away within a few days. No long-lifetime activity was observed after the neutron activation.
The NA62 experiment at CERN SPS aims to measure the Branching Ratio of the very rare kaon decay K+ -> pi+ nu nubar collecting O(100) events with a 10% background to make a stringent test of the Standard Model. One of the main backgrounds to the proposed measurement is represented by the K+ -> pi+ pi0 decay. To suppress this background an efficient photo veto system is foreseen. In the 1-10 mrad angular region the NA48 high performance liquid krypton electromagnetic calorimeter is used. The design, implementation and current status of the Liquid Krypton Electromagnetic Calorimeter Level 0 Trigger are presented.
138 - K. Ueshima , K. Abe , T. Iida 2008
The intensity of scintillation light emission from liquid xenon at room temperature was measured. The scintillation light yield at 1 deg. was measured to be 0.64 +/- 0.02 (stat.) +/- 0.06 (sys.) of that at -100 deg. Using the reported light yield at -100 deg. (46 photons/keV), the measured light yield at 1 deg. corresponds to 29 photons/keV. This result shows that liquid xenon scintillator gives high light yield even at room temperature.
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